Cleaning composition and process for cleaning semiconductor devices and/or tooling during manufacturing thereof
a technology for semiconductor devices and tooling, applied in the field of semiconductor device manufacturing, can solve the problems of semiconductor devices as well as cmp pads/brushes being often contaminated, inherently very dirty processes, and fragile structures
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example 1
[0040]In this example, a comparison was made between prior art cleaning chemistries and a cleaning process with an aqueous cleaning solution in accordance with the present disclosure. A cleaning solution in accordance with the present disclosure, referred to herein as dAS, was compounded in aqueous solution and included 1% (w / w) ascorbic acid in 2% (w / w) sulfuric acid as active agents. The dAS solution was used to clean a substrate including a TiN surface having a defined thickness at room temperature (25° C.) for two different immersion times: 60 seconds and 300 seconds. Following immersions, the substrates were rinsed with deionized water and dried. Thickness of the TiN layer was measured before and after cleaning. The results are shown in Table 1 below.
TABLE 1dAS Cleaning ProcessPre-ImmersionPostThicknessEtch RateThickness ofTimeThickness ofDifference(Å / SampleTiN (Å)(seconds)TiN (Å)(Å)minute)A94.886094.500.380.08B57.9230057.630.290.29
[0041]The results indicate that neither dAS ex...
example 2
[0044]In this example, we have studied the use of hot sulfuric acid as a pre-step to remove organic contamination prior to dAS cleaning. This sequence of hot sulfuric followed by dAS was also evaluated with respect to TiN loss. The process included immersing a substrate including TiN to sulfuric acid at 55° C. for 600 seconds followed by immersion to dAS at 25° C. with a subsequent deionized water rinse and drying process. The results are shown in Table 3 below.
TABLE 3Hot Sulfuric Acid / dAS Cleaning SequenceHotsulfuricaciddASTotal TiNHot sulfuricexposureexposureRemovalacid TiNdAS TiNSample(seconds)(seconds)(Å)Removal (Å)Removal (Å)G60030010.6510.570.08
[0045]As demonstrated above, the exposure of the hot sulfuric acid dominates and / or dictates the TiN removal in this process sequence. The measured TiN loss from only the hot sulfuric acid step is about 10.57 Angstroms and is similar to that observed from the soft SC1 in Example 1 that had a loss of about 10 to 15 angstroms. Thus, a com...
example 3
[0047]In this example, the cleaning solution was used to remove ceria from CMP contaminated pads. The pads were exposed to an aqueous solution of dAS as in example 1 for a period of 600 seconds followed by a 30 second deionized rinsing step.
[0048]FIGS. 1 and 2 provide scanning electron microscopy-energy dispersive spectroscopic (SEM-EDS) data, respectively, of the contaminated pad. As shown, significant deposits of ceria and ceria derivatives on the pad are clearly evident. FIGS. 3 and 4 provide SEM-EDS data, respectively, after cleaning the pad with the aqueous cleaning solution. As clearly demonstrated, no ceria signature is evident indicating that the aqueous cleaning solution was highly effective for removing ceria and ceria derivatives from the contaminated pads.
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