Unlock instant, AI-driven research and patent intelligence for your innovation.

Preparation method for Zn0.25Cd0.75S/Zn2GeO4 compound visible-light-driven photocatalyst

A visible light and catalyst technology, applied in the field of environmental pollution control, can solve the problems of low electron-hole separation efficiency and narrow light response range, and achieve the effects of improving the light absorption range, the preparation process is easy to operate, and the crystallinity is good.

Inactive Publication Date: 2017-06-23
UNIV OF JINAN
View PDF5 Cites 1 Cited by
  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Solved the problem of narrow photoresponse range and low electron-hole separation efficiency of photocatalyst in photocatalysis technology

Method used

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
View more

Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0019] Example 1 Zn 2 GeO 4 Preparation of one-dimensional nanowires

[0020] Preparation of Zn by Mixed Solvothermal Method 2 GeO 4 For one-dimensional nanowires, add 1 mM germanium dioxide and 2 mM zinc acetate dihydrate to 75 mL of a mixed solvent of ethylenediamine and deionized water with a volume ratio of 2:1 under magnetic stirring, and add 0.5 g MW =130000 The PVP was uniformly dispersed by ultrasonic wave and stirred for 10 h to obtain a mixed solution; the above mixed solution was transferred to an autoclave and reacted at 180 °C for 18 h; after the autoclave was gradually cooled to room temperature, it was centrifugally precipitated and used After washing with deionized water three times, the product was dried in an oven at 60 °C for 6 h.

Embodiment 2

[0021] Example 2 Zn 2 GeO 4 Preparation of one-dimensional nanowires

[0022] Preparation of Zn by Mixed Solvothermal Method 2 GeO 4 For one-dimensional nanowires, add 2 mM germanium dioxide and 4 mM zinc acetate dihydrate to 75 mL of ethylenediamine and deionized water with a volume ratio of 3:1 under magnetic stirring, and add 1 g MW =130000 The PVP was uniformly dispersed by ultrasonic, and stirred for 10 h to obtain a mixed solution; the above mixed solution was transferred to an autoclave, and reacted for 20 h at 190 °C; after the autoclave was gradually cooled to room temperature, centrifugal precipitation was used to After washing with deionized water three times, the product was dried in an oven at 60 °C for 6 h.

Embodiment 3

[0023] Example 3 Zn 2 GeO 4 Preparation of one-dimensional nanowires

[0024] Preparation of Zn by Mixed Solvothermal Method 2 GeO 4 For one-dimensional nanowires, under magnetic stirring, add 3 mM germanium dioxide and 6 mM zinc acetate dihydrate to 75 mL of a mixed solvent of ethylenediamine and deionized water with a volume ratio of 5:1, and add 2.0 g MW =130000 The PVP was uniformly dispersed by ultrasonic, and stirred for 10 h to obtain a mixed solution; the above mixed solution was transferred to an autoclave, and reacted at 200 °C for 24 h; after the autoclave was gradually cooled to room temperature, centrifuged to precipitate, and After washing with deionized water three times, the product was dried in an oven at 60 °C for 6 h.

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

PUM

No PUM Login to View More

Abstract

The invention discloses a preparation method for Zn0.25Cd0.75S / Zn2GeO4 compound visible-light-driven photocatalyst, and belongs to the technical field of environmental pollution control. The preparation method is characterized by comprising the following steps: firstly, preparing a Zn2GeO4 one-dimensional nanowire through a mixed solvothermal method; then, adopting a hydrothermal method to prepare the Zn0.25Cd0.75S / Zn2GeO4 compound visible-light-driven photocatalyst, and applying to the visible light catalytic degradation of pollutants MO (Methyl Orange) and AP (Acetaminophen). The preparation method disclosed by the invention has the advantages of simpleness in operation, stable performance, no other pollutants in a preparation process, wide application prospect and high use value.

Description

technical field [0001] The invention belongs to the technical field of environmental pollution control, in particular to a Zn 0.25 CD 0.75 S / Zn 2 GeO 4 Preparation method of composite visible light catalyst. Background technique [0002] At present, photocatalytic technology mainly uses photocatalysts to degrade organic pollutants under the illumination of ultraviolet light, visible light and infrared light. The principle of photocatalysis is to use light as energy to transition the electrons in the catalyst from the valence band to the conduction band, thereby generating hydroxyl radicals and holes, and degrading the pollutants adsorbed on the surface of the catalyst. Zn 2 GeO 4 It is considered as an n-type semiconductor with a large band gap, and the photogenerated electrons and holes are easily separated, but its large energy level difference is not easy to be excited. Zn 0.25 CD 0.75 The S band gap is narrow, easy to excite, and the energy level structure match...

Claims

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

Application Information

Patent Timeline
no application Login to View More
Patent Type & Authority Applications(China)
IPC IPC(8): B01J27/04B01J35/10C02F1/30C02F101/38
CPCC02F1/30B01J27/04C02F2101/40C02F2101/38C02F2305/10B01J35/39B01J35/61
Inventor 闫涛吴廷廷崔一哲蒋冠宇张伦文孙蒙闫良国杜斌
Owner UNIV OF JINAN