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Preparation method for high-viscosity, temperature-resisting and low-filtration-loss polyanionic cellulose

A technology of polyanion and cellulose, which is applied in the field of preparation of polyanion cellulose, can solve the problems of polyanion cellulose such as low viscosity, high fluid loss, insufficient temperature resistance, etc., and achieve simple and easy modification method, high filtration Increased loss and excellent performance

Inactive Publication Date: 2017-10-27
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The purpose of the present invention is to propose a method for preparing a high-viscosity and temperature-resistant polyanion cellulose, so as to solve the problems of low viscosity, high fluid loss and insufficient temperature resistance of the polyanion cellulose obtained by the existing preparation method

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] A method for preparing polyanionic cellulose with high viscosity, temperature resistance and low fluid loss. The specific operation method is as follows:

[0027] (1) Alkalization of cellulose: 1500g of 40% (w / w) sodium hydroxide aqueous solution and 1800g of 92% (v / v) ethanol aqueous solution are put into the kneader and mixed together in the kneader After cooling for 20 minutes, the temperature is lowered to 15° C., and 1000 g of refined cotton cellulose that has been preliminarily pulverized is put into the kneader, and alkali cellulose is obtained after an alkalinization reaction for 1.5 hours.

[0028] (2) Etherification of cellulose: 1100g of chloroacetic acid (prepared as a 50% aqueous solution) and alkali cellulose are mixed by spraying within 20-30min, etherification is reacted at 50℃ for 1h, and then the temperature is raised Etherification reaction at 75°C for 1h.

[0029] (3) Crosslinking of cellulose: Dissolve 7.5g of N,N-dimethylacrylamide and 0.0075g of potassi...

Embodiment 2

[0032] A method for preparing polyanionic cellulose with high viscosity, temperature resistance and low fluid loss. The specific operation method is as follows:

[0033] (1) Alkalization of cellulose: 1500g of 50% (w / w) sodium hydroxide aqueous solution and 1800g of 92% (v / v) ethanol aqueous solution are put into the kneader and mixed together in the kneader After cooling for 20 minutes, the temperature is lowered to 40° C., 1000 g of refined cotton cellulose that has been preliminarily pulverized is put into the kneader, and alkali cellulose is obtained after an alkalinization reaction for 1.5 hours.

[0034] (2) Etherification of cellulose: 1300g of chloroacetic acid (prepared as a 50% aqueous solution) and alkali cellulose are mixed by spraying within 20-30min, and the etherification reaction is carried out at 50℃ for 1h, and then the temperature is raised. Etherification reaction at 75°C for 2h.

[0035] (3) Cross-linking of cellulose: Dissolve 15g of N,N-dimethylacrylamide and ...

Embodiment 3

[0038] A method for preparing polyanionic cellulose with high viscosity, temperature resistance and low fluid loss. The specific operation method is as follows:

[0039] (1) Alkalization of cellulose: 1500g of 45% (w / w) sodium hydroxide aqueous solution and 1800g of 92% (v / v) ethanol aqueous solution are put into the kneader and mixed together in the kneader After cooling for 20 minutes, the temperature is lowered to 30° C., and the preliminarily pulverized 1000 g of refined cotton cellulose is put into the kneader, and alkali cellulose is obtained after 1.5 hours of alkalization.

[0040] (2) Etherification of cellulose: Mix 1200g of chloroacetic acid (prepared as an aqueous solution with a concentration of 50%) and alkali cellulose within 20-30 minutes by spraying, and etherify at 50°C for 1 hour, and then heat up Etherification reaction at 75℃ for 1.5h.

[0041] (3) Cross-linking of cellulose: 10g of N,N-dimethylacrylamide and 0.015g of potassium persulfate dissolved in 95% (v / v)...

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PUM

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Abstract

The invention discloses a preparation method for high-viscosity, temperature-resisting and low-filtration-loss polyanionic cellulose. The preparation method takes refined cotton as a cellulose raw material and comprises the following steps: (a) carrying out alkalinization on the cellulose; (b) carrying out etherification on the cellulose; (c) carrying out neutralization and washing; and (d) carrying out after-treatment on a product. The preparation method further comprises a micro-crosslinking reaction step; the micro-crosslinking reaction step is carried out after step (b) of carrying out the etherification on the cellulose is carried out; a micro-crosslinking reaction is realized by adding a crosslinking agent N,N-dimethylacrylamide into the cellulose and carrying out a crosslinking reaction. The polyanionic cellulose prepared by the method has the characteristics of high viscosity, high substitution degree, low filtration loss and good temperature resistance and has a certain industrial application prospect.

Description

Technical field [0001] The invention relates to a method for preparing polyanionic cellulose, in particular to a method for preparing high-viscosity polyanionic cellulose. Background technique [0002] Polyanionic cellulose (PAC for short) is a water-soluble ionic cellulase obtained by chemical modification based on natural cellulose. It is an important mud treatment agent in petroleum drilling. For drilling, completion, and national wells, it plays a role in viscosity increase, fluid loss reduction, and suspension. Due to the continuous expansion of the petroleum exploration field and the increasing average drilling depth, the quality requirements of PAC continue to increase, requiring PAC to have higher viscosity, salt resistance and temperature resistance. [0003] In terms of improving the quality of PAC, cellulose crushing, nitrogen sealing, increasing the ratio of solvent to liquid, adding antioxidants, etc. can be used to achieve the purpose of improving PAC viscosity, degr...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08B15/00C08B11/12C08B1/08C09K8/035
CPCC08B1/08C08B11/12C08B15/005C09K8/035C09K2208/08
Inventor 庞雨微袁俊秀封心领逯贵广靳志超
Owner CHINA PETROLEUM & CHEM CORP