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A kind of graphitized carbon purification method

A graphitized carbon and composite carbon technology, applied in chemical instruments and methods, carbon compounds, inorganic chemistry, etc., can solve problems such as difficulty in separating amorphous carbon, achieve excellent electromagnetic shielding performance, strong external destructive ability, and high energy density Effect

Active Publication Date: 2022-08-02
FUJIAN NORMAL UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] The technical problem to be solved by the present invention is to provide a low-cost graphitized carbon purification method and its application for the existing problem of difficult separation of amorphous carbon left in graphitized carbon. Amorphous carbon is removed from graphitized carbon to obtain pure graphitized carbon, and the prepared graphitized carbon materials exhibit excellent performance in energy storage, environmental treatment, functional plastics and other fields

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0024] 1. Dilute concentrated nitric acid to prepare 4 mol / L nitric acid solution;

[0025] 2. Soak 10 mg of one-dimensional composite carbon fiber in 25 mL of 4 mol / L nitric acid solution;

[0026] 3. Transfer the solution of the above step 2 to a 50 mL hydrothermal reaction kettle at a temperature of 170 °C, and react for 15 h. After the reaction kettle is cooled and filtered to obtain one-dimensional graphite carbon fibers;

[0027] 4. Wash the obtained one-dimensional graphite carbon fiber with distilled water and 95% alcohol for 3 times in sequence, after washing, the pH value is 6.5, and dry;

[0028] 5. Heat treatment at 500 °C for 30 min under the condition of vacuum degree -100torr while passing hydrogen / argon mixed gas through the dried one-dimensional graphite carbon fiber to remove the oxidized functional groups;

[0029] 6. Prepare a lithium ion electrode according to a conventional method: the prepared graphite carbon fiber is used as the working electrode, the ...

Embodiment 2

[0031] 1. Dilute concentrated nitric acid to prepare 6 mol / L nitric acid solution;

[0032] 2. Soak 10 mg of composite carbon nanofibers embedded with nickel particles in 20 mL of 6 mol / L nitric acid solution;

[0033] 3. Transfer the solution of the above step 2 to a 50 mL hydrothermal reaction kettle at a temperature of 150 °C, and react for 12 h. After the reaction kettle is cooled and filtered to obtain hollow carbon nanomaterials;

[0034] 4. The hollow carbon nanomaterials obtained were sequentially cleaned 3 times with distilled water and 95% alcohol, and the pH value after cleaning was 6.8, and dried;

[0035] 5. The dried hollow graphitized carbon nanomaterials are evacuated to a vacuum degree of -200 torr while being passed through a hydrogen / nitrogen gas mixture, and then heat-treated at 600 °C for 30 min to remove the oxidized functional groups;

[0036] 6. Prepare capacitor electrodes by conventional methods: use the prepared hollow graphitized carbon nanomateria...

Embodiment 3

[0038] 1. Dilute concentrated nitric acid to prepare 7 mol / L mixed acid, wherein the molar ratio of nitric acid to hydrochloric acid is 9.5:0.5;

[0039] 2. Soak 10 mg of two-dimensional composite carbon film in 25 mL of 7 mol / L mixed acid solution;

[0040] 3. Transfer the solution of the above step 2 to a 50 mL hydrothermal reaction kettle at a temperature of 180 °C, and react for 10 h. After the reaction kettle is cooled and filtered, a two-dimensional ultra-thin graphitized carbon film is obtained;

[0041] 4. The obtained two-dimensional ultra-thin graphitized carbon film is sequentially cleaned 3 times with distilled water and 95% alcohol, and the pH value is 6.5 after cleaning, and dried;

[0042] 5. The dried two-dimensional ultra-thin graphitized carbon film was evacuated to a vacuum degree of -300 torr while passing hydrogen / argon mixed gas, and then heat-treated at 700 °C for 30 min to remove impurity functional groups;

[0043] 6. Put the prepared material into wa...

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Abstract

The invention relates to a method for purifying graphitized carbon. The method includes the following steps: 1) preparing an acid solution with a concentration of 0.5-10 mol / L; 2) soaking the composite carbon in the acid solution to obtain a composite carbon / acid solution, wherein the composite carbon accounts for 1-80% of the weight of the acid solution; 3) The obtained composite carbon / acid solution is reacted under high temperature and high pressure, and the amorphous carbon left in the composite carbon is removed by selective etching of the composite carbon by acid to obtain graphitized carbon; 4) The obtained graphitized carbon is obtained Cleaning and heat treatment are successively performed to obtain pure graphitized carbon material. The invention has the following beneficial effects: the purification technology has the advantages of high efficiency, rapidity, high selectivity, and is not restricted by the morphology of the purified material; the graphitized carbon material prepared by the method of the invention has a wide range of applications.

Description

technical field [0001] The invention relates to a method for purifying graphitized carbon, in particular to a method for purifying graphitized carbon material by acid selective etching of amorphous carbon. Background technique [0002] Graphitized carbon materials have attracted attention in the fields of electronic devices, sensors, and energy storage due to their unique structural and physicochemical properties. Techniques such as template method and electrospinning technology can nanosize materials and have been widely used to prepare functional materials such as ordered mesoporous carbon, carbon nanofibers, and carbon nanotubes. For example, carbon nanofibers can be obtained by calcining electrospun polyacrylonitrile at a high temperature of 700 degrees, but the obtained carbon is an amorphous carbon material. Catalysts (nickel, cobalt, iron, etc.) can catalyze the transformation of amorphous carbon into graphitized carbon to obtain graphitized carbon. However, the eff...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C01B32/215
CPCC01B32/215
Inventor 李小燕陈育明陈庆华钱庆荣肖荔人李轩王曼茜李川平李瑞玲何佳波邱敏
Owner FUJIAN NORMAL UNIV