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An unsaturated, substrate-based technology, applied in chemical instruments and methods, polishing compositions containing abrasives, and other chemical processes, can solve problems that cannot fully meet the stringent requirements of the semiconductor industry
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Embodiment 1
[0050] This example illustrates the effect of an amphiphilic nonionic surfactant in a polishing composition on copper dishing and erosion values as a function of the surfactant HLB value.
[0051] Similar patterned substrates (Sematech 931 mask wafers) containing copper, tantalum and titanium dioxide were polished with different polishing compositions (Polishing Compositions 1A-1E). Each polishing composition contained 12% by weight condensation-precipitated silica, 0.10% by weight benzotriazole, 0.30% by weight acetic acid, 3% by weight hydrogen peroxide, and 200 ppm of surfactant, pH 10 (adjusted with KOH ). Polishing compositions 1A (comparative example) and 1B-1E (present invention) respectively contain polyoxyethylene (2) isooctylphenyl ether with HBL of 4.6, polyoxyethylene (5) isooctylphenyl ether with HBL of 10 Ether, polyoxyethylene(9) nonylphenyl ether with HBL 13, polyoxyethylene(40) nonylphenyl ether with HBL 17.8, and polyoxyethylene(100) nonylphenyl ether with...
Embodiment 2
[0056] This example illustrates the effect of an amphiphilic nonionic surfactant on copper dishing and erosion values as a function of surfactant concentration in a polishing composition.
[0057] Similar patterned substrates (Sematech 931 shielded wafers) containing copper, tantalum and titanium dioxide were polished with different polishing compositions (Polishing Compositions 2A-2D). Each polishing composition contained 12% by weight condensation-precipitated silica, 0.10% by weight benzotriazole, 0.30% by weight acetic acid, and 3% by weight hydrogen peroxide, at a pH of 10 (adjusted with KOH). Polishing Compositions 2A-2D (invention) also included 0, 100, 125, and 250 ppm, respectively, of 2,4,7,9-tetramethyl-5-decyne-4,7-diol ethoxylated surfactant agent. The percent improvement in dishing in the 50 micron line region of the patterned substrate was measured for each polishing composition.
[0058] image 3 A graph showing % improvement in copper dishing for 50 micro...
Embodiment 3
[0061] This example demonstrates that the presence of amphiphilic nonionic surfactants in the polishing compositions of the present invention can be used in first step copper polishing for removal of large amounts of copper.
[0062] Similar blanket wafer substrates containing copper, tantalum, or titanium dioxide were polished with different polishing compositions (Polishing Compositions 3A-3F). Polishing Composition 3A (blank) was free of amphiphilic nonionic surfactants and comprised 0.7% by weight lactic acid, 1.11% by weight polyacrylic acid, 0.111% by weight benzotriazole, 3% by weight hydrogen peroxide, and 0.556% by weight heat Decomposed alumina, the fumed alumina was coated with polystyrene sulfonic acid (0.5% by weight alumina and 0.052% by weight polystyrene sulfonic acid) at a pH of 4.5. Polishing Compositions 3B-3E (invention) were identical to Polishing Composition 3A, except that they also included 0.02%, 0.05%, 0.075%, and 0.10% by weight of polyalkylene oxide...
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