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Magnetically separable ferrite/expanded graphite wastewater treating agent as well as preparation method and application

A technology of wastewater treatment agent and expanded graphite, which is applied in separation methods, adsorption water/sewage treatment, combustible gas purification/transformation, etc. It can solve the problems of separation and recovery difficulties, and achieve the solution of small adsorption capacity, difficult recovery, distribution uniform effect

Active Publication Date: 2013-04-24
海宁市袁花镇工业投资有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] The purpose of the present invention is to provide a low-cost, reliable performance, convenient separation and recovery, high adsorption capacity and repeated use for the disadvantages of the current use of expanded graphite as a water treatment agent, which is difficult to separate and recover in use. Magnetically separable ferrite / expanded graphite wastewater treatment agent with high efficiency, preparation method and application

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] Example 1: ZnFe 2 o 4 Wastewater treatment agent ZnFe with a mass fraction of 0.1-0.6 2 o 4 Preparation method and application of / EG complex

[0026] 1. Wastewater treatment agent ZnFe 2 o 4 Preparation of / EG complex

[0027] ⑴Weigh a certain quality of ordinary graphite, treat the ordinary graphite with concentrated sulfuric acid or concentrated nitric acid, wash with water, and dry to obtain expandable graphite; quickly put a certain amount of expandable graphite (analytical pure) into the In the muffle furnace at ℃, take it out of the furnace quickly after 10-60s, and cool naturally to get expanded graphite (EG);

[0028] (2) Weigh 1.2-1.8g EG and ultrasonically disperse it in an appropriate amount of ethanol-distilled water mixed solvent;

[0029] ⑶ According to ZnFe 2 o 4 Mass fraction (0.1~0.6) equivalent mass (0.2~1.2g), accurately weigh 0.2468~1.4808g Zn(NO 3 ) 2 ·6H 2 O and 0.6703~4.0218g Fe(NO 3 ) 3 9H 2 O, dissolved in distilled water, added ...

Embodiment 2

[0040] Example 2: CoFe 2 o 4 Wastewater treatment agent CoFe with a mass fraction of 0.1-0.6 2 o 4 Preparation method and application of / EG complex

[0041] 1. Wastewater treatment agent CoFe 2 o 4 Preparation of / EG complex

[0042] (1) Weigh a certain quality of ordinary graphite and process it according to step (1) to obtain expanded graphite;

[0043] (2) Weigh 1.2-1.8g EG and ultrasonically disperse it in an appropriate amount of ethanol-distilled water mixed solvent;

[0044] ⑶ Press and CoFe 2 o 4 Mass fraction (0.1~0.6) equivalent mass (0.2~1.2g), accurately weigh 0.2481~1.4886g Co(NO 3 ) 2 ·6H 2 O and 0.6888~4.1328g Fe(NO 3 ) 3 9H 2 O, dissolved in distilled water, added to the solution of (2), and processed according to step (3) to obtain the precursor;

[0045] ⑷The precursor is processed according to step 4 to obtain CoFe 2 o 4 CoFe with a mass fraction of 0.1 to 0.6 2 o 4 / EG waste water treatment agent.

[0046] 2. Wastewater treatment agent ...

Embodiment 3

[0055] Example 3: MnFe 2 o 4 Wastewater treatment agent MnFe with a mass fraction of 0.1-0.6 2 o 4 Preparation method and application of / EG complex

[0056] 1. Wastewater treatment agent MnFe 2 o 4 Preparation of / EG complex

[0057] (1) Weigh a certain quality of ordinary graphite and process it according to step (1) to obtain expanded graphite;

[0058](2) Weigh 1.2-1.8g EG and ultrasonically disperse it in an appropriate amount of ethanol-distilled water mixed solvent;

[0059] ⑶ According to MnFe 2 o 4 Mass fraction (0.1~0.6) equivalent mass (0.2~1.2g), accurately weigh 0.2160~1.2961g Mn(NO 3 ) 2 4H 2 O and 0.7024~4.2143g Fe(NO 3 ) 3 9H 2 O, dissolved in distilled water, added to the solution of (2), and processed according to step (3) to obtain the precursor;

[0060] ⑷The precursor is processed according to step 4 to obtain MnFe 2 o 4 MnFe with a mass fraction of 0.1 to 0.6 2 o 4 / EG waste water treatment agent.

[0061] 2. Wastewater treatment agent...

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Abstract

The invention discloses a magnetically separable ferrite / expanded graphite wastewater treating agent as well as a preparation method and application. The magnetically separable ferrite / expanded graphite wastewater treating agent provided by the invention is a ferrite / expanded graphite compound; a preparation method of the magnetically separable ferrite / expanded graphite wastewater treating agent comprises the following steps of: carrying out acid treatment, washing, drying, high temperature treatment and naturally cooling on graphite to obtain expanded graphite; ultrasonically dispersing the expanded graphite into an ethanol-distilled water mixing solvent; weighing a transition metal salt, dissolving with distilled water, adding into a mixed solution of the expanded graphite and the ethanol-distilled water; carrying out constant-temperature stirring reaction and drying to obtain a precursor; and vacuumizing and sintering the precursor in high temperature, thereby obtaining a ferrite / expanded graphite compound. The magnetically separable ferrite / expanded graphite wastewater treating agent has the characteristics of cheap price, reliable property and high adsorption capacity and reuse efficiency, and is convenient to separate and recycle.

Description

technical field [0001] The invention relates to the technical field of magnetic materials and waste water treatment, in particular to a magnetically separable ferrite / expanded graphite waste water treatment agent and its preparation method and application. Background technique [0002] Expanded graphite is the product of ordinary graphite after high-temperature heat treatment. It has the characteristics of large specific surface area, high porosity, good adsorption performance and chemical stability. It has been widely used in environmental protection and industrial fields. For example, expanded graphite is a good water purification material, which can absorb inorganic and organic pollutants in the water phase, and can effectively remove the chroma and chemical oxygen demand of wastewater. However, when expanded graphite is used as a water treatment agent, due to its light weight and easy drift, it is difficult to separate and recover it in practical applications. At the sam...

Claims

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Application Information

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IPC IPC(8): B01J20/20B01J20/28B01J20/30B01J20/34C02F1/28
Inventor 李良超陈海峰许锋肖秋实马歌李涓碧丁艳
Owner 海宁市袁花镇工业投资有限公司