Supercritical oxidation process for the treatment of corrosive materials
A supercritical oxidation and supercritical technology, applied in sludge treatment, oxidation treatment of sludge, chemical instruments and methods, etc., can solve problems such as damage to the auxiliary piping system of the reactor, erosion, etc.
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Embodiment 1
[0027]Referring to FIG. 3 , the molybdenum sulfide concentrate and water are mixed with a solid:liquid ratio of 1:4 and delivered to the feed tank 25 as a slurry. From the holding tank, the slurry was pumped with pumps 26 and 27 through heaters at T = 390°C to reactors 30 and 31 . The oxidant is supplied to the reactor at a pressure of 22-25 MPa.
[0028] Under these conditions, the oxidation reaction of molybdenum sulfide occurs:
[0029] MoS 2 +3H 2 O+4.5O 2 =H 2 MoO 4 +2H 2 SO 4
[0030] The resulting slurry was transferred to the cooling chamber 31 having the above-mentioned configuration, and a cooling solution (10°C-25°C) was injected into the cooling chamber 31 . Circulation of said solution in a 2:1 ratio to the stock solution caused a rapid drop in temperature of the slurry to about 200°C.
[0031] When the concentration of the circulating sulfuric acid solution exceeds a predetermined limit, it is removed from the process to further recover the molybdenum. ...
Embodiment 2
[0033] The same experiment was performed with mixed copper sulfide (chalcopyrite). The solid:liquid ratio is 1:5, T=400°C, P=20-25MPa. As in Example 1, the cooling of the reaction was accomplished by using the circulating solution (10° C.-25° C.) as a cooling agent in a ratio of 2:1 to the original solution. Thereby, the desired temperature of the slurry, ie T2 SO 4 ;5g / l Fe;
[0034] Experiments performed have shown that cooling with a cooled circulating solution (T=10°C-25°C) lowers the temperature below 200°C while preventing corrosion in the cooling chamber and connecting parts.
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