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Production method for controlling yttrium-barium-copper-oxygen superconducting thick film in-plane oriented growth in oxygen ambient

A technology of yttrium barium copper oxide and orientation growth, which is applied in the directions of single crystal growth, crystal growth, single crystal growth, etc., can solve problems such as few experimental data, and achieve low cost, simple process, good epitaxial orientation and crystal quality Effect

Inactive Publication Date: 2009-06-03
SHANGHAI JIAO TONG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

But it is worth noting that the predecessors' research work in this area was done in the atmospheric environment, and only YBCO superconducting thick films with pure 0° in-plane orientation could be obtained, while other types of oxygen environments Preferential growth phenomena have been studied but little experimental data

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Using the YBCO thin film with eight-fold symmetry as the seed film, the YBCO superconducting thick film with pure 45° in-plane orientation is grown by liquid phase epitaxy (the growth temperature is lower than the peritectic melting temperature 10K)

[0018] 1) with BaCO 3 +CuO powder is mixed, and the Ba / Cu atomic ratio is controlled to be 0.5;

[0019] 2) to BaCO 3 +CuO powder is ground, then calcined at 850°C for 48 hours, and sintered into a uniform Ba-Cu-O powder;

[0020] 3) Add Ba-Cu-O powder to Y placed in the furnace 2 o 3 In the crucible, heat the furnace to 40K above the peritectic melting temperature of YBCO, and keep it warm for 35 hours to melt the Ba-Cu-O powder evenly to obtain a Y-Ba-Cu-O melt;

[0021] 4) Change the atmosphere in the furnace to a 100% pure oxygen atmosphere, and keep the furnace airtight and the airflow stable;

[0022] 5) cooling the Y-Ba-Cu-O melt to 10K below the peritectic melting temperature of YBCO as the epitaxial growth te...

Embodiment 2

[0025] Using the YBCO thin film with eight-fold symmetry as the seed film, the YBCO superconducting thick film with pure 45° in-plane orientation is grown by liquid phase epitaxy (the growth temperature is 20K lower than the peritectic melting temperature)

[0026] 1) with BaCO 3 +CuO powder is mixed, and the Ba / Cu atomic ratio is controlled to be 0.6;

[0027] 2) to BaCO 3 +CuO powder is ground, then calcined at 900°C for 44 hours, and sintered into a uniform Ba-Cu-O powder;

[0028] 3) Add Ba-Cu-O powder to Y placed in the furnace 2 o3 In the crucible, heat the furnace to 35K above the peritectic melting temperature of YBCO, and keep it warm for 40 hours to melt the Ba-Cu-O powder evenly to obtain a Y-Ba-Cu-O melt;

[0029] 4) Change the atmosphere in the furnace to a 100% pure oxygen atmosphere, and keep the furnace airtight and the airflow stable;

[0030] 5) cooling the Y-Ba-Cu-O melt to 20K below the peritectic melting temperature of YBCO, as the epitaxial growth tem...

Embodiment 3

[0033] Using the YBCO thin film with eight-fold symmetry as the seed film, the YBCO superconducting thick film with pure 45° in-plane orientation is grown by liquid phase epitaxy (the growth temperature is 30K lower than the peritectic melting temperature)

[0034] 1) with BaCO 3 +CuO powder is mixed, and the Ba / Cu atomic ratio is controlled to be 0.7;

[0035] 2) to BaCO 3 +CuO powder is ground, then calcined at 950°C for 40 hours, and sintered into a uniform Ba-Cu-O powder;

[0036] 3) Add Ba-Cu-O powder to Y placed in the furnace 2 o 3 In the crucible, heat the furnace to 30K above the peritectic melting temperature of YBCO, and keep it warm for 45 hours to melt the Ba-Cu-O powder evenly to obtain a Y-Ba-Cu-O melt;

[0037] 4) Change the atmosphere in the furnace to a 100% pure oxygen atmosphere, and keep the furnace airtight and the airflow stable;

[0038] 5) cooling the Y-Ba-Cu-O melt to 30K below the peritectic melting temperature of YBCO, as the epitaxial growth t...

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Abstract

The invention relates to a preparing way for an yttrium barium copper oxygen (YBCO) superconductive thick film in form of inner-oriented growth controlled by an oxygen atmosphere. Wherein, a liquid-phase extension growth device is used to prepare YBCO film in a pure oxygen atmosphere. Ba-Cu-O powder is prepared in proportion of 0.5-0.7 of Ba / Cu atoms, which is placed in a Y2O3 crucible to heat and melt after lapping and baking, then molten Y-Ba-Cu-O is obtained. The atmosphere in an enclosed furnace is changed into pure oxygen atmosphere, the temperature of the molten Y-Ba-Cu-O is adjusted to be 10-30K lower than the melting temperature of YBCO peritectic. An YBCO film with octuplicate symmetricity is taken as a seed film, the liquid phase grows epitaxially and YBCO film with pure 45-degree inner orientation with high crystallization quality is obtained. By changing oxygen content in the atmosphere, the invention makes the former liquid-phase epitaxial process that can only prepare pure YBCO film with 0-degree inner orientation possible to get YBCO film with pure 45-degree inner orientation in a wider temperature range.

Description

technical field [0001] The invention relates to a preparation method for in-plane orientation growth of yttrium barium copper oxide superconducting thick film controlled by oxygen atmosphere. By changing the oxygen content in the liquid phase epitaxial growth environment, high-quality yttrium barium copper oxide superconducting film with specific in-plane orientation can be obtained. guide thick film. The invention belongs to the technical field of high-temperature superconducting material preparation. Background technique [0002] Since scientists discovered REBa 2 Cu 3 Oz (referred to as REBCO, rare earth barium copper oxide), a high temperature superconducting material (High Temperature Superconductor, referred to as HTS), which has great application prospects, people have focused a lot of research energy on coated superconducting materials and various superconducting related materials. Electronic devices and other directions. In the application of high-temperature su...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C30B29/22C30B19/00
Inventor 姚忻蔡衍卿
Owner SHANGHAI JIAO TONG UNIV