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Photoelectrocatalysis method for degrading sulfamethoxazole by utilizing synergistic effect of microorganisms

A technology of sulfamethoxazole and synergistic effect, applied in the field of bioelectrochemistry, to achieve the effects of reducing energy consumption, efficient degradation, and efficient and thorough degradation

Pending Publication Date: 2022-06-28
SUN YAT SEN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

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Problems solved by technology

However, most of the current research on SMX degradation focuses on the anaerobic oxidation and conversion of biological anodes. In this process, various electron donors such as acetate and lactate are required. Microorganisms need to use external energy to play their role. , therefore, it is necessary to find a more energy-saving method for degrading SMX

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  • Photoelectrocatalysis method for degrading sulfamethoxazole by utilizing synergistic effect of microorganisms
  • Photoelectrocatalysis method for degrading sulfamethoxazole by utilizing synergistic effect of microorganisms
  • Photoelectrocatalysis method for degrading sulfamethoxazole by utilizing synergistic effect of microorganisms

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Embodiment 1

[0035] A photoelectric catalytic method for degrading sulfamethoxazole by the synergistic action of microorganisms, comprising the following steps:

[0036] Step 1: The substrate is made of FTO fluorine-doped tin dioxide conductive glass, and the photoanode is prepared by hydrothermal method; in order to facilitate the connection of the titanium wire for conduction, the edge of the conductive surface of the glass is scraped by about 0.3cm, and the conductive surface of the glass is scraped at 550 in a muffle furnace. ℃ temperature annealing for 3h;

[0037] Step 2: Build a light energy-driven microbial electrolysis system (PMES) and build a dual-chamber reactor; the volumes of the anode and cathode compartments are 15 mL and 30 mL, respectively, and the two polar compartments are separated by a cation exchange membrane (CEM). The anode electrode is prepared using well coated with TiO 2 FTO conductive glass, the cathode adopts carbon brush electrode (16 strands × 3cm), and the...

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Abstract

The invention belongs to the technical field of bioelectrochemistry, and particularly relates to a photoelectrocatalysis method for degrading sulfamethoxazole by utilizing a synergistic effect of microorganisms, which comprises the following steps: step 1, preparing a photoanode by adopting FTO fluorine-doped tin dioxide conductive glass as a substrate and adopting a hydrothermal method; scraping the edge of the conductive surface of the glass by about 0.3 cm in order to facilitate the connection of the titanium wire for electric conduction, and annealing in a muffle furnace at the temperature of 550 DEG C for 3 hours; 2, a light energy driven microbial electrolysis system (PMES) is built, and a double-chamber reactor is built; and step 3, preparing catholyte and anolyte which are reasonable in structure, reducing energy consumption by adopting a light energy driven microbial electrolysis system (PMES), and realizing efficient degradation of sulfamethoxazole by utilizing the synergistic effect of homoacetogens and sulfate reducing bacteria. Meanwhile, the degradation pathway of SMX is determined by measuring intermediate products at different time points.

Description

technical field [0001] The invention relates to the technical field of bioelectrochemistry, in particular to a photoelectric catalysis method for degrading sulfamethoxazole by the synergistic action of microorganisms. Background technique [0002] Sulfamethoxazole (SMX) is one of the most frequently detected drugs in aquatic ecosystems. It is a broad-spectrum bacteriostatic sulfonamide antibiotic, which is widely used in various industries. Synthesis results in stunted growth and reproduction of microorganisms. Since the accumulation and persistence of sulfamethoxazole in the environment can have detrimental effects on aquatic organisms and human health, it is crucial to explore methods to effectively remove sulfamethoxazole from wastewater. [0003] At present, the treatment technology for sulfamethoxazole wastewater mainly includes three aspects: physical adsorption removal, chemical advanced oxidation removal and biodegradation removal. Among them, biological treatment ...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C02F3/00C02F3/34C02F101/38
CPCC02F3/005C02F3/34C02F2101/40C02F2101/38
Inventor 骆海萍朱曦白加敏刘广立张仁铎
Owner SUN YAT SEN UNIV