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A kind of preparation method of activated carbon for supercapacitor

A technology of supercapacitor and activated carbon, which is applied in chemical instruments and methods, inorganic chemistry, non-metallic elements, etc., can solve the problems of limiting supercapacitor power density, low electrolyte diffusion and migration rate, etc., to improve practical potential and application. effect of value

Inactive Publication Date: 2015-11-18
LUXI GRP
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Activated carbon uses its porous characteristics to complete energy storage, but due to the limitation of pore size, the rate of electrolyte diffusion and migration is not high, which will limit the power density of supercapacitors

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] Put 5Kg of coconut shell activated carbon in a 100L reaction kettle, add 50L of distilled water, heat to 50°C, and stir for 4 hours to obtain an aqueous dispersion of activated carbon; take 450g of graphene dry powder and 45g of 9-anthracene formic acid, disperse them in 10L of ethanol, and heat to 40°C and stirred for 1 hour to obtain an ethanol dispersion of graphene; dropwise add the ethanol dispersion of graphene into the water dispersion of activated carbon at a rate of 10mL / min, wherein the ethanol dispersion of graphene and the water dispersion of activated carbon The liquid mass ratio is 20:1, stirring; after the dropwise addition, the temperature is raised to 80°C, and stirred and distilled for 8 hours; the heating and stirring are stopped, and the temperature is naturally lowered to room temperature; the obtained slurry is separated from solid and liquid to obtain a precursor; The body was heated up to 600° C. under the protection of nitrogen atmosphere in a tu...

Embodiment 2

[0023] Put 3.5Kg of petroleum coke activated carbon in a 100L reaction kettle, add 50L of ethanol, heat to 30°C, and stir for 36 hours to obtain an ethanol dispersion of activated carbon; take 250g of graphite milk and 50g of benzoic acid, disperse them in 1L of ethanol, and heat to Stir at 40°C for 1 hour to obtain the ethanol dispersion of graphene; drop the ethanol dispersion of graphene into the ethanol dispersion of activated carbon at a rate of 1mL / min, wherein the ethanol dispersion of graphene and the mass of the ethanol dispersion of activated carbon The ratio is 6.59:1, stirring; after the dropwise addition, the temperature is raised to 50°C, and stirred and distilled for 36 hours; the heating and stirring are stopped, and the temperature is naturally lowered to room temperature; the obtained slurry is separated from solid and liquid to obtain a precursor; Under the protection of argon atmosphere in a tube furnace, the temperature was raised to 500° C., kept for half ...

Embodiment 3

[0025] Put 4Kg of coconut shell modified activated carbon in a 100L reactor, add 50L of N-methylpyrrolidone, heat to 70°C, and stir for 72 hours to obtain an N-methylpyrrolidone dispersion of activated carbon; take 4000g of graphene dry powder graphite oxide, 200g Disperse naphthoic acid in 5L ethanol, heat to 40°C, and stir for 1 hour to obtain an ethanol dispersion of graphene; add the ethanol dispersion of graphene to the N-methylpyrrolidone dispersion of activated carbon dropwise at a rate of 100mL / min Among them, the mass ratio of the ethanol dispersion of graphene to the active carbon N-methylpyrrolidone dispersion is 42:1, stirring; after the dropwise addition is completed, the temperature is raised to 70°C, and stirring and distillation are carried out for 72 hours; heating and stirring are stopped, and naturally Cool down to room temperature; separate the solid and liquid from the obtained slurry to obtain a precursor; raise the temperature of the precursor to 500° C. ...

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Abstract

The invention discloses a preparation method for activated carbon for a super capacitor. The preparation method comprises the following steps: the first step, activated carbon or modified activated carbon and graphene are subjected to coprecipitation-loading in dispersion liquids: first, activated carbon or modified activated carbon and a dispersion liquid are mixed and stirred, then heated to the temperature of 30-100 DEG C for continued 1-96h, and an activated carbon dispersion liquid is obtained; second, graphene or graphene precursors or graphene dry powder and stabilizing agents are mixed and dispersed in ethanol, and the concentration of the ethanol dispersion liquid of graphene is 0.01-100g / L; third, the obtained ethanol dispersion liquid of graphene is dropwise added into the activated carbon dispersion liquid at a speed of 0.5mL / min-500mL / min, the mixture is stirred and heated to the temperature of 30-100 DEG C for continued 1-96h, and a loaded slurry is obtained; the second step, the loaded slurry is subjected to solid-liquid separation and precursors are obtained; the third step: the precursors are subjected to atmosphere calcination for activation at the temperature of 500-600 DEG C for 0.5-3h, and activated carbon for a super capacitor is obtained. The beneficial effects of the preparation method are that the volume specific capacity and the antidamping capability are raised.

Description

technical field [0001] The invention relates to a preparation method of activated carbon, in particular to a preparation method of activated carbon for supercapacitors. Background technique [0002] Supercapacitors are between batteries and ordinary capacitors. They have the characteristics of large current and fast charging and discharging of capacitors, and also have the characteristics of energy storage of batteries, and have a long repeated service life. Energy-to-electricity conversion, the whole process does not have any chemical reaction, and does not cause pollution to the surrounding environment. It is an ideal energy storage device. In recent years, activated carbon with high specific surface area and high purity has attracted much attention as an electrode material for supercapacitors. Activated carbon uses its porous characteristics to complete energy storage, but due to the limitation of pore size, the rate of electrolyte diffusion and migration is not high, wh...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C01B31/08C01B32/354C01B32/36
Inventor 张文景海伟周继光
Owner LUXI GRP