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Acrylate rubber as well as preparation method and application thereof

A technology of acrylate and rubber, which is applied in the field of acrylate rubber and its preparation, which can solve the problems of difficult industrialization, complex synthesis process, low gel content, etc., to avoid the use of solvents, stable reaction temperature, and oligomer content low effect

Active Publication Date: 2022-03-11
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] The purpose of the present invention is to provide a kind of preparation method of acrylate rubber in order to overcome the problem that the acrylate rubber synthesis process existing in the prior art is complicated and difficult to realize industrialization , acrylate rubber and its application, the preparation method can accurately control the polymerization heat during the polymerization reaction of acrylate rubber, realize the continuous production of acrylate rubber, the acrylate rubber thus obtained has high molecular weight and low gel content and low volatile

Method used

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Comparison scheme
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preparation example Construction

[0015] The first aspect of the present invention provides a kind of preparation method of acrylate rubber, it is characterized in that, this preparation method comprises the following steps:

[0016] S1. Premixing: premixing the polymerization monomer and the initiator to obtain a premix;

[0017] S2. Polymerization reaction: transfer the premixed material in step S1 to a polymerization reaction device for polymerization reaction;

[0018] Wherein, the polymerization reaction device is a tubular reactor and / or a twin-screw extruder.

[0019] In the present invention, after premixing the polymerization monomer and the initiator, bulk polymerization is carried out in a tubular reactor and / or a twin-screw extruder to obtain acrylate rubber.

[0020] In the present invention, the polymerized monomers containing acrylate monomers are bulk polymerized in tubular reactors and / or twin-screw extruders, which can significantly reduce the amount of polymerization caused by the difficult...

Embodiment 1

[0065] Put 100 parts of ethyl acrylate, 2.5 parts of vinyl chloroacetate and 0.06 parts of azobisisobutyronitrile at one time into a stirring mixing tank with temperature control below 40°C and mix thoroughly. After mixing, enter the tubular reaction through a metering pump. device (the length-to-diameter ratio is 4:1), the tubular reactor is controlled at 60°C, and the reaction time is 1h. The conversion rate of the polymerized monomer in the tubular reactor is 50%, and then enters the twin-screw extruder (the long-diameter The ratio is 32:1), the temperature of the reaction section of the twin-screw extruder is controlled at 80°C, the temperature of the extrusion section of the twin-screw extruder is controlled at 70°C, the shear speed of the extruder is 65r / min, and the extrusion time is 15min. Acrylate rubber A1 was prepared. Wherein, the polymerization temperature of the tubular reactor is 20° C. lower than that of the twin-screw extruder.

[0066] After testing, the num...

Embodiment 2

[0068] Put 100 parts of ethyl acrylate, 2.5 parts of vinyl chloroacetate and 0.1 part of azobisisobutyronitrile at one time into a stirring mixing tank with temperature control below 40°C and mix them thoroughly. After mixing, enter the tube reaction through a metering pump. device (length-to-diameter ratio is 4:1), the tubular reaction is controlled at 60°C, the reaction time is 0.8h, and the conversion rate of polymerized monomer in the tubular reactor is 55%, and then enters the twin-screw extruder (long-diameter The ratio is 32:1), the temperature of the reaction section of the twin-screw extruder is controlled at 80°C, the temperature of the extrusion section of the twin-screw extruder is controlled at 70°C, the shear speed of the extruder is 65r / min, and the extrusion time is 12min. Acrylate rubber A2 was prepared. Wherein, the polymerization temperature of the tubular reactor is 20° C. lower than that of the twin-screw extruder.

[0069] After testing, the number avera...

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Abstract

The invention relates to the field of rubber preparation, and discloses acrylate rubber as well as a preparation method and application thereof. The preparation method comprises the following steps: S1, premixing: premixing a polymeric monomer and an initiator to obtain a premix; s2, polymerization reaction: transferring the premix in the step S1 into a polymerization reaction device for polymerization reaction; wherein the polymerization reaction device is a tubular reactor and / or a double-screw extruder. According to the preparation method, the polymerization heat during the polymerization reaction of the acrylate rubber can be accurately controlled, the continuous production of the acrylate rubber is realized, and the acrylate rubber prepared by the method has low gel content and low volatile matter while having high molecular weight.

Description

technical field [0001] The invention relates to the field of rubber preparation, in particular to an acrylic rubber and its preparation method and application. Background technique [0002] Acrylate rubber is an elastomer obtained by copolymerization of acrylate as the main monomer. Its main chain is a saturated carbon chain and its side groups are polar ester groups. It has excellent heat resistance, aging resistance, oil resistance, ozone resistance, Anti-ultraviolet and other properties, using it to make oil-resistant rubber products used under high-temperature conditions has special advantages, and has now become the most cost-effective high-temperature oil-resistant special rubber. [0003] At present, the production methods of acrylate rubber mainly include suspension polymerization (represented by Goodrich Company of the United States) and emulsion polymerization (represented by Japan East Asia Paint Company). In addition, Du Pont has also developed a solution polyme...

Claims

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Application Information

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IPC IPC(8): C08F220/18C08F218/04C08F220/28C08F2/01C08F2/02C08F2/00
CPCC08F220/1802C08F2/01C08F2/02C08F2/001C08F218/20C08F220/1804C08F220/281
Inventor 杜影齐可非赵丽娜
Owner CHINA PETROLEUM & CHEM CORP