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Preparation method of artificial graphite anode material

A technology of artificial graphite negative electrode and graphitization treatment, applied in battery electrodes, electrical components, circuits, etc., can solve the problem that the conductive agent and artificial graphite materials cannot be in good contact, affect the coating processing performance of artificial graphite, reduce the conductive effect, etc. problems, to achieve the effect of reducing viscosity, improving processing performance, and reducing internal resistance

Active Publication Date: 2015-02-18
CNOOC TIANJIN CHEM RES & DESIGN INST +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Chinese patent CN103872288 promptly mixes conductive carbon black into artificial graphite to prepare slurry, but this method is because the conductive agent is in an independently dispersed state in the artificial graphite material, and the conductive agent and the artificial graphite material cannot be well contacted, reducing the Conductive effect
In addition, since the conductive agents are all nano-scale materials, the viscosity of the entire slurry is increased after addition, which affects the processing performance of artificial graphite coating

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] In this example, the green coke raw materials are first pulverized and spheroidized, and the mass ratio is added to the stirred tank filled with xylene according to the ratio of spheroidized green coke: polyaniline (PANI): petroleum pitch = 85:5:10 Stir evenly, evaporate and remove the solvent, then purify at 1000°C for 10 hours in a non-oxygen atmosphere, and then graphitize at 3000°C for 120 hours. The prepared artificial graphite material was assembled into an effective battery according to the conventional battery preparation process, and the internal resistance of the battery was measured to be 38.5mΩ, and the cycle number was 1400 cycles.

Embodiment 2

[0020] In this example, the green coke raw materials are first crushed and spheroidized, and the mass ratio is added to the stirred tank filled with xylene according to the ratio of spheroidized green coke: polyaniline (PANI): petroleum pitch = 97.5:0.5:2 Stir evenly, evaporate and remove the solvent, then purify at 1000°C for 10 hours in a non-oxygen atmosphere, and then graphitize at 3000°C for 120 hours. The prepared artificial graphite material was assembled into an effective battery according to the conventional battery preparation process, and the internal resistance of the battery was measured to be 40.6mΩ, and the cycle number was 1300 cycles.

Embodiment 3

[0022] In this example, the green coke raw materials are first pulverized and spheroidized, and the mass ratio is added to the stirred tank filled with xylene according to the ratio of spheroidized green coke: polyaniline (PANI): petroleum pitch = 89:3:8 Stir evenly, evaporate and remove the solvent, then purify at 1000°C for 10 hours in a non-oxygen atmosphere, and then graphitize at 3000°C for 120 hours. The prepared artificial graphite material was assembled into an effective battery according to the conventional battery preparation process, and the internal resistance of the battery was measured to be 32.4mΩ, and the cycle number was 1600 cycles.

[0023] Embodiment three

[0024] Comparative Example The green coke raw materials were pulverized and spheroidized, followed by purification at 1000°C for 10 hours in a non-oxygen atmosphere, and then graphitization at a high temperature of 3000°C for 120 hours. The prepared artificial graphite material was assembled into an ef...

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Abstract

The invention discloses a preparation method of an artificial graphite anode material of a lithium ion battery. The method comprises the following steps: after grinding and balling raw materials such as cokes, adding the balled raw materials, a conductive polymer and an adhesive into a stirring kettle filled with a solvent to uniformly stir, wherein the ratio of the conductive polymer is 0.5 to 5 percent of the total mass and the ratio of the adhesive is 2 to 10 percent of the total mass; after removing the solvent, carrying out purification for 2 to 10hr in the non-oxygen atmosphere of 800 to 1,000 DEG C; and then carrying out graphitization for not less than 24hr at a high temperature of 2,500 to 3,000 DEG C to prepare the artificial graphite anode material of which the surface is coated with a conductive material. When the artificial graphite anode material with excellent conductivity is used for the lithium ion battery, the battery has a low internal resistance and good cycling performance.

Description

technical field [0001] The invention relates to the field of lithium-ion secondary batteries, in particular to the preparation of artificial graphite as a lithium-ion battery negative electrode material. Background technique [0002] With the urgent need of low-carbon, green and circular economy, research on new energy power batteries, especially lithium-ion power batteries, has developed rapidly. Due to the advantages of high working voltage, high energy density, stable discharge voltage, good low temperature performance, small self-discharge, no memory effect, environmental friendliness and long working life, lithium-ion power batteries are widely used in pure electric vehicles and hybrid vehicles. , Large power tools. [0003] As a kind of anode material for lithium-ion batteries, artificial graphite has the characteristics of high compaction density, high capacity and good cycle performance. It is an ideal anode material for lithium-ion batteries, especially lithium-ion...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): H01M4/1393
CPCH01M4/1393Y02E60/10
Inventor 张晓波叶学海刘红光肖彩英张磊夏继平于晓微
Owner CNOOC TIANJIN CHEM RES & DESIGN INST