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Organic amine desulfurization desorption accelerant as well as preparation method and application thereof

A technology of accelerator and organic amine, which is applied in the field of organic amine desulfurization and desorption accelerator and its preparation, to achieve the effects of improving desorption efficiency, reducing desorption energy consumption, and accelerating mass transfer rate

Pending Publication Date: 2022-07-29
双盾环境科技有限公司 +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Patent CN112452109A invented the double-tower double-effect + low pressurization two deep desorption process, which improves the desorption of SO by the desulfurization absorbent 2 efficiency; patent CN108722118A adopts the recovery of the thermal energy of the top material of the desorption tower to generate low-pressure steam, which is used as the heat source of the reboiler at the bottom of the desorption tower after compression and pressurization, which reduces the consumption of raw steam, but these methods all need to carry out the actual desulfurization device Equipment modification

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0036] The organic amine absorbent used was N,N-dihydroxyethylpiperazine, the amine concentration was 20% by weight, concentrated sulfuric acid was added, the pH value of the solution was adjusted to 7, and the rest was water. After absorbing the simulated flue gas for 3 hours, the rich amine solution was obtained, and the rich amine solution was divided into 4 parts. One part was directly heated and desorbed at 105 °C for 4 hours without desorption accelerator, as a comparison; the other three parts were added to 1-3 in Table 1 respectively. No. desorption accelerator, and then heated the rich amine solution at 105 °C for 4 h. The weight ratio of the desorption accelerator to the organic amine desulfurizer is 0.05. The process effect is expressed by desorption rate and desorption energy consumption, and the results are shown in Table 2.

[0037] The desorption rate of table 2 embodiment one and desorption energy consumption result

[0038] Desorption accelerator ...

Embodiment 2

[0040] The organic amine absorbent used is the mixed amine of N,N-dihydroxyethylpiperazine and N-hydroxyethylpiperazine, and the amine concentration is 10% (weight), and concentrated sulfuric acid is added to adjust the pH value of the solution to 6.5 , and the rest is water. After absorbing the simulated flue gas for 6 hours, the rich amine solution was obtained. The rich amine solution was divided into 4 parts, and one part was directly heated and desorbed at 105 °C for 4 hours without adding desorption accelerator; for comparison, the remaining three parts were added to 4-6 in Table 1. No. desorption accelerator, and then heated the rich amine solution at 105 °C for 4 h. The weight ratio of the desorption accelerator to the organic amine desulfurizer is 0.05. The process effect is expressed by desorption rate and desorption energy consumption, and the results are shown in Table 3.

[0041] The desorption rate of table 3 embodiment two and desorption energy consumption res...

Embodiment 3

[0044] The organic amine absorbent used is the mixed amine of N,N-dihydroxypropylpiperazine and N-hydroxyethylpiperazine, the amine concentration is 20% (weight), and concentrated sulfuric acid is added, and the pH value of the solution is adjusted to 6.5 , and the rest is water. After absorbing the simulated flue gas for 5 hours, the rich amine solution was obtained. The rich amine solution was divided into 4 parts, and one part was directly heated and desorbed at 105 °C for 4 hours without adding desorption accelerator; for comparison, the remaining three parts were added to 7-9 in Table 1 respectively. No. desorption accelerator, and then heated the rich amine solution at 105 °C for 4 h. The weight ratio of desorption accelerator to organic amine desulfurizer was 0.10. The process effect is expressed by desorption rate and desorption energy consumption, and the results are shown in Table 4.

[0045] The desorption rate of table 4 embodiment three and desorption energy con...

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PUM

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Abstract

The invention discloses an organic amine desulfurization desorption accelerant as well as a preparation method and application thereof, and belongs to the technical field of industrial flue gas desulfurization. The desorption accelerant comprises 30-50 parts by weight of an acidic activating agent, 5-20 parts by weight of a complexing auxiliary agent and 30-65 parts by weight of water. The preparation method comprises the following steps: firstly, adding the acidic activator into water for reaction to form a solution A, and then dropwise adding the complexing aid into the solution A for continuous reaction to obtain the desorption accelerant. When the desorption accelerant is used, the desorption accelerant is added into the organic amine desulfurizing agent according to a proportion, or is added into an absorbed rich amine solution or a desorbed lean amine solution. The desorption accelerant can weaken the binding force between piperazine organic amine and sulfurous acid, sulfuric acid and the like, the mass transfer rate of SO2 from a liquid phase to a gas phase is increased, and the desorption efficiency is improved; in addition, generation of thermal-stability amine salt in the desulfurization process can be inhibited, the absorption rate and desorption rate of the organic amine on SO2 are increased, the desorption effect of the organic amine is improved, and desorption energy consumption is reduced.

Description

technical field [0001] The invention relates to the technical field of industrial flue gas desulfurization, in particular to an organic amine desulfurization and desorption accelerator and a preparation method and application thereof. Background technique [0002] Piperazine organic amine wet flue gas desulfurization technology has high desulfurization efficiency and recovered SO 2 It has the advantages of high purity and recyclable absorbent, and has been successfully commercialized; however, in practical engineering, the absorbed rich amine solution needs to be heated to 5-10°C above the boiling point of the solution for thermal desorption, and the desorption temperature is high. The low desorption efficiency and large steam consumption result in the high cost of organic amine desulfurization, which restricts its wide application. Ultrasound and decompression can speed up the desorption rate under certain conditions, but will increase equipment investment and operating co...

Claims

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Application Information

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IPC IPC(8): B01D53/96B01D53/50B01D53/78
CPCB01D53/96B01D53/78B01D53/50B01D2258/0283
Inventor 魏凤玉宋小良王麒麟徐光泽
Owner 双盾环境科技有限公司