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Preparation of plural gel water absorbent material composed of silk fibroin/acrylic acid/acrylamide

A technology of silk fibroin and acrylamide, which is applied in the field of preparation of silk fibroin/acrylic acid/acrylamide composite gel water-absorbing materials, which can solve the problems of easily polluted environment, material sources, preparation and processing costs, insufficient influence of soil structure, and not easy to degrade and other issues to achieve the effect of reducing environmental pollution

Inactive Publication Date: 2011-05-25
ZHEJIANG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] At present, although the widely used synthetic polymer water-absorbing materials have high water absorption rate, they are not easy to degrade and pollute the environment after use.
The natural polymer water-absorbing materials that have been developed include starch, cellulose, alginic acid, polylactic acid, etc., which have certain biodegradability. It has a shortpart
Except for gelatin and feathers, protein-based water-absorbing materials are less developed at present.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0022] Preparation of silk fibroin solution:

[0023] The cleaned silkworm waste cocoons were subjected to Na 2 CO 3 After boiling water degumming, use 50% CaCl by weight 2 The solution was dissolved at 98°C, filtered, dialyzed, and concentrated to obtain an SF solution with a concentration of 8%, which was set aside.

Embodiment 1

[0025] (1) Weigh 2.65g of analytically pure AA solution into a beaker, and add 1.03g of 10% (w / w) NaOH solution dropwise at room temperature of 20-30°C to make the neutralization degree of AA reach 70%; then add 1.35 g of analytically pure AM solid was stirred to obtain a mixed solution of monomer (AA / AM).

[0026] (2) Add 2g of SF into a reactor containing 25ml of distilled water, place it on a constant temperature magnetic stirrer for heating in a water bath (70°C); then add 0.072g of ammonium persulfate (APS for short), and then add monomer (AA / AM) mixed solution and 0.006g N,N'-dimethylbisacrylamide (abbreviated as MBA).

[0027] (3) Control the temperature of the water bath to 70°C, and stir while heating. When the reactant becomes gel and becomes viscous and difficult to stir, stop stirring, and then stand still. The total reaction time of stirring and standing is 2 hours.

[0028] (4) The prepared gel was taken out and washed with deionized water to obtain a hydrogel-l...

Embodiment 2

[0037] (1) Weigh 2.65g of AA solution into a beaker, and add 1.177g of 10% (w / w) NaOH solution dropwise at room temperature of 20-30°C to make the neutralization degree of AA reach 80%; then add 1.35g AM solid, after stirring, a mixed solution of monomer (AA / AM) was obtained.

[0038] (2) Add 2g of SF into a reactor containing 25ml of distilled water, place it on a constant temperature magnetic stirrer for heating in a water bath (80°C); then add 0.1g of ammonium persulfate (APS for short), and then add monomer (AA / AM) mixed solution and 0.012g N,N'-dimethylbisacrylamide (abbreviated as MBA).

[0039] (3) Control the temperature of the water bath to 80°C, and stir while heating. When the reactant becomes gel and becomes viscous and difficult to stir, stop stirring, and then stand still. The total reaction time of stirring and standing is 2 hours.

[0040] (4) The prepared gel was taken out and washed with deionized water to obtain a hydrogel-like composite water-absorbing mat...

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Abstract

The invention discloses a method for preparing plural gel water absorbent material composed of silk fibroin / acrylic acid / acrylamide, comprising the following steps: dropping NaOH solution and acrylamide solids into analytical pure acrylic acid solution to obtain mixed solution of acrylic acid / acrylamide monomer after stirring; heating silk fibroin solution water bath, then adding initiating agentammonium persulfate and the mixed solution of acrylic acid / acrylamide monomer, finally adding a cross linker N, N'-dimethyl bisacrylamide; heating and stirring to form gel, taking out the gel after standing, washing the gel by deionized water to obtain the plural gel water absorbent material composed of silk fibroin / acrylic acid / acrylamide. The material of the invention has not only hydrophile hygroscopicity but also biodegradability.

Description

technical field [0001] The invention relates to the field of processing and utilization of silk fibroin, in particular to a preparation method of a silk fibroin / acrylic acid / acrylamide composite gel water-absorbing material for water absorption and water retention. Background technique [0002] Silk fibroin (Silk Fibroin: SF) is a natural structural protein consisting of crystalline and non-crystalline regions. Because of its special molecular structure, it has hydrophilic and hygroscopic properties, biodegradability, and mechanical extension properties. The water-absorbing material base material can be prepared by extracting waste silkworm cocoons. [0003] Acrylic acid (acrylic acid: AA) is a colorless liquid, soluble in water, ethanol and ether, etc. It is used in construction, papermaking, leather, textile, daily chemical industry, water treatment and other fields with resin and synthetic rubber emulsion. Polypropylene and acrylic acid copolymers produced from acrylic ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08F289/00C08H1/00
Inventor 朱良均汪琦翀闵思佳张海萍
Owner ZHEJIANG UNIV