Titania thin film possessing high catalytic activity under visible light and preparation method
A high catalytic activity, titanium dioxide technology, applied in the direction of catalyst activation/preparation, chemical instruments and methods, physical/chemical process catalysts, etc., can solve the problems of high heat treatment temperature, waste of energy, difficulties in practical application, etc., and achieve high photocatalytic activity Effect
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[0012] The invention provides a titanium dioxide thin film with high catalytic activity under visible light and a preparation method thereof. Technical concept of the present invention is such:
[0013] According to the semiconductor defect theory, the addition of Sb ions can change the TiO 2 The corresponding energy level structure enables it to expand and absorb in the range of visible light. And by sol-gel method on TiO 2 LiNO was added to the sol 3 method that can reduce TiO 2 The crystal transition temperature of the film from amorphous to anatase phase, and under low temperature heat treatment conditions, the denser anatase phase TiO 2 film. Therefore, simultaneously doping Sb and Li ions into TiO 2 After sol, TiO with higher photocatalytic performance can be obtained at a lower heat treatment temperature 2 film.
[0014] The composition of the titanium dioxide thin film with high catalytic activity is by weight percentage:
[0015] 10%-30% tetrabutyl titanate, ...
Embodiment 1
[0026] (1) Pour 54% ethanol, 15% tetrabutyl titanate, 15% acetylacetone and 1% hydrochloric acid into the reaction vessel, and stir at room temperature for 0.5-1 hour;
[0027] (2) Slowly pour 15% water into the solution prepared in step (1), and stir at room temperature for 1-2 hours;
[0028] (3) Add the sol to the coating equipment, clean the surface of the glass to be coated, and put it into the coating equipment to coat the film. Generally, the coating can be carried out by pulling method, rotation method, etc., and the glass after coating Heat treatment, the heat treatment temperature is 350 ° C, and naturally cooled to room temperature, that is, TiO 2 film.
Embodiment 2
[0030] (1) TiO 2 Sol preparation:
[0031] Take 15% of isopropyl titanate, 15% of acetylacetone, 50% of propanol, 15% of water and 1% of hydrochloric acid by weight percentage, and prepare with steps (1) and (2) in Example 1;
[0032] (2) Add 2% lithium nitrate and 2% antimony chloride to the sol prepared in step (1), and continue to stir for 2-4 hours;
[0033] (3) Coating film
[0034] With embodiment 1.
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