Submicron non metallic microsphere with nano metal film and its preparation method
A nano-metal film and sub-micron technology, which is applied in the field of sub-micron non-metallic microspheres and their preparation, can solve the problems of poor microstructure uniformity, influence on optical properties, impure composition of film layers, etc., and achieves low cost and wide range of materials. , the effect of a wide range of sizes
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Embodiment 1
[0020] 0.05g of 300nm silica glass microspheres are added into a mixed solution of ethanol-water (molar ratio 0.5±0.3) of sodium hydroxide (0.2mol) and sodium carbonate (0.2±1mol) to react for 10-120 minutes. Then under ultrasonic vibration, add hydrochloric acid (0.1±0.3mol), tin dichloride (0.3±0.3mol) and deionized water (50±10mol) mixed solution at 5~80℃ for 2~ 120 minutes. Then add silver nitrate (0.2±0.1mol), ammonia water (0.01±0.005mol), and formaldehyde (0.2±0.1mol) to the ethanol-water (molar ratio 0.5±0.3) mixed solution to adjust the pH value to 8-12.10 After ~60 minutes, add silver nitrate (0.2±0.1mol), ammonia water (0.01±0.005mol), formaldehyde (0.2±0.1mol) to the mixed solution of ethanol-water (molar ratio 0.5±0.3) After standing in an environment of 10-80° C. for 1-120 hours, submicron glass microspheres coated with a metal film with a thickness of about 14 nanometers are obtained.
Embodiment 2
[0022] 0.03g of 100nm silicon dioxide glass microspheres are added into a mixed solution of ethanol-water (molar ratio 0.5±0.3) of sodium hydroxide (0.2mol) and sodium carbonate (0.2±1mol) to react for 10-120 minutes. Then under ultrasonic vibration, add hydrochloric acid (0.1±0.3mol), tin dichloride (0.3±0.3mol) and deionized water (50±10mol) mixed solution at 5~80℃ for 2~ 120 minutes. Then add silver nitrate (0.01±0.05mol), ammonia water (0.01±0.005mol), formaldehyde (0.01±0.05mol) in ethanol-water (molar ratio 0.5±0.3) mixed solution, adjust the pH value to 6~12.10 After ~60 minutes, add silver nitrate (0.05±0.05mol), ammonia water (0.08±0.05mol), formaldehyde (0.05±0.05mol) in the mixed solution of ethanol-water mixture (molar ratio 0.5±0.3) After standing in an environment of 10-50° C. for 1-120 hours, silver-coated submicron glass microspheres with a thickness of about 5 nanometers are obtained.
Embodiment 3
[0024] Add hydrochloric acid (0.2±0.3mol), tin dichloride (0.2±0.3mol) and deionized water (50±10mol) to 0.05g of 600nm polystyrene microspheres under ultrasonic vibration at 20-30°C In the mixed solution, the time ranges from 2 to 120 minutes. Then add silver nitrate (0.01±0.0051mol), ammonia water (0.01±0.005mol), formaldehyde (0.01±0.005mol) in ethanol-water (molar ratio 0.5±0.3), adjust the pH value to 8~11. 10~60 After 10 minutes, add it to the mixed solution composed of silver nitrate (0.01±0.005mol), ammonia water (0.01±0.005mol), formaldehyde (0.01±0.005mol) ethanol-water mixed solution (molar ratio 0.5±0.5), in 10~ After standing at 80° C. for 1 to 120 hours, polystyrene microspheres coated with a silver film with a thickness of about 5 nanometers were obtained.
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