Light emitting material and organic light emitting element using same
A technology of organic light-emitting elements and light-emitting materials, which is applied in the fields of light-emitting materials, electrical components, organic chemistry, etc., and can solve problems such as the usefulness of compound light-emitting materials that are not mentioned
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[0312] Hereinafter, the characteristics of the present invention will be described more specifically with reference to synthesis examples and examples. Materials, processing contents, processing procedures, and the like shown below can be appropriately changed as long as they do not deviate from the gist of the present invention. Therefore, the scope of the present invention should not be limitedly interpreted by the specific examples shown below.
Synthetic example 1
[0314] In this synthesis example, compound 1 was synthesized according to the following scheme.
[0315] [Chemical 53]
[0316]
[0317] 3-carbazolylcarbazole (0.25g, 0.75mmol), 2-bromo-4,6-diphenyl-1,3,5-triazine (0.29g, 0.75mmol), copper iodide (0.021g , 0.11mmol), 18-crown-6 (0.030g, 0.11mmol), potassium carbonate (0.62g, 4.5mmol) were added to dodecylbenzene (2.0mL), and heated at 220°C under nitrogen atmosphere 2 days. After the reaction, extract with dichloromethane, dry with sodium carbonate, and then purify using silica gel column chromatography (developing solvent: hexane / dichloromethane=80 / 20) to obtain compound 1 (yield 0.25 g (4.0 mmol), 53% yield).
[0318] 1 HNMR (500MHz, CDCl 3 ): δ (ppm) 9.08 (d, J = 9.0Hz, 2H), 8.84 (d, J = 6.5Hz, 4H), 8.32 (d, J = 2.0Hz, 1H), 8.20 (d, J = 8.0Hz ,2H),8.15(d,J=7.5,1H),7.91(d,J=8.5Hz,2H),7.75(d,J=9.0Hz,1H),7.67-7.59(m,8H),7.55- 7.51(m,1H),7.45-7.41(m,4H),7.38-7.35(m,1H),7.33-7.29(m,2H)
Synthetic example 2
[0320] In this synthesis example, compound 2 was synthesized according to the following scheme.
[0321] [Chemical 54]
[0322]
[0323] [Scheme 1] Synthesis of 3,6-tert-butyl-9-(9-tosyl-9H-carbazol-3-yl)-9H-carbazole
[0324] 3-Bromo-9-tosyl-9H-carbazole (4.47g, 11.5mmol), 3,6-di-tert-butyl-9H-carbazole (3.04g, 10.9mmol), copper(I) oxide ( 3.96 g, 27.6 mmol) was added into dodecylbenzene (2.0 mL), and heated at 220° C. for 20 hours under nitrogen atmosphere. After the reaction was completed, copper oxide (I) was removed by filtration, followed by column chromatography on silica gel (developing solvent: hexane / dichloromethane=70 / 30) for purification (yield 2.21g (11.5mmol), yield 32.2%).
[0325] 1 HNMR (500MHz, CDCl 3 ): δ (ppm) 8.38 (d, J = 8.5Hz, 1H), 8.16 (d, J = 1.5Hz, 1H), 8.07 (d, J = 2.0Hz, 1H), 7.87 (d, J = 7.5Hz ,1H),7.80(d,J=8.5Hz,2H),7.66(dd,J=2.5Hz,J=2.0Hz,1H),7.57-7.53(m,1H),7.46(dd,J=2.0Hz ,J=1.5Hz,2H),7.40-7.37(m,1H),7.32(d,J=9.0Hz,2H),7.20(d,J=8.0Hz,2H...
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