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A preparation method of carbon fiber-loaded nano-titanium dioxide photocatalytic composite material

A technology of nano-titanium dioxide and composite materials, which is applied in the field of preparation of carbon fiber-supported nano-titanium dioxide photocatalytic composite materials, can solve problems such as easy aggregation, easy deactivation of nano-titanium dioxide, and difficulty in separation and recovery, and achieve increased specific surface area, good synergy, The effect of a short reaction cycle

Active Publication Date: 2021-06-15
江西国计纳米科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, powdery nano-titanium dioxide has problems such as easy deactivation, agglomeration, and difficulty in separation and recovery, which is one of the important reasons that limit the large-scale application of nano-titanium dioxide in actual production.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0015] This example illustrates a method for preparing a carbon fiber-supported nano-titanium dioxide photocatalytic composite material provided by the present invention.

[0016] Step 1: Immerse 5g of carbon fiber in 100mL of hydrogen peroxide with a mass percent solubility of 30%, ultrasonically treat it at room temperature for 30 minutes, and then react in an oil bath at 60°C for 3 hours. After the reaction, the product is washed 5 times with deionized water , placed in a vacuum drying oven at 110°C for 24 hours to obtain oxidized carbon fibers;

[0017] Step 2: Add 5g of oxidized carbon fiber to 100mL of a mixed solution of ethanol and vinyltrimethoxysilane with a volume ratio of 97:3, adjust the pH value of the solution to 6 with acetic acid, ultrasonically treat for 30 minutes at room temperature, and then The reaction was carried out in an oil bath at ℃ for 8 hours. After the reaction, the product was washed 5 times with a mixed solution of ethanol and deionized water, ...

Embodiment 2

[0021] This example illustrates a method for preparing a carbon fiber-supported nano-titanium dioxide photocatalytic composite material provided by the present invention.

[0022] Step 1: Immerse 5g of carbon fiber in 150mL of hydrogen peroxide with a mass percent solubility of 30%, ultrasonically treat it for 45 minutes at room temperature, and then react in an oil bath at 80°C for 2 hours. After the reaction, the product is washed 5 times with deionized water , placed in a vacuum drying oven at 110°C for 24 hours to obtain oxidized carbon fibers;

[0023] Step 2: Add 5g of oxidized carbon fiber to 150mL of a mixed solution of ethanol and methacryloxypropyltrimethoxysilane with a volume ratio of 97:3, adjust the pH of the solution to 5 with acetic acid, and ultrasonicate at room temperature 45 minutes, and then reacted for 6 hours under 80°C oil bath conditions. After the reaction, the product was washed 5 times with a mixed solution of ethanol and deionized water, and dried ...

Embodiment 3

[0027] This example illustrates a method for preparing a carbon fiber-supported nano-titanium dioxide photocatalytic composite material provided by the present invention.

[0028] Step 1: Immerse 5g of carbon fiber in 200mL of hydrogen peroxide with a mass percent solubility of 30%, ultrasonically treat it at room temperature for 60 minutes, and then react in an oil bath at 90°C for 1 hour. After the reaction, the product is washed 5 times with deionized water , placed in a vacuum drying oven at 110°C for 24 hours to obtain oxidized carbon fibers;

[0029] Step 2: Add 5g of oxidized carbon fiber to 200mL of a mixed solution of ethanol and methylvinyldiethoxysilane with a volume ratio of 97:3, adjust the pH value of the solution to 4 with acetic acid, and ultrasonically treat for 60 minutes at room temperature. Then react in an oil bath at 90°C for 4 hours. After the reaction, the product is washed 5 times with a mixed solution of ethanol and deionized water, and dried in a vac...

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Abstract

The invention provides a method for preparing a carbon fiber-loaded nano-titanium dioxide photocatalytic composite material, the steps of which are as follows: (1) using hydrogen peroxide to carry out surface treatment on carbon fibers to obtain oxidized carbon fibers; (2) oxidizing carbon fibers and vinyl silane Coupling agent reaction obtains the modified carbon fiber containing vinyl silane coupling agent; (3) obtains nano titanium dioxide containing vinyl silane coupling agent by reacting nano-titanium dioxide with vinyl silane coupling agent; (4) contains vinyl silane Coupling agent modified carbon fiber, vinyl silane-containing coupling agent modified nano-titanium dioxide and dimercapto compound are mixed, and ultraviolet light is used to initiate the reaction between mercapto group and vinyl group, and finally carbon fiber-supported nano-titanium dioxide photocatalytic composite material is obtained. The invention has short reaction period, high yield, few by-products and no harm, and the obtained photocatalytic composite material has high photocatalytic activity.

Description

technical field [0001] The invention relates to the technical field of photocatalytic materials, in particular to a method for preparing a carbon fiber-supported nano titanium dioxide photocatalytic composite material. Background technique [0002] Since the beginning of the 21st century, my country has accelerated the pace of industrialization, followed by more and more resource and environmental issues that need to be dealt with. Nano-titanium dioxide is a photocatalytic material with excellent performance, and has the advantages of high activity, low cost, and environmental friendliness, and has been widely used in the treatment of various environmental pollution. However, powdery nano-titanium dioxide has problems such as easy deactivation, agglomeration, and difficulty in separation and recovery, which is one of the important reasons that limit the large-scale application of nano-titanium dioxide in actual production. An important way to solve this problem is to load n...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J21/18
CPCB01J21/18B01J35/39
Inventor 熊磊李晨颖詹凤刘芳
Owner 江西国计纳米科技有限公司