Process for producing extruded polyhydroxyalkanoate resin foam
A technology for extrusion foaming and hydroxycaproate, which is applied in the field of preparation of polyhydroxyalkanoate resin extrusion foams, can solve problems such as undisclosed foaming ratio, and achieve the effect of excellent water resistance
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Embodiment 1
[0080] Alcaligenes eutrophus AC32 (J. Bacteriol., 179, 4821 (1997) was used in which the PHA synthase gene derived from Aeromonas caviae was introduced into Alcaligenes eutrophus. ) as microorganisms, suitably adjust raw materials, culture conditions, produce PHBH (HH rate 10mol%, Mw=530,000).After PHBH melts and kneads at 135 ℃ of cylinder temperature in the uniaxial extruder of φ 35mm, from Extrude from the small hole die head of 3mmφ at the front end of the extruder, and the extruded strands pass through the granulator, cut off, and produce PHBH particles A (Mw=450,000, Tg=1°C, Tm=135°C) with a particle weight of 5mg , Tc=68 ℃).This particle A is supplied to the two-stage extruder connected in series with a diameter of 65mm and a diameter of 90mm with a ratio of about 40kg / hr.The aforementioned resin mixture supplied to the extruder of a diameter of 65mm is heated to 135°C (T1), melt kneading, add foaming agent, and supply to an extruder with a diameter of 90 mm connected t...
Embodiment 2
[0083] Alcaligenes eutrophus (Alcaligenes eutrophus) AC32 (J.Bacteriol., 179, 4821 (1997) into which PHA synthetase gene derived from Aeromonas caviae was introduced into Alcaligenes eutrophus was used ) as microorganisms, properly adjust raw materials, culture conditions, and produce PHBH (7mol% HH rate, Mw=720,000).After PHBH melts and kneads at 145°C of barrel temperature in a single-screw extrusion molding machine of φ 35mm, the Extrude at the small hole die of 3mmφ at the front end of the extruder, and the extruded strands pass through the granulator, cut off, and produce PHBH particles B (Mw=570,000, Tg=1°C, Tm=145°C) with a particle weight of 5mg , Tc=73 ℃).This particle B is supplied to the two-stage extruder of caliber 65mm and caliber 90mm connected in series with the ratio of about 40kg / hr.The aforementioned resin mixture supplied to the extruder of caliber 65mm is heated To 145°C (T1), melt kneading, add a foaming agent, and supply to an extruder with a diameter of...
Embodiment 3
[0086] Alcaligenes eutrophus (Alcaligenes eutrophus) AC32 (J.Bacteriol., 179, 4821 (1997) into which PHA synthetase gene derived from Aeromonas caviae was introduced into Alcaligenes eutrophus was used ) as microorganisms, properly adjust raw materials and culture conditions, and produce PHBH (HH rate 12mol%, Mw=560,000).After PHBH is melted and kneaded at 140° C. Extrude at the small hole die head of 3mmφ at the front end of the extruder, and the extruded strands pass through the granulator, cut off, and produce PHBH pellets C (Mw=520,000, Tg=2°C, Tm=142°C) with a particle weight of 5mg , Tc=72 ℃).This particle C is supplied to the two-stage extruder connected in series with a diameter of 65mm and a diameter of 90mm with a ratio of about 40kg / hr.The aforementioned resin mixture supplied to the extruder of a diameter of 65mm is heated to 140°C (T1), melt kneading, add foaming agent, and supply to an extruder with a diameter of 90 mm connected to an extruder with a diameter of ...
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