Emulsion binder, aqueous pigment ink for inkjet containing same, and method for producing emulsion binder
A manufacturing method and linking material technology, applied in the direction of copying/marking method, ink, application, etc., can solve the problem of poor ink redispersibility, etc., and achieve the effect of excellent ejection stability and low viscosity
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Embodiment 1
[0099] (Example 1: Preparation of emulsion vehicle (1))
[0100] 131.7 parts of diethylene glycol dimethyl ether (hereinafter referred to as "DMDG"), 1.0 parts of iodine, and 4.9 parts of 2,2' -Azobis(4-methoxy-2,4-dimethylvaleronitrile) (hereinafter referred to as "V-70"), 44 parts of benzyl methacrylate (hereinafter referred to as "BzMA"), 13 parts 2-Hydroxyethyl methacrylate (hereinafter referred to as "HEMA") and 0.11 parts of N-iodosuccinimide. The mixture was stirred and heated to 40°C to perform polymerization. After 3 hours, the iodine brown color disappeared. From this point of view, it was confirmed that iodine reacted with V-70, and an iodine compound (polymerization initiating compound) was generated in the reaction system. The temperature was kept constant and polymerization was further performed for 4 hours, followed by natural cooling to obtain a solution of the A polymer block.
[0101] When a part of the solution was sampled and the solid content concentra...
Embodiment 2
[0105] (Example 2: Preparation of emulsion vehicle (2))
[0106]In addition to using 362.3 parts of DMDG, 1.0 parts of iodine, 4.9 parts of V-70, 105 parts of MMA, 148.5 parts of 2-ethylhexyl methacrylate (hereinafter referred to as "2EHMA"), 45.5 parts of HEMA and 0.17 parts of diphenyl Except for methane, a solution of the A polymer block was obtained in the same manner as in Example 1 above. The polymerization rate was 80.5%. The Mn of the obtained A polymer block is 22000, the PDI is 1.56, the polymer composition is MMA / 2EHMA / HEMA≈35 / 50 / 15, the Tg calculated by theoretical calculation is 31.5°C, and the acid value is 0mgKOH / g. In addition, when a part of the sampled solution was added to water, a soft polymer was deposited. From this, it was confirmed that the obtained A polymer block was a substantially water-insoluble polymer.
[0107] Except adding a mixture of 40 parts of MMA, 17.2 parts of MAA and 0.6 parts of V-70 to the solution of the obtained A polymer block, t...
Embodiment 3
[0109] (Example 3: Preparation of emulsion vehicle (3))
[0110] In addition to using 197.1 parts of DMDG, 0.4 parts of iodine, 2.4 parts of V-70, 54 parts of MMA, 49 parts of butyl methacrylate (hereinafter referred to as "BMA"), 50 parts of dodecyl methacrylate (hereinafter referred to as "LMA"), 3 parts of MAA, and 0.1 part of di-tert-butylhydroxytoluene (hereinafter referred to as "BHT") were polymerized for 6 hours, and a solution of polymer block A was obtained in the same manner as in Example 1 above. . The polymerization rate was about 100%. The Mn of the obtained A polymer block is 30000, the PDI is 1.61, the polymer composition is MMA / BMA / LMA / MAA≈35 / 31 / 32 / 2, the Tg calculated by theoretical calculation is 7.7°C, and the acid value is 12.6mgKOH / g.
[0111] In addition, when a part of the sampled solution was added to water, a soft polymer was deposited. Since the A polymer block has a carboxyl group, it may be dissolved in alkaline water. Therefore, 0.2 g of the...
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