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Transparent laminated film and its mfg. method

A manufacturing method and a barrier technology, which are applied in the field of barrier laminate films and their manufacture, can solve the problems of coating obstacles, film breakage, and inability to directly use coating laminates and the like

Inactive Publication Date: 2004-10-06
TOHCELLO CO LTD (JP)
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0008] In addition, although the composition of polyvinyl alcohol and (meth)acrylic polymer has good barrier properties, according to the research of the present inventors, it is known that when the thermoplastic resin used as the base material is polypropylene, the coating cannot be directly used. layering
[0009] On the other hand, the laminate described in Patent Document 8 improves the water resistance of the polyvinyl alcohol polymer, and has good barrier properties and transparency. However, when the viscosity of the coating liquid is too high, it will hinder the coating. , The countermeasure for this problem is to reduce the viscosity. In this regard, when using an ethylene-vinyl alcohol copolymer with a degree of polymerization of 500 or less, there is a problem that when the laminate is stretched to about 10 times, it cannot be followed and the film is broken.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0113] An ethylene-vinyl alcohol copolymer (polymerization degree: 500, saponification degree: 98.5 mol%, ethylene content: 8 mol%) was dissolved in hot water to obtain a 5% aqueous solution A. Separately, polyacrylic acid (manufactured by Wako Pure Chemical Industries, Ltd., polymerization degree: 2080, 25% aqueous solution) was neutralized with sodium hydroxide at 10%, and diluted with water to obtain a 5% aqueous solution B. Then, A and B were mixed at each ratio shown in Table 1 to prepare a coating liquid.

[0114] The coating solution was coated on the corona-treated surface of a biaxially stretched polyester film (trade name "EMBLET PET12" made by UNITIKA) with a thickness of 12 μm using a Mayer bar, and dried with a hot air dryer to form a thick 1.5 μm barrier layer. Then, this film was fixed on a cardboard, and heat-treated in an oven at 200° C. for 15 minutes to obtain a barrier laminated film.

[0115] The properties of the obtained barrier laminated film were eva...

Embodiment 2

[0129] The 5% aqueous solution A of the ethylene-vinyl alcohol copolymer obtained in Example 1 and the aqueous solution B of polyacrylic acid were mixed at a ratio of A:B=25:75 to obtain a coating liquid.

[0130] This coating solution was applied to a 12 μm thick aluminum oxide vapor-deposited biaxially stretched polyethylene terephthalate film (trade name "TL-PET H#12" manufactured by Tocel Corporation) with a Meyer bar. The alumina vapor-deposited surface was dried with a hot air dryer to form a barrier layer with a thickness of 0.5 μm. Then, this laminated film was fixed on a thick paper, and heat-treated in an oven at 200° C. for 5 minutes to obtain a barrier laminated film.

[0131] The oxygen permeability of the measured barrier laminated film is 3.0ml / m 2 · day · MPa. And the light transmittances of the obtained barrier laminated film at wavelengths of 500 nm and 400 nm were measured to be 91% and 89%.

Embodiment 3

[0133] Using the same coating liquid as in Example 2, except that the thickness of the barrier layer was 0.25 μm, a barrier laminated film was obtained in the same manner as in Example 2. The oxygen permeability of the obtained barrier laminated film was 2.9ml / m 2 ·day·MPa, the light transmittance of wavelength 500nm and 400nm is 92% and 89%.

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PUM

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Abstract

Provided is a gas barrier laminated film having excellent transparency and a high gas barrier property under a high humid condition with no fear of reduction of transparency with cross-linking, and also to provide a method for producing the gas barrier laminated film. In the gas barrier laminated film, a gas barrier layer of a composition comprising an ethylene / vinyl alcohol copolymer (b1) having an ethylene content of 1-19 mol% and a (meth)acrylic acid polymer (b3) is laminated at least on one surface of a substrate film. When used, as a substrate film, of a film on whose surface is formed a deposited layer of an inorganic oxide or an OPP film on whose surface is formed a modified propylene polymer layer, a gas barrier film having more excellent adhesiveness to the substrate can be obtained.

Description

technical field [0001] The present invention relates to a laminated film having excellent barrier properties such as transparency, oxygen barrier property and vapor barrier property, especially high temperature barrier properties, and excellent barrier properties when used as packaging materials and The production method thereof, specifically, relates to a barrier layer formed on at least one side of a film substrate as a barrier layer composed of an ethylene-vinyl alcohol copolymer and a (meth)acrylic acid polymer composition. Permeable laminated membrane and method for its manufacture. Background technique [0002] In recent years, materials with barrier properties such as oxygen barrier properties or vapor barrier properties have attracted much attention, such as vacuum evaporation method, sputtering method, ion plating method, chemical vapor growth method, etc. Transparent barrier film of inorganic oxides such as silicon and alumina. Since this kind of transparent barr...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B32B27/36B32B27/32C08J7/043C08J7/048
CPCY10T428/31928Y10T428/31909Y10S428/91C08J7/047B32B27/32Y10T428/31938C08J2429/00C08J2433/00Y10T428/31667C08J7/0427C08J7/048C08J7/043E02D17/083E02D17/04B32B2307/31B32B27/306B32B2307/518B32B2398/20B32B27/08B32B27/36B32B2307/7242B32B2305/72
Inventor 中村修户田钦一
Owner TOHCELLO CO LTD (JP)