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Compound ceramic film lamination high energy storage density capacitor and preparation method thereof

A technology of high energy storage density and composite ceramics, applied in the direction of multilayer capacitors, fixed capacitor dielectrics, fixed capacitor components, etc., can solve the problem of not being able to significantly improve the breakdown field strength of ceramic-polymer films, and achieve low cost , The effect of high energy storage density and high specific power

Inactive Publication Date: 2012-06-13
NORTHWEST INST OF NUCLEAR TECH +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0009] Aiming at the problem that the prior art cannot significantly improve the breakdown field strength of the ceramic-polymer film, the present invention provides a composite ceramic film laminated capacitor with high energy storage density and a preparation method thereof

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0056] Take by weighing 5.510g PMN ceramic powder (density is 8.3g / cm 3 ) accounted for 60% by volume, 0.755gPVDF (polyvinylidene fluoride, density 1.7g / cm 3 ) accounted for 40% by volume, measured 6mL DMF (N, N-dimethylformamide), added to a 50mL agate ball mill jar, and ball milled for 15 hours to obtain a precursor slurry; the slurry was naturally flowed on a clean substrate Unfold flat, place in a vacuum drying oven, and vacuum dry at 50-160°C to remove the solvent DMF to obtain a composite ceramic film; wherein, the volume fraction of PMN ceramic powder is 60%; cut the obtained composite film into a circle Sheet or square sheet, with aluminum foil on both sides or between them as electrodes, heated in vacuum at 170-200°C to soften PVDF, and hot-pressed at 10-120MPa to obtain a single-layer or multi-layer capacitor. electrical properties. The thickness of the composite film is 67-80 μm. Under the measurement conditions of 1kHz, 1.0V, and 25°C, the relative dielectric con...

Embodiment 2

[0058] Take by weighing 3.018g PMN ceramic powder (density is 8.3g / cm 3 ) accounted for 63% by volume, 0.358gPVDF (density 1.7g / cm 3 ) accounted for 37% by volume percentage, measured 6mL DMF, added to a 50mL agate ball mill jar, and ball milled for 30h to obtain a precursor slurry; the slurry was naturally leveled on a clean substrate, placed in a vacuum oven, and Vacuum drying at 50-160°C removes the solvent DMF to obtain a composite ceramic film; wherein, the volume fraction of PMN ceramic powder is 63%; the obtained composite film is cut into circular or square pieces, and the two sides or between each The backing aluminum foil is used as an electrode, and the PVDF is softened by vacuum heating at 170-200 ° C, and hot-pressed at 10-120 MPa to obtain a single-layer or multi-layer capacitor, and its dielectric properties are measured. The thickness of the composite film is 20-40 μm. Under the measurement conditions of 1kHz, 1.0V, and 25°C, the relative dielectric constant i...

Embodiment 3

[0060] Take by weighing 5.520g PMN ceramic powder (density is 8.3g / cm 3 ) accounted for 69% by volume, 0.505gPVDF (density 1.7g / cm 3 ) accounted for 31% by volume percentage, measured 6mL DMF, added to a 50mL agate ball mill jar, and ball milled for 10 hours to obtain a precursor slurry; the slurry was naturally leveled on a clean substrate, placed in a vacuum oven, and Vacuum drying at 50-160°C removes the solvent DMF to obtain a composite ceramic film; wherein, the volume fraction of PMN ceramic powder is 69%; the obtained composite film is cut into circular or square pieces, and the two sides or between each The backing aluminum foil is used as an electrode, and the PVDF is softened by vacuum heating at 170-200 ° C, and hot-pressed at 10-120 MPa to obtain a single-layer or multi-layer capacitor, and its dielectric properties are measured. The thickness of the composite film is 100-120 μm. Under the measurement conditions of 1kHz, 1.0V, and 25°C, the relative dielectric con...

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Abstract

The invention relates to a compound ceramic film lamination high energy storage density capacitor and a preparation method thereof. The high energy storage density capacitor provided by the invention is formed by superposition of multilayer compound ceramic films. Ceramic particles with a high dielectric constant are taken as a matrix of the compound ceramic films. An organic polymer with high breakdown field strength is taken as a filler and a binding agent which are filled in gap between ceramic particles to prepare the close compound film. High temperature sintering with energy consumption is avoided, large area preparation is available, air micro bubble which easily causes breakdown can be completely eliminated, and a high dielectric constant and withstand voltage intensity are provided. The capacitor prepared by superposition of the compound ceramic films has high work voltage and energy storage density.

Description

technical field [0001] The invention belongs to the technical field of energy storage, and in particular relates to a composite ceramic film laminated capacitor with high energy storage density and a preparation method thereof. Background technique [0002] Capacitors with high energy storage density have broad application prospects in both civil and military applications due to their inherent advantages of long life, high specific power, high safety, and environmental friendliness. [0003] With the development of national economy, energy shortage and energy security are becoming more and more serious. The development of renewable energy is the only way to solve the energy shortage and maintain sustainable economic development. Renewable energy power generation must be regulated by a smart grid equipped with power storage devices to function; electric vehicles need short-term high-power power supply to start, accelerate and climb hills. Therefore, capacitors with high ene...

Claims

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Application Information

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IPC IPC(8): H01G4/06H01G4/30
Inventor 王武尚涂国荣杨裕生
Owner NORTHWEST INST OF NUCLEAR TECH