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A kind of preparation method of ozone catalyst for water treatment and its product and application

A catalyst and water treatment technology, applied in the field of preparation of ozone catalysts for water treatment, can solve the problems of catalyst falling off, low adsorption performance, weak bonding between catalyst and carrier, etc., and achieve the effect of increasing the active area and improving the binding force.

Active Publication Date: 2019-11-29
SHANGHAI NAT ENG RES CENT FORNANOTECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The specific surface area of ​​the ozone catalyst prepared by the granulation method is much lower than that of porous materials such as activated carbon or molecular sieve, and the adsorption performance is not high, while the impregnation method has a large specific surface area and high adsorption performance, but the catalyst is not firmly combined with the carrier. During the wastewater treatment process, a certain proportion of the catalyst will fall off from the surface of the carrier

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] A kind of preparation method of ozone catalyst for water treatment, according to the following steps:

[0024] (1) Mix zinc diacetate and ethanol at a mass ratio of 1:200 to obtain a zinc diacetate alcohol solution. Immerse the pretreated molecular sieve in the zinc diacetate alcohol solution for 0.5 h, take out the molecular sieve and dry it in an oven at 80 °C for 2 h, then impregnate it and then dry it, repeat this process for 3 times, and finally calcinate it in a muffle furnace at 300 °C for 4 h. That is, the catalyst carrier with zinc oxide film wrapped on the surface is obtained;

[0025] (2) Mix CTAB, urea, cerium nitrate, and water at a mass ratio of 1:4:20:3000, and then stir on a magnetic stirrer to obtain a colorless and transparent mixed solution; the molecular sieve wrapped with zinc oxide film and The mixed solution was transferred to a 20 mL stainless steel reactor lined with polytetrafluoroethylene, sealed, placed in an oven, heated to 120 °C for 5 h, ...

Embodiment 2

[0028] Another kind of preparation method of ozone catalyst for water treatment, according to the following steps:

[0029] (1) Mix zinc diacetate and ethanol at a mass ratio of 1:250 to obtain a zinc diacetate alcohol solution. Immerse the pretreated molecular sieve in zinc diacetate alcohol solution for 1 h, take out the molecular sieve and bake in an oven at 90 °C for 1.5 h, then impregnate and then dry, repeat this process for 3 times, and finally calcinate in a muffle furnace at 350 °C for 3 h , that is, to obtain a catalyst carrier whose surface is coated with a zinc oxide film;

[0030] (2) Mix CTAB, urea, cerium nitrate, and water at a mass ratio of 1:5:30:4000, and then stir on a magnetic stirrer to dissolve all the solutes to obtain a colorless and transparent mixed solution; the carrier and The mixed solution was transferred to a 20 mL stainless steel reactor lined with polytetrafluoroethylene, sealed, placed in an oven, heated to 140 °C for 4 h, and then naturally...

Embodiment 3

[0033] Another kind of preparation method of ozone catalyst for water treatment, according to the following steps:

[0034] (1) Mix zinc diacetate and ethanol at a mass ratio of 1:300 to obtain a zinc diacetate alcohol solution. The pretreated molecular sieves were immersed in zinc diacetate alcohol solution for 1.5 h, then the molecular sieves were taken out and dried in an oven at 100 °C for 1 h, then impregnated and then dried, repeated three times, and finally calcined in a muffle furnace at 400 °C for 2 h , that is, to obtain a catalyst carrier whose surface is coated with a zinc oxide film;

[0035] (2) Mix CTAB, urea, cerium nitrate, and water at a mass ratio of 1:6:20:5000, and then stir on a magnetic stirrer to dissolve all the solutes to obtain a colorless and transparent mixed solution; the carrier and The mixed solution was transferred to a 20 mL stainless steel reactor lined with polytetrafluoroethylene, sealed, placed in an oven, heated to 160 °C for 3 h, and th...

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PUM

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Abstract

The invention relates to an ozone catalyst for water treatment, a preparation method thereof and application. The method comprises the steps of loading a zinc oxide nano-film to the surface of a molecular sieve carrier and in-situ growth of cerium oxide nanosheets on the zinc oxide nano-film. Compared with a conventional dipping method for preparation of the ozone catalyst, the method of first generating the zinc oxide nano-film on the surface of the molecular sieve carrier and then performing in-situ growth of the cerium oxide nanosheets on the nano-film not only improves binding force of the catalyst and the carrier, but also greatly increases activity area of the ozone catalyst, so that the decomposition of ozone is accelerated to generate hydroxyl radicals, thereby accelerating the oxidation rate of organic matter in wastewater. The ozone catalyst is simple to prepare and high in catalytic efficiency, does not fall easily and can be reused.

Description

technical field [0001] The invention belongs to the field of waste water treatment, and in particular relates to a preparation method of an ozone catalyst for water treatment and its product and application. Background technique [0002] Ozone catalytic oxidation technology is an efficient wastewater advanced treatment technology, and it is a research hotspot in the field of industrial wastewater treatment in recent years. Compared with ozone alone as an oxidizing agent, the hydroxyl radicals produced by the interaction of ozone and catalysts have stronger oxidizing ability and faster oxidation rate for organic matter in wastewater, and can oxidize almost all pollutants. Compared with the homogeneous ozone catalytic oxidation technology, the catalyst in the heterogeneous ozone catalytic oxidation technology exists in solid form, which is easy to separate from the wastewater and can be reused. It is widely used in the actual wastewater treatment. [0003] At present, there a...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J29/00C02F1/78C02F101/30
CPCB01J29/00C02F1/725C02F1/78C02F2101/30C02F2101/306C02F2305/02
Inventor 何丹农代卫国童琴金彩虹
Owner SHANGHAI NAT ENG RES CENT FORNANOTECH