Dielectric adjustable low-loss wolframite microwave dielectric ceramic and preparation method thereof
A technology of microwave dielectric ceramics and wolframite, which is applied in the field of electronic information materials and devices, to achieve the effects of stable and single composite phase, low synthesis temperature and precise control of stoichiometric ratio
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Embodiment 1
[0024] (1) Mixing: According to ZnSn x Ti 1-x Nb 2 O 8 (x=0.40) The stoichiometric ratio of the microwave dielectric ceramic phase, using a precision balance to weigh 4.0695g of zinc oxide (ZnO) with a purity of 99.99%, titanium oxide (TiO 2 )2.3950g, tin oxide (SnO 2 )3.0138g and niobium oxide (Nb 2 o 5 ) 13.2905g, pour the weighed powder into the mixing bottle, and add 40g of absolute ethanol and 400g of zirconia grinding balls. The grinding balls with a diameter of 1 cm and a diameter of 0.5 cm are loaded in a mass ratio of 2:1; the mixing bottle of powder, grinding balls and absolute ethanol is placed on the mixer for continuous mixing for about 24 hours, and the mixer The rotation speed is 200 r / min; the mixed slurry and the grinding balls are separated by a coarse screen, and the separated slurry is dried in a drying oven at 70-90°C.
[0025] (2) Pre-burning: put the dried powder in step (1) in a muffle furnace and pre-burn at 1050°C for 4 hours to obtain t...
Embodiment 2
[0031] (1) Mixing: According to ZnSn x Ti 1-x Nb 2 O 8 (x=0.425) The stoichiometric ratio of the microwave dielectric ceramic phase, using a precision balance to weigh 4.0695g of zinc oxide (ZnO) with a purity of 99.99%, titanium oxide (TiO 2 )2.2961g, tin oxide (SnO 2 )3.2022g and niobium oxide (Nb 2 o 5 ) 13.2905g, pour the weighed powder into the mixing bottle, and add 40g of absolute ethanol and 400g of zirconia grinding balls. The grinding balls with a diameter of 1 cm and a diameter of 0.5 cm are loaded in a mass ratio of 2:1; the mixing bottle of powder, grinding balls and absolute ethanol is placed on the mixer for continuous mixing for about 24 hours, and the mixer The rotation speed is 200 r / min; the mixed slurry and the grinding balls are separated by a coarse screen, and the separated slurry is dried in a drying oven at 70-90°C.
[0032] (2) Pre-burning: put the dried powder in step (1) in a muffle furnace and pre-burn at 1050°C for 4 hours to obtain ...
Embodiment 3
[0038] (1) Mixing: According to ZnSn x Ti 1-x Nb 2 O 8 (x=0.45) The stoichiometric ratio of the microwave dielectric ceramic phase, using a precision balance to weigh 4.0695g of zinc oxide (ZnO) with a purity of 99.99%, titanium oxide (TiO 2 )2.1963g, tin oxide (SnO 2 )3.3905g and niobium oxide (Nb 2 o 5 ) 13.2905g, pour the weighed powder into the mixing bottle, and add 40g of absolute ethanol and 400g of zirconia grinding balls. The grinding balls with a diameter of 1 cm and a diameter of 0.5 cm are loaded in a mass ratio of 2:1; the mixing bottle of powder, grinding balls and absolute ethanol is placed on the mixer for continuous mixing for about 24 hours, and the mixer The rotation speed is 200 r / min; the mixed slurry and the grinding balls are separated by a coarse screen, and the separated slurry is dried in a drying oven at 70-90°C.
[0039] (2) Pre-burning: put the dried powder in step (1) in a muffle furnace and pre-burn at 1050°C for 4 hours to obtain t...
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