pressure sensitive adhesive composition
A pressure-sensitive adhesive, pressure-sensitive adhesive technology, applied in the direction of adhesives, film/sheet adhesives, non-polymer adhesive additives, etc., can solve the problem of insufficient tight adhesion, pollution, pressure-sensitive adhesive Mixture residues, etc.
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preparation example 1
[0164] Preparation Example 1: Preparation of Acrylic Block Copolymer (A1)
[0165] 0.1 g of ethyl 2-bromoisobutyrate (EBiB) and 28.4 g of methyl methacrylate (MMA) were mixed with 12.4 g of ethyl acetate (EAc). The flask holding the resulting mixture was sealed with a rubber stopper, purged with nitrogen at about 25° C. for about 30 minutes, and stirred. Thereafter, dissolved oxygen was removed by bubbling. Then, 0.002 g of CuBr was added to the deoxygenated mixture 2 , 0.005g tris(2-pyridylmethyl)amine (TPMA), and 0.017g 2,2'-azobis(2,4-dimethylvaleronitrile) (V-65), then at about 67°C Soak in the reaction bath to initiate the reaction (polymerization of the first block). When the conversion of methyl methacrylate reached about 75%, a previously sparged mixture of the following was added in the presence of nitrogen: 310 g butyl acrylate (BA), 1.6 g hydroxybutyl acrylate (HBA), and 500 g Ethyl acetate (EAc). Subsequently, 0.006 g of CuBr was added to the reaction flask 2...
preparation example 2 and 3
[0166] Preparation Examples 2 and 3: Preparation of Acrylic Block Copolymers (A2) and (A3)
[0167] As listed in Table 1 below, a block copolymer was prepared in the same manner as in Preparation Example 1 except that the type of source material (monomer, etc.) and polymerization conditions used to polymerize the block copolymer were adjusted .
[0168] Table 1
[0169]
Embodiment 1
[0171] Preparation of pressure sensitive adhesive composition (coating solution)
[0172] Based on 100 parts by weight of the block copolymer (A1) prepared in Preparation Example 1, the following were mixed: 0.1 parts by weight of a crosslinking agent (Coronate LS commercially available from Nippon Polyurethane Industry Co., Ltd.), 0.5 parts by weight Multifunctional epoxy compound (N,N,N',N'-tetraglycidylethylenediamine), 1.0 parts by weight ionic liquid (FC-4400 commercially available from 3M), 0.01 parts by weight 2-methylimidazole (commercially available from Acros Pvt.Ltd.), 0.01 parts by weight of dibutyltin dilaurate (commercially available as DBTDL from AlfaAesar), and 0.4 parts by weight of a silane coupling agent containing a β-cyanoacetyl group (commercially available as AD M-812 from LG Chem. Ltd.), and then blending ethyl acetate as a solvent to achieve a coating solids content of about 10% to 13% by weight, thereby preparing a coating solution (i.e., pressure sen...
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