Fluorine-modified organic silicon material as well as preparation method and application thereof
A technology of fluorine-modified silicone and fluorine materials, used in adhesive additives, non-polymer adhesive additives, polymer adhesive additives, etc. Expensive and other issues, to achieve high moisture resistance, good thermal shock resistance, and improve quality
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preparation example 1
[0060] This preparation example is used to illustrate the fluorine material-modified silicone resin provided by the present invention and its preparation process.
[0061] Add 1 mol of organic silicon shown in formula (3-1), 3 mol of organic silicon shown in formula (4-1), 4 mol of organic silicon shown in formula (5-1) and 1 mol of formula (6-1) in the three-necked flask ), mixed evenly, then added dropwise 0.03L of HCl solution with a concentration of 1% by weight at 10°C, and the dropwise addition was completed within 1h; then the reaction temperature was raised to 40°C and reacted at this temperature for 4h ;Raise the reaction temperature to 90°C for fractional distillation, and distill out the generated by-products. When the temperature of the distillation head reaches 80°C, stop the reaction and lower the temperature; then add 4.5g of ammonia water and 200ml of toluene, mix well, and start to heat up to 110°C , when the temperature of the distillation head reaches 86°C, ...
preparation example 2
[0064] This preparation example is used to illustrate the fluorine material-modified silicone resin provided by the present invention and its preparation process.
[0065] According to the process of Preparation Example 1, the difference is that the organosilicon added is 6 mol of organosilicon represented by formula (3-1), 7 mol of organosilicon represented by formula (4-1), and 4 mol of organosilicon represented by formula (5-1). The organosilicon shown in the formula (6-1) and 4 mol of the organosilicon shown in formula (6-1), other preparation conditions were kept consistent with the preparation example 1, finally obtained the silicone resin A2 modified by fluorine material.
preparation example 3
[0067] This preparation example is used to illustrate the fluorine material-modified silicone resin provided by the present invention and its preparation process.
[0068] According to the process of Preparation Example 1, the difference is that the organosilicon added is 5 mol of organosilicon represented by formula (3-1), 4 mol of organosilicon represented by formula (4-1), and 1 mol of organosilicon represented by formula (5-1). Organosilicon shown in 2mol formula (6-1), 4.5g of ammonia water is replaced by 7g of sodium bicarbonate solution, other preparation conditions are consistent with Preparation Example 1, and finally the organosilicon modified by fluorine material is obtained Resin A3.
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