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A kind of rare earth modified fiber reinforced polylactic acid and its preparation method

A technology of fiber reinforcement and rare earth modification, which is applied in the field of rare earth modified fiber reinforced polylactic acid and its preparation, can solve the problem that the mechanical properties of polylactic acid need to be improved, the mechanical properties of polylactic acid are deteriorated, and it is difficult to obtain ultra-high tensile strength and tensile modulus. The amount of polylactic acid and other issues

Active Publication Date: 2022-05-06
HUNAN UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Among the several biodegradable materials that have been developed, polylactic acid is known as one of the most promising products due to its good mechanical properties, but compared with traditional engineering plastics, its mechanical properties still need to be improved
[0003] Cellulose fibers have high tensile strength and high tensile modulus. Filling modified polylactic acid with cellulose fibers is an effective way to improve its mechanical properties. The most commonly used method is to melt blend cellulose and polylactic acid, but When the amount of cellulose fiber added exceeds a certain limit, the mechanical properties of polylactic acid deteriorate with the increase of cellulose fiber filling, and it is difficult to obtain polylactic acid with ultra-high tensile strength and tensile modulus.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0023] The invention provides a preparation method of rare earth modified fiber reinforced polylactic acid, comprising the following steps:

[0024] Mix the rare earth compound, cellulose fiber and water to obtain A solution;

[0025] dissolving polylactic acid in an organic solvent to obtain solution B;

[0026] Blending the A solution and the B solution to obtain the C solution;

[0027] Mixing the C solution and the flocculant to obtain the D solution;

[0028] Remove the water and organic solvent in the D solution to obtain solid E;

[0029] The solid E is hot-pressed to obtain rare earth modified fiber reinforced polylactic acid.

[0030] In the present invention, unless otherwise specified, all raw material components are commercially available products well known to those skilled in the art.

[0031] The invention mixes rare earth compound, cellulose fiber and water to obtain A solution. In the present invention, the mass ratio of the rare earth compound to the cel...

Embodiment 1

[0050] In parts by weight, 5 parts of Ce(C 8 h 15 o 2 ) 3 , 50 parts of nanocellulose and 1100 parts of water were ultrasonically mixed at 30°C for 12 hours to obtain A solution;

[0051] 40 parts of PLLA were dissolved in 800 parts of dichloromethane to obtain B solution;

[0052] The A solution and the B solution were blended for 60 minutes and stirred to obtain the C solution;

[0053] Add 8 parts of polyacrylamide into the C solution, blend and stir at 30°C for 3 hours to obtain D solution;

[0054] The D solution was heated and concentrated on a rotary evaporator to obtain a colloid; the colloid was filtered and dried to obtain a solid E;

[0055] The solid E was placed between two stainless steel plates, and hot-pressed at 180° C. and 20 MPa for 2 minutes to obtain rare earth-modified fiber-reinforced polylactic acid.

[0056] The rare earth modified fiber reinforced polylactic acid prepared in this example has a tensile strength of 105 MPa and a tensile modulus of...

Embodiment 2

[0058] In parts by weight, 3 parts of La(ClO) 3 , 20 parts of softwood fiber and 460 parts of water were ultrasonically mixed at 50°C for 6 hours to obtain solution A;

[0059] 50 parts of PDLA and 27 parts of PLDLLA were dissolved in 1500 parts of toluene to obtain B solution;

[0060] The A solution and the B solution were blended for 90 minutes and stirred to obtain the C solution;

[0061] Add 5 parts of polyacrylamide and 5 parts of polyaluminum ferric silicate into the C solution, blend at 40°C for 2 hours and stir to obtain D solution;

[0062] The D solution was heated and concentrated on a rotary evaporator to obtain a colloid; the colloid was filtered and dried to obtain a solid E;

[0063] The solid E was placed between two stainless steel plates, and hot-pressed at 190° C. and 20 MPa for 3 minutes to obtain rare earth-modified fiber-reinforced polylactic acid.

[0064] The rare earth modified fiber reinforced polylactic acid prepared in this example has a tensil...

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Abstract

The invention provides a rare earth modified fiber reinforced polylactic acid and a preparation method thereof, and relates to the technical field of biodegradable packaging materials. The invention combines a solution blending method and a hot pressing method to prepare a high-content fiber-filled polylactic acid composition with good mechanical properties. First of all, the present invention modifies the cellulose fiber with rare earth, on the one hand, it can reduce the hydrophilicity of the hydroxyl group on the surface of the cellulose fiber; Compatibility of lactic acid; adding flocculant can effectively maintain the uniform mixing of cellulose fiber and polylactic acid, prevent sedimentation and cause stratification; then, the present invention can improve the compactness of cellulose fiber and polylactic acid and fix the cellulose Orientation of fibers; finally biodegradable rare-earth modified fiber-reinforced polylactic acid with ultrahigh tensile strength and tensile modulus is obtained.

Description

technical field [0001] The invention relates to the technical field of biodegradable packaging materials, in particular to a rare earth modified fiber reinforced polylactic acid and a preparation method thereof. Background technique [0002] Bio-based materials are one of the country's strategic emerging industries, and also one of the materials proposed by the country for key development. Making full use of abundant biomass resources, developing environmentally friendly and biodegradable materials, and replacing traditional polymer materials to the greatest extent is expected to alleviate the environmental pollution caused by refractory plastic waste. Among the several biodegradable materials that have been developed, polylactic acid is known as one of the most promising products due to its good mechanical properties. However, compared with traditional engineering plastics, its mechanical properties still need to be improved. [0003] Cellulose fibers have high tensile str...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08J5/06C08L67/04C08L1/02C08L97/02
CPCC08J5/06C08J2367/04C08J2401/02C08J2497/02C08J2467/04
Inventor 吴银财刘跃军郝喜海林凤龙林新土刘小超
Owner HUNAN UNIV OF TECH