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Magnesium-based hydrogen storage alloy block and preparation method thereof

A technology of magnesium-based hydrogen storage alloy and magnesium block, which is applied in the direction of metal extrusion control equipment, metal processing equipment, manufacturing tools, etc., can solve the problems of unsatisfactory hydrogen absorption performance, achieve lower temperature, high cycle times, The effect of reducing the hydrogen charging and discharging time

Active Publication Date: 2022-05-17
GUANGDONG INST OF NEW MATERIALS
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] But at present, magnesium-based hydrogen storage materials mainly exist in the form of powder, and the hydrogen absorption performance of bulk magnesium-based hydrogen storage materials under short-term and low-pressure conditions is not ideal.

Method used

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Effect test

preparation example Construction

[0028] The present application proposes a method for preparing a magnesium-based hydrogen storage alloy block, which includes the following steps: the magnesium block, the magnesium-nickel master alloy, and the magnesium-rare-earth master alloy are mixed according to the mass ratio of magnesium element, nickel element, and rare earth element to 50-90:10 -20:1-10 smelting and pouring to obtain alloy ingots; then the alloy ingots are hot-extruded into alloy rods and processed into alloy electrodes; then the alloy electrodes are atomized and powdered to obtain magnesium-nickel-rare earth hydrogen storage Alloy powder, the magnesium-nickel-rare earth hydrogen storage alloy powder is pressed into shape.

[0029] By adding a magnesium-nickel master alloy to the raw material, the nickel contained in it can form a solid solution with the magnesium in the raw material. The binding force between nickel and hydrogen is weak, and the formation enthalpy of hydride is low. Nickel has a catal...

Embodiment 1

[0067] This embodiment provides a magnesium-based hydrogen storage alloy block, which is prepared by the following method:

[0068] According to the composition of Mg:Ni:Y mass ratio of 80:10:10, mix magnesium block, magnesium-nickel master alloy and magnesium rare earth master alloy, and melt in a well-type resistance furnace at 720°C and 500r / min for 2 hours , Pouring at 690°C for 20min. The above smelting and pouring process are in SF 6 and CO 2 under the protection of the mixed gas.

[0069] The poured alloy ingot was hot-extruded at 450° C. with an extrusion deformation ratio of 100:1 to obtain an alloy rod. Before extrusion, the mold is preheated at a preheating temperature of 200°C, and the extrusion cylinder is preheated at a preheating temperature of 250°C.

[0070] Process the prepared alloy rod into an alloy electrode, put the electrode into the plasma rotating electrode powder making equipment for atomization and powder making, the electrode rotation speed is 1...

Embodiment 2

[0074] This embodiment provides a magnesium-based hydrogen storage alloy block, which is prepared by the following method:

[0075] According to the composition of Mg:Ni:Y mass ratio of 80:15:5, mix magnesium block, magnesium-nickel master alloy and magnesium rare earth master alloy, and melt in a well-type resistance furnace at 710°C and 200r / min for 3h , Pouring at 680°C for 5 minutes. The above smelting and pouring process are in SF 6 and CO 2 under the protection of the mixed gas.

[0076] The poured alloy ingot was hot-extruded at 430° C. with an extrusion deformation ratio of 200:1 to obtain an alloy rod. Before extrusion, the mold is preheated at a preheating temperature of 100°C, and the extrusion barrel is preheated at a preheating temperature of 100°C.

[0077] Process the prepared alloy rods into alloy electrodes according to the required size, put the electrodes into the plasma rotating electrode powder making equipment for atomization and powder making, the el...

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Abstract

The invention discloses a magnesium-based hydrogen storage alloy block and a preparation method thereof, and belongs to the technical field of magnesium-based hydrogen storage materials. The method comprises the following steps that a magnesium block, a magnesium-nickel intermediate alloy and a magnesium-rare earth intermediate alloy are smelted and poured according to the mass ratio of the magnesium element to the nickel element to the rare earth element being (50-90): (10-20): (1-10), and an alloy ingot is obtained; performing hot extrusion on the alloy ingot to form an alloy bar and processing the alloy bar into an alloy electrode; and then the alloy electrode is subjected to atomization powdering, magnesium-nickel-rare earth hydrogen storage alloy powder is obtained, and the magnesium-nickel-rare earth hydrogen storage alloy powder is subjected to compression molding. The method is simple, easy to operate and suitable for preparing the magnesium-based hydrogen storage alloy blocks in batches. The magnesium-based hydrogen storage alloy block prepared from the magnesium-based hydrogen storage alloy material can achieve high hydrogen absorption capacity within a short time under low pressure, and can be recycled up to 1500-2000 times.

Description

technical field [0001] The invention relates to the technical field of magnesium-based hydrogen storage materials, in particular to a magnesium-based hydrogen storage alloy block and a preparation method thereof. Background technique [0002] Magnesium-based hydrogen storage material is a medium-temperature hydrogen storage material with high safety, easy storage and transportation, and its low relative density and low cost are considered to be the most valuable hydrogen storage materials for application and development. [0003] But at present, magnesium-based hydrogen storage materials mainly exist in the form of powder, and the hydrogen absorption performance of bulk magnesium-based hydrogen storage materials under short-term and low-pressure conditions is not ideal. [0004] In view of this, the present invention is proposed. Contents of the invention [0005] One of the objectives of the present invention is to provide a method for preparing a magnesium-based hydroge...

Claims

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Application Information

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IPC IPC(8): C22C23/00C22C23/06C22C1/03B22F3/02B22F9/14B21C31/00
CPCC22C23/00C22C23/06C22C1/03B22F9/14B22F3/02B21C31/00C22C2202/04Y02E60/32
Inventor 韩胜利郑开宏张玉桧徐静
Owner GUANGDONG INST OF NEW MATERIALS