Red-light organic luminous material and use
A light-emitting material and organic technology, applied in the field of red light organic light-emitting materials and their preparation, can solve the problems of poor stability, poor film formation, lack of electron transport ability, etc., and achieve the effects of high thermal stability and high luminous efficiency
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Embodiment 1
[0031] Synthesis of 2-(4-(N,N'-dimethyl)anilino)-3-phenoxyflavone (A):
[0032] The first step is the synthesis of 4-(N,N’-dimethylamino)benzaldehyde:
[0033] The reaction route is as follows:
[0034]
[0035]The newly distilled phosphoryl chloride (0.023 mol) was added to a 50 ml pear-shaped flask containing 9 ml of freshly distilled and dried dimethylformamide (DMF) at 0°C until completely dissolved. 0.02 mol (N,N'-dimethyl)aniline was dissolved in 3.5 ml of newly distilled and dried dimethylformamide (DMF) and added to the above-mentioned pear-shaped flask to prepare a reaction solution. The reaction solution was heated to about 95°C, stirred for 2 hours, the temperature was lowered to room temperature and poured into 30 ml of ice water. Adjust the system to pH=7 with saturated sodium acetate, a light green precipitate appears, and place it in the refrigerator overnight. The precipitate was filtered and washed with water and n-hexane, and the precipitate was dissolved in et...
Embodiment 2
[0045] The synthesis method of 2-(4-(N,N'-dimethylamino)phenyl)-3-biphenoxy-7-fluoroflavonoid (B) refers to Example 1. The first step yield is 79%. The yield in the second step was 70%, and the yield in the third step was 80%. IR(cm -1 ): 3282, 3105, 2942, 1718, 1624, 1508, 1438, 1376, 965, 732; MS (EI) m / z (%): 454 (M+, 8); Anal.calcd for C 29 H 24 FNO 3 : C76.65, H5.28, N3.08; found C76.71, H5.25, N3.03.
Embodiment 3
[0047] Synthesis method of 2-(4-(N,N'-dimethylamino)phenyl)-3-p-phenoxyphenoxy-7-(N,N'-dimethylamino)flavonoid (C) Referring to Example 1, the yield in the first step was 79%, the yield in the second step was 50%, and the yield in the third step was 69%. IR(cm -1 ): 3241, 3054, 2978, 1721, 1614, 1538, 1448, 1354, 951, 714; MS (EI) m / z (%): 495 (M+, 16); Anal.calcd forC 31 H 30 N 2 O 4 : C75.30, H6.07, N5.67; found C75.25, H56.10, N5.71.
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