Metal organic framework derived carbon-based photo-thermal phase change energy storage material as well as preparation method and application thereof
A metal-organic framework and metal-organic framework technology, applied in the field of metal-organic framework-derived carbon-based photothermal phase change energy storage materials and their preparation, can solve the problem of ignoring the adjustment and enhancement effects of metal materials, the single function of carbon materials, and the preparation method. Cumbersome and other problems, to achieve the effect of enhancing stability and photothermal conversion ability, improving crystallization ability, and high degree of graphitization
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Embodiment 1
[0049] (1) Preparation of cobalt-based metal-organic framework (MOF)
[0050] Dissolve 3mmol of terephthalic acid and 3mmol of cobalt acetate tetrahydrate in 25ml of dimethyl sulfoxide, stir at room temperature for 12h, wash with N,N-dimethylformamide and ethanol three times as detergents, and place in a vacuum oven at 60°C Dry in medium for 24h.
[0051] (2) Preparation of metal-organic framework-derived carbon
[0052] The MOF powder in step (1) was raised to 1000°C at a rate of 5°C / min in a nitrogen atmosphere in a tube furnace, and kept at 1000°C for 3 hours, and the final product obtained was metal-organic framework-derived carbon 1 .
[0053] (3) Preparation of metal-organic framework-derived carbon-based composite phase change materials
[0054] Dissolve 0.6g of stearyl alcohol and 0.4g of MOF-derived carbon in step (2) in 15ml of ethanol, sonicate for 20min to dissolve the stearyl alcohol, and mix evenly. The ethanol is completely volatilized, and the obtained soli...
Embodiment 2
[0056] (1) Preparation of cobalt-based metal-organic framework (MOF)
[0057] Dissolve 3mmol terephthalic acid and 2mmol cobalt acetate tetrahydrate in 25ml dimethyl sulfoxide, stir at room temperature for 12h, wash three times with N,N-dimethylformamide and ethanol respectively, and place in a vacuum oven at 60°C Dry in medium for 24h.
[0058] (2) Preparation of metal-organic framework-derived carbon
[0059] The MOF powder in step (1) was raised to 1000°C at a rate of 5°C / min in a nitrogen atmosphere in a tube furnace, and kept at 1000°C for 3 hours, and the final product obtained was metal-organic framework-derived carbon 2 .
[0060] (3) Preparation of metal-organic framework-derived carbon-based composite phase change materials
[0061] Dissolve 0.6g stearyl alcohol and 0.4g MOF-derived carbon in step (2) in 15ml ethanol, sonicate for 20min to dissolve stearyl alcohol, and mix evenly. The ethanol is completely volatilized, and the obtained solid is the composite phas...
Embodiment 3
[0064] (1) Preparation of cobalt-based metal-organic framework (MOF)
[0065] Dissolve 3mmol terephthalic acid and 1mmol cobalt acetate tetrahydrate in 25ml dimethyl sulfoxide, stir at room temperature for 12h, wash with N,N-dimethylformamide and ethanol three times as detergents, and place in a vacuum oven at 60°C Dry in medium for 24h.
[0066] (2) Preparation of metal-organic framework-derived carbon
[0067] The MOF powder in step (1) was raised to 1000°C at a rate of 5°C / min under nitrogen in a tube furnace, and kept at 1000°C for 3 hours, and the final product obtained was metal-organic framework-derived carbon 3.
[0068] (3) Preparation of metal-organic framework-derived carbon-based composite phase change materials
[0069] Dissolve 0.6g stearyl alcohol and 0.4g MOF-derived carbon in step (2) in 15ml ethanol, sonicate for 20min to dissolve stearyl alcohol, and mix evenly. The ethanol is completely volatilized, and the obtained solid is the composite phase change ma...
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