Synthetic polyurethane elastomers based on soft segment prepolymers and non-mercury catalysts for subsea pipeline insulation
A composite polyurethane, non-mercury catalyst technology, applied in polyurea/polyurethane coatings, pipeline protection through thermal insulation, pipeline protection, etc., can solve the problems of exposure of the underlying substrate, loss of thermal insulation efficiency, etc.
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example 1
[0073] Example 1 and Comparative Samples A and B
[0074] Polyol A is a nominally trifunctional polyether made by adding propylene oxide to a trifunctional initiator followed by ethylene oxide. Polyol A contains about 15% by weight ethylene oxide. It contains mainly primary hydroxyl groups and has a hydroxyl equivalent weight of about 2050.
[0075] The Zn / Zr catalyst is a mixture of zinc carboxylate and zirconium carboxylate, wherein the weight ratio of zinc to zirconium is 99-99.5:0.5-1. Catalysts contain some species with M-O-M bonds, where M represents a metal, ie Zn or Zr.
[0076] The microspheres are 3M grade S38HS glass microspheres.
[0077] Polyisocyanate A is a modified MDI with an isocyanate equivalent weight of 160 g / mol and an isocyanate functionality of about 2.
[0078] Polyurethane Elastomer Example 1 was produced by reacting 62.5 g of Polyol A with 45.5 g of Polyisocyanate A under nitrogen until the isocyanate content was reduced to about 8% by weight. G...
specific Embodiment
[0084] Specific embodiment: in specific embodiment, the present invention is:
[0085] 1. A cured syntactic polyurethane elastomer comprising an alkanediol chain extender, microspheres ranging from 5% to 50% by weight of the reaction mixture, and an isocyanate content of 3% to 12% by weight The reaction product of a reaction mixture of an isocyanate-terminated prepolymer and a non-mercury catalyst, wherein (i) said prepolymer is a mixture of at least one polyether polyol having an average hydroxyl equivalent weight of at least 800 with an excess of aromatic polyisocyanate The reaction product, (ii) the amount of prepolymer provided to the reaction mixture is sufficient to provide an isocyanate index of 80 to 130, and (iii) the reaction mixture is substantially free of mercury compounds.
[0086] 2. The preceding embodiment, wherein the cured composite elastomer comprises a polyurethane matrix with microspheres embedded therein.
[0087] 3. Any preceding embodiment, wherein th...
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Abstract
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