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A Method for Selectively Removing Chloride Ion Using Ion Imprinted Polymer

A technology of ion imprinting and polymer, applied in the field of water treatment, can solve problems such as corrosion of pipelines and equipment, achieve low investment and operating costs, and simple operation and management

Active Publication Date: 2017-08-11
浙江常山利盛新材料有限公司 +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0009] The purpose of the present invention is to provide a method for selectively removing chloride ions in wastewater by using ion-imprinted polymers to solve the problem of pipeline and equipment corrosion caused by high chloride ion content in the process of industrial water reuse

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] (1) Pretreatment of orange peel cellulose: Take 10 grams of orange peel powder and 200ml of ethanol solution (80% concentration), extract it in a water bath at 80°C for 4 hours, extract the flavonoids from the mother liquor, and recycle it; add 100ml of the reaction product NaOH solution (0.1mol / L), stirred for 1 hour, separated by a centrifuge, then added 100ml of isopropanol solution (20% concentration), soaked overnight, and the soaked solution was separated by a centrifuge;

[0023] (2) Hydroxymethylation: Pour the product after the above post-pretreatment into a dry three-necked flask equipped with a mechanical stirrer and a condenser, adjust the pH value to 7 with dilute hydrochloric acid solution, and then add 1.67g mass fraction of 36% HCHO aqueous solution, hydroxymethylation reaction occurred at 25°C for 3 h;

[0024] (3) Grafting reaction: According to n (HCHO): n (acrylamide): n (thiosemicarbazide) = 1:1:1, weigh acrylamide and thiosemicarbazide and add them...

Embodiment 2

[0028] (1) Orange peel cellulose pretreatment: Take two flasks each, take 10 grams of orange peel powder and 200ml of ethanol solution (80% concentration), extract in a water bath at 80°C for 4 hours, and extract flavonoids from the mother liquor Recover and apply; add 100ml of NaOH solution (0.1mol / L) to the reaction product, stir for 1 hour, separate with a centrifuge, add 100ml of isopropanol solution (20% concentration), soak overnight, and use a centrifuge to soak the solution separation;

[0029] (2) Hydroxymethylation: Pour the product after the above post-pretreatment into a dry three-necked flask equipped with a mechanical stirrer and a condenser, adjust the pH value to 7 with dilute hydrochloric acid solution, and then add 1.67g mass fraction of 36% HCHO aqueous solution, hydroxymethylation reaction occurred at 25°C for 3 h;

[0030] (3) Grafting reaction: According to n (HCHO): n (acrylamide): n (vinylimidazole) = 1:1:1, weigh acrylamide and vinylimidazole and add ...

Embodiment 3

[0034] In a 5000mL reaction vessel, measure 4000mL of chlorine-containing wastewater with a chloride ion concentration of 5000mg / L, add a certain amount of the ion-imprinted polymer (80g) prepared in Example 1, react for 8 hours, filter and recover the ion-imprinted polymer, The concentration of chloride ions finally reaches below 100 mg / L, meeting the requirements for chloride ions in recycled water quality.

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Abstract

The invention provides a method for selectively removing chlorine ions by using an ion imprinted polymer, belonging to the technical field of water treatment. The ion imprinted polymer used as a treating agent is an orange peel cellulose-base modification product, which is a product prepared by carrying out surface grafting modification, imprinting reaction, crosslinking closing and elution on the base orange peel cellulose; and the ion imprinted polymer can selectively remove chlorine ions in wastewater. When being used for treating chlorine-containing wastewater, the ion imprinted polymer can lower the chlorine ion concentration in the wastewater to 100 mg / L.

Description

technical field [0001] The invention belongs to the technical field of water treatment, and in particular provides a method for selectively removing chloride ions in wastewater by using an ion imprinted polymer. Background technique [0002] Chloride ion is the most common anion in water and wastewater. Excessively high concentration of chloride ion will cause bitter and salty drinking water, soil salinization, pipeline corrosion, difficult plant growth, and endanger human health. Therefore, chloride ion must be controlled emission concentration. At present, the national sewage discharge standard has not yet made corresponding requirements on the discharge standard of chloride ions. Only some local standards have made relevant regulations on chloride in wastewater. The concentration of chloride ions in the waste water of the network system shall not exceed 1000mg / L. [0003] Hydrochloric acid and salts containing chloride ions are commonly used raw materials in the product...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C02F1/28B01J20/24B01J20/32C02F101/12
Inventor 吕亮曾惠明吾国强王玉林
Owner 浙江常山利盛新材料有限公司