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A kind of preparation method of monolithic CO reduction denitration catalyst

A denitration catalyst and integrated technology, applied in chemical instruments and methods, physical/chemical process catalysts, separation methods, etc., can solve problems such as air pollution and huanglong, and achieve the effect of improving use efficiency

Active Publication Date: 2019-06-11
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The above technologies all add nitrates during the preparation of the catalyst, and a large amount of NOx enters the catalyst tail gas during roasting, resulting in "yellow dragon" and causing serious air pollution

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0024] (1) The particle size of activated carbon is 500 mesh, polyacrylamide is used as the binder, the precursor of the active component is a mixture of ferric nitrate / chromium nitrate, the slurry is made by adding water, and pressed into a plate type; the material ratio is activated carbon : polyacrylamide: active component precursor: ceramic powder: water = 0.5: 5.0: 6.5: 75: 11.7;

[0025] (2) Put the spherical particles in the furnace, heat up at a rate of 10°C / min and keep the temperature constant to 500°C for calcination. The calcination time is 240min. During this period, a mixed gas of nitrogen and air is introduced to control the O in the mixed gas. 2 The concentration is 2.0-4.0%. During this period, the nitrate decomposes to produce NOx, the activated carbon powder is oxidized and converted into CO, and the two gases undergo a redox reaction under the action of the catalyst to generate CO 2 and N 2 .

[0026] The concentrations of CO and NOx in the tail gas prod...

Embodiment 2

[0028] (1) The particle size of activated carbon is 900 mesh, polymethacrylamide is used as the binder, the precursor of the active component is a mixture of nickel nitrate and copper nitrate, the slurry is made by adding water, and extruded into a honeycomb shape; the material The ratio is activated carbon: polymethacrylamide: active component precursor: ceramic powder: water = 1.2: 7.0: 10: 70: 11.8;

[0029] (2) Put the honeycomb precursor in the furnace, heat up at a rate of 10°C / min and keep the temperature at 400°C for calcination. The calcination time is 360min. During the period, a mixed gas of helium and air is introduced to control the O in the mixed gas. 2 The concentration is 2.0-4.0%. During this period, the nitrate decomposes to produce NOx, the activated carbon powder is oxidized and converted into CO, and the two gases undergo a redox reaction under the action of the catalyst to generate CO 2 and N 2 .

[0030] The concentrations of CO and NOx in the tail ga...

Embodiment 3

[0032] (1) The particle size of activated carbon is 200 mesh, polymethacrylamide is used as binder, the precursor of active component is a mixture of nickel nitrate and copper nitrate, with cerium nitrate as auxiliary agent, water is added to make slurry, and Extruded into a honeycomb shape; the material ratio is activated carbon: polymethacrylamide: active component precursor: cerium nitrate: ceramic powder: water=1.8:7.0:10:1.5:69.7:10;

[0033] (2) Put the honeycomb precursor in the furnace, heat up at a rate of 10°C / min and keep the temperature constant to 450°C for calcination. The calcination time is 360min. During the period, a mixed gas of argon and air is introduced to control the O in the mixed gas. 2 The concentration is 2.0-4.0%. During this period, the nitrate decomposes to produce NOx, the activated carbon powder is oxidized and converted into CO, and the two gases undergo a redox reaction under the action of the catalyst to generate CO 2 and N 2 .

[0034] Th...

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Abstract

The invention discloses a preparation method of an integral CO reduction denitration catalyst. The method comprises the following steps of (1) uniformly mixing ceramic powder, active carbon powder, bonding agents and active ingredient precursors; adding water for preparing slurry; performing strip extrusion forming; (2) drying forming materials; then, performing roasting in oxygen-deficient atmosphere to obtain the integral CO reduction denitration catalyst. The method provided by the invention has the advantages that the clean production of the CO reduction denitration catalyst can be realized; meanwhile, the use efficiency of the catalyst is improved.

Description

technical field [0001] The invention relates to a preparation method of an integral CO reduction denitration catalyst. Background technique [0002] In the process of fuel combustion or incineration, due to the incomplete combustion of fuel, in addition to NOx, the emitted flue gas usually contains considerable CO, such as coal-fired boiler flue gas, catalytic cracking unit regeneration flue gas and automobile exhaust However, the research on exhaust gas denitrification using CO as a reducing agent is currently mainly limited to automobile exhaust. Precious metal catalysts including platinum, palladium, etc. are a type of catalyst that has been studied more in CO reduction and denitrification catalysts, especially rhodium, as one of the catalysts with the highest CO+NO reaction activity, is widely used in catalytic converters for automobile exhaust gas However, due to the high price, people are looking for a catalytic material with reduced rhodium content or no rhodium, inc...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J23/86B01J23/755B01D53/86B01D53/56
Inventor 王明星阮宗林李欣魏晓霞姜阳
Owner CHINA PETROLEUM & CHEM CORP