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Method for preparing aperture gradient homogeneous Ti-Al intermetallic compound filter membrane

A technology of intermetallic compounds and filter membranes, applied in chemical instruments and methods, membrane technology, semi-permeable membrane separation, etc., can solve problems such as short service life, poor structure stability of metal materials, poor formability and sintering performance of ceramic particles, etc. , to achieve the effect of improving filtration performance and service life, improving anti-oxidation performance and excellent mechanical properties

Inactive Publication Date: 2007-03-28
CHENGDU INTERMENT TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

These preparation technologies often have disadvantages such as complex process, high cost, and difficulty in controlling the pore size of the filter membrane.
Compared with the preparation process, the quality of inorganic membranes is limited by the materials used to a greater extent
For metal materials, their oxidation resistance and acid and alkali corrosion resistance are often poor, which greatly restricts the use environment of the filter membrane, and the structure stability of metal materials is poor, and the service life is short. At the same time, due to hydrogen embrittlement Difficult to compound with other dense membranes
For ceramic materials, because of its hard and brittle phase, solid particle sintering method is used to prepare filter membranes. The formability and sintering performance of ceramic particles are often poor, and the energy consumption in the production process is high. At the same time, ceramics are brittle and difficult to weld and assemble. Disadvantages limit the application of ceramic membranes

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] Ti powder with a particle size of 100-150 μm and Al powder with a particle size of 50-100 μm are used for mixing according to the composition ratio of Ti-46.5at.% Al; then molded under a pressure of 200 MPa, and the Al foil is placed in the The end of the punch of the ordinary molding machine is made into a composite sheet blank with a diameter of 50mm and a thickness of 1-2mm; the sintering adopts a two-stage reaction method, the atmosphere is vacuum, and the vacuum degree is controlled at 1×10 -2 ~1×10 -3 Pa, the low-temperature pre-reaction temperature is 600°C, the holding time is 60min, the high-temperature short-term reaction temperature is 1300°C, and the holding time is 20min; after the reaction is completed, the cooling rate is controlled at 40°C / min; Gradient homogeneous sheet filter membrane with a porosity of 40-45% and an open porosity of 30-35%. It also has good oxidation resistance and corrosion resistance.

Embodiment 2

[0020] Ti powder with a particle size of 20-50 μm and Al powder with a particle size of 50-100 μm are used for mixing according to the composition ratio of Ti-48at.% Al; then cold isostatic pressing is used to form a tubular billet, and the Al foil is closely attached to the On the outer side of the core rod, the taper of the core rod is 0.5°, and the pressure is 150MPa. After a small amount of machining, a composite tubular forming blank with an outer diameter of 30mm, an inner diameter of 28-29mm, and a height of 200mm is obtained; the sintering adopts a two-stage reaction method, The atmosphere is vacuum, and the vacuum degree is controlled at 1×10 -2 ~1×10 -3 Pa; the low-temperature pre-reaction temperature is 620°C, the holding time is 40min, the high-temperature short-term reaction temperature is 1260°C, and the holding time is 30min; after the reaction is completed, the cooling rate is controlled at 30°C / min. In this way, a TiAl intermetallic compound pore size gradien...

Embodiment 3

[0022] Ti powder with a particle size of 150-200μm and Al powder with a particle size of 20-50μm are used for mixing according to the composition ratio of Ti-48.5at.%Al; molded under a pressure of 200MPa to make a diameter of 50mm and a thickness of 1-2mm flake billet; then the composite forming billet is made by immersing the surface of Al liquid, the immersion temperature is 700°C, the immersion time is 2min, and the thickness of the immersion layer is 20μm; sintering adopts low-pressure hot isostatic pressing , the atmosphere is Ar gas, the pressure is 0.1MPa, the low-temperature pre-reaction temperature is 620°C, and the holding time is 40min; the high-temperature short-term reaction temperature is 1300°C, and the holding time is 10min; after the reaction, the cooling rate is controlled at 20°C / min. The thus prepared TiAl intermetallic compound pore size gradient homogeneous sheet filter membrane has a porosity of 35-40%, an open porosity of 25-35%, and has good oxidation r...

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PUM

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Abstract

The present invention relates to production of semipermeable membrane, in particular it relates to a special preparation method of semipermeable membrane for separation process. Said preparation method includes the following steps: firstly, utilizing die pressing forming or isostatic cool pressing forming mode to obtain composite formed blank; in the following sintering process utilizing low-temperature prereaction and high-temperature short-term reaction two-stage vacuum sintering synthesizing process to prepare TiAl intermetallic compound pore diameter gradient homogeneous fitlering membrane. Said filtering membrane can be directly used as microfiltering membrane and nanofiltering membrane with excellent performance.

Description

Technical field: [0001] The invention relates to the production of a semi-permeable membrane, a special preparation method for the semi-permeable membrane used in a separation process, in particular to a method for preparing a homogeneous TiAl intermetallic compound filter membrane with a pore size gradient. Background technique: [0002] At present, the materials used for inorganic membranes mainly include ceramic bodies, such as alumina and glass, and metals such as copper, nickel, and stainless steel. Ultrafiltration and microfiltration membranes; glass membranes prepared by phase separation; microporous membranes or dense membranes prepared by chemical vapor deposition and electroless plating. These preparation technologies often have disadvantages such as complex process, high cost, and difficulty in controlling the pore size of the filter membrane. Compared with the preparation process, the quality of inorganic membranes is limited by the materials used to a greater e...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01D71/02
Inventor 贺跃辉江垚林小芹汤义武徐南平高海燕张启修
Owner CHENGDU INTERMENT TECH