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A kind of filled modified polyurethane film and preparation method thereof

A polyurethane membrane and modification technology, applied in chemical instruments and methods, membranes, membrane technology, etc., can solve problems such as difficult dispersion and weak affinity, and achieve the effects of improved membrane separation performance, easy operation, and good selectivity

Inactive Publication Date: 2021-04-13
BEIJING TECHNOLOGY AND BUSINESS UNIVERSITY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

But both have their own disadvantages. Silica can only be prepared into non-porous or mesoporous particles, which has no selectivity for the target system, while ZIF-8 surface groups have weak affinity with polyurethane (PU) materials and are difficult to disperse.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0042] (1) Preparation of ZIF-8 nanoparticles

[0043] Will contain 2.933g (9.87mmol) commercially available Zn(NO 3 ) 2 ·6H 2 200 mL of methanol solution of O was quickly poured into 200 mL of methanol solution containing 6.489 g (79.04 mmol) of commercially available 2-methylimidazole, the mixture slowly became turbid, and after standing for 1 hour, the nanocrystals were separated from the milky dispersion by centrifugation, And wash with fresh methanol to obtain ZIF-8 nanoparticles;

[0044] (2) Preparation of aminated ZIF-8 particles

[0045] Take by weighing the ZIF-8 nanoparticles that 0.5g step (1) makes, immerse in 50mL concentration and be the ammoniacal solution of 3mol / L, obtain mixture, mixture is placed in 100mL glass beaker, beaker is placed in constant temperature water bath, Shake at room temperature for 24 hours, then transfer the beaker to a heating plate and heat to 140°C until the ammonia solution is completely volatilized. Finally, wash the above produ...

Embodiment 2

[0053] (1) Preparation of ZIF-8 nanoparticles

[0054] Will contain 2.933g (9.87mmol) commercially available Zn(NO 3 ) 2 ·6H 2 200 mL of methanol solution of O was quickly poured into 200 mL of methanol solution containing 6.489 g (79.04 mmol) of commercially available 2-methylimidazole, the mixture slowly became turbid, and after standing for 1 hour, the nanocrystals were separated from the milky dispersion by centrifugation, And wash with fresh methanol to obtain ZIF-8 nanoparticles;

[0055] (2) Preparation of aminated ZIF-8 particles

[0056] Take by weighing the ZIF-8 nanoparticle that 0.5g step (1) makes, be immersed in the ammoniacal solution of 3mol / L in 50mL concentration, the mixture is placed in the 100mL glass beaker, above-mentioned beaker is placed in the constant temperature water bath, at room temperature Shake for 24 hours under the same conditions, then transfer the beaker to the heating plate and heat to 140°C until the ammonia solution is completely vol...

Embodiment 3

[0064] (1) Preparation of ZIF-8 nanoparticles

[0065] Will contain 2.933g (9.87mmol) commercially available Zn(NO 3 ) 2 ·6H 2 200 mL of methanol solution of O was quickly poured into 200 mL of methanol solution containing 6.489 g (79.04 mmol) of commercially available 2-methylimidazole, the mixture slowly became turbid, and after standing for 1 hour, the nanocrystals were separated from the milky dispersion by centrifugation, And wash with fresh methanol to obtain ZIF-8 nanoparticles;

[0066] (2) Preparation of aminated ZIF-8 particles

[0067] Take by weighing the ZIF-8 nanoparticle that 0.5g step (1) makes, be immersed in the ammoniacal solution of 3mol / L in 50mL concentration, mixture is placed in the 100mL glass beaker, above-mentioned beaker is placed in constant temperature water bath, in Shake at room temperature for 24 hours, then transfer the beaker to a heating plate and heat to 140°C. Until the ammonia solution is completely volatilized; finally, the above pr...

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Abstract

The invention discloses a filled modified polyurethane membrane and a preparation method thereof, belonging to the technical field of pervaporation membrane separation; the method comprises the following steps: (1) preparation of ZIF-8 nanoparticles; (2) amination of ZIF-8 particles (3) Preparation of composite particles of aminated ZIF‑8 and silica; (4) Preparation of composite particles of aminated ZIF‑8 and silica filled polyurethane film. The filled modified polyurethane membrane and the preparation method thereof of the present invention have the characteristics of high permeation flux, good selectivity, low cost, easy operation of the preparation process and the like. In the preparation method of the filled modified polyurethane film of the present invention, when the temperature of the water etching reaction is 90°C and the filling amount of the silicon-based composite particles is 1%, the porous inorganic composite particle-filled polyurethane film prepared, for the mass percentage of phenol It is a 1% phenol / water mixture, and when the operating temperature is 60°C, the PSI can reach 810.139kg·μm·m ‑2 h ‑1 , which is 1.54 times higher than that of pure polyurethane film (523.23) under the same conditions.

Description

technical field [0001] The invention relates to a polyurethane film and a preparation method thereof, in particular to a filled modified polyurethane film and a preparation method thereof, and belongs to the technical field of pervaporation membrane separation. Background technique [0002] Pervaporation membrane separation technology is a high-tech technology, which is driven by the vapor pressure difference of the components in the liquid mixture and uses the difference in the dissolution and diffusion rates of the components through the membrane to achieve separation. It is especially suitable for the separation of near-boiling point, azeotropic point mixtures and isomers that are difficult or impossible to separate by distillation. It has obvious advantages in the removal of trace water in organic solvents and mixed solvents and the separation of small amounts of organic pollutants in wastewater. technical and economic advantages. [0003] The core of membrane separatio...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01D71/54B01D67/00
CPCB01D67/0079B01D71/54B01D2323/345
Inventor 叶宏董纯瑄吴奕辰王澍
Owner BEIJING TECHNOLOGY AND BUSINESS UNIVERSITY