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A kind of deoxidation catalyst and its preparation method and application

A deoxidation catalyst, catalyst technology, applied in chemical instruments and methods, metal/metal oxide/metal hydroxide catalysts, physical/chemical process catalysts, etc., can solve problems such as high energy consumption

Active Publication Date: 2021-08-31
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, non-noble metals are limited by their activity and need to be reacted at a higher temperature, which consumes a lot of energy.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] Preparation of modified silica: by impregnation method silicon oxide (commercially available, the following properties: specific surface area of ​​335m 2 / G, pore volume of 0.86ml / g) was immersed Nd nitrate, nickel nitrate aqueous solution of Nd, Ni molar concentration of metal ions was 0.5mol / L, after impregnation by drying, calcining, drying time of the IH, dried temperature of 100 deg.] C; the roasting time 2h, the temperature is 900 deg.] C;

[0022] Preparation of silica supported cobalt: by impregnation drying method, a solution of cobalt nitrate impregnation after calcination, is impregnated on a modified silica, the drying time was 2h, the drying temperature is 130 ℃; the roasting time 4h, the temperature to 400 deg.] C;

[0023] The silica supported cobalt and zirconium sulfate type shape into mixed, dried and calcined to obtain the deoxygenation catalyst, the drying time of 4h, a drying temperature of 100 deg.] C; the roasting time 6h, temperature of 400 ℃. S...

Embodiment 2

[0026] Preparation of modified silica: by impregnation method silicon oxide (commercially available, the following properties: specific surface area of ​​335m 2 / G, pore volume of 0.86ml / g) was immersed Nd nitrate, nickel nitrate aqueous solution of Nd, Ni molar concentration of metal ions was 1.5mol / L, after impregnation by drying, calcining, the drying time was 2h, dried temperature of 100 deg.] C; the roasting time 8h, temperature of 700 deg.] C;

[0027] Preparation of silica supported cobalt: by impregnation drying method, the impregnation of cobalt sulfate solution after calcination, is impregnated on a modified silica, the drying time was 3h, the drying temperature is 120 deg.] C; the roasting time 5h, temperature to 450 deg.] C;

[0028] The silica supported cobalt and zirconium sulfate type shape into mixed, dried and calcined to obtain the deoxygenation catalyst, the drying time of 4h, a drying temperature of 100 deg.] C; the roasting time 6h, temperature of 400 ℃. ...

Embodiment 3

[0031] Preparation of modified silicon oxide: using an equal volume impregnation method in silica (commercially available goods, the nature is as follows: specific surface 335m 2 / g, the hole is 0.86 mL / g) impregnated nd, nickel nickel nickel solution, ND in solution, and nickel metal ions were 1 mol / L, dried after immersion, and the drying time was 0.5 h, drying The temperature is 130 ° C; the calcination time is 5 h, the temperature is 800 ° C;

[0032] The silicon oxide silicon oxide was prepared: the hydrominated cobalt bromide solution was impregnated with an equal volume impregnation method, and dried, calcined, and the drying time was 4 h, the drying temperature was 100 ° C; the baking time is 4h, The temperature is 500 ° C;

[0033] The silicon oxide of the preparation of cobalt is prepared: the hydraulous sulfate solution is impregnated on the modified silicon oxide, and drying, the drying time is 3 h, the drying temperature is 120 ° C; the drying time is 5 h, temper...

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Abstract

The invention discloses a deoxidation catalyst and a preparation method thereof. The preparation method of the deoxidation catalyst comprises the following steps: (1) co-impregnating silicon oxide with a mixed solution containing Nd and nickel, and then drying and roasting at a high temperature to prepare obtain modified silica; (2) load cobalt on the modified silica prepared in step (1), dry and roast to obtain cobalt-loaded silica; (3) combine zirconium sulfate with step (3) The prepared silicon oxide loaded with cobalt is kneaded and molded, dried and calcined to obtain a deoxidation catalyst. The catalyst has the advantages of high activity, low reaction temperature, simple preparation method, low cost and the like when used for coal bed gas deoxidation.

Description

Technical field [0001] The present invention relates to a deoxygenation catalyst and preparation method and application thereof, and more particularly relates to a composite CBM deoxygenation catalyst and preparation method and application. Background technique [0002] Our country is the largest producer of coal each year due to the production of coal bed methane would yield a large number of different concentrations of coal-bed methane development and effective use of technology to reduce direct emissions of methane is my country's construction of environmentally friendly energy model of sustainable development, to build a low-carbon economy an integral part of the system. Combined with energy conservation and improvement of environmental requirements, practical and rational development of coalbed methane in this low-grade energy and convert it to a good use of resources, expand the scope and scale of coalbed methane, improve the utilization of coal-bed methane efficiency, ener...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J23/847C10L3/00C10L3/10
Inventor 李杰张信伟倪向前王海洋
Owner CHINA PETROLEUM & CHEM CORP