Five-carbon or six-carbon monosaccharide-L-menthoxyacetyl acid monoester compound as well as preparation method and application thereof
A six-carbon monosaccharide and acetic acid monoester technology, which is applied in the field of monosaccharide monoester tobacco humectants, five-carbon or six-carbon monosaccharide-L-menthoxyacetic acid monoester compounds, and can solve the problem of water content in finished cigarettes The effect of smoking comfort is not really satisfactory, the dryness and irritation are enhanced, and the influence of tobacco is greater, so as to achieve the effects of smoking safety, comfortable and harmonious aroma, and easy promotion and application
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Embodiment 1
[0030] Preparation of 6-(L-menthoxyacetic acid)-D-glucopyranosyl ester (compound I):
[0031] Add 18.0 g (0.1 mol) of D-glucose, 25.72 g (0.12 mol) of L-menthoxyacetic acid and 200 ml of pyridine in sequence in the reaction flask, stir at room temperature until the solid dissolves, then add 2.46 g of 4-dimethylaminopyridine ( 0.02 mol), after cooling the reaction liquid to 0-5°C, add 26.83g (0.13 mol) of dicyclohexylcarbodiimide, continue to stir and react for 30min at 0-5°C, then naturally warm up to room temperature and stir for 18h, the reaction ends Afterwards, the solvent was evaporated under reduced pressure, the residue was dissolved in 200 ml of ethyl acetate, and the solid was precipitated by filtration. The filtrate was washed successively with 50 ml of 10% aqueous hydrochloric acid solution, 50 ml of saturated aqueous sodium carbonate solution and 50 ml of saturated brine to obtain acetic acid Ethyl ester solution over anhydrous Na 2 SO 4 Dry, filter, and evaporat...
Embodiment 2
[0033] Preparation of 6-(L-menthoxyacetic acid)-D-galactopyranosyl ester (compound II):
[0034] The operation process is the same as in Example 1, except that D-glucose is replaced with D-galactose, and dicyclohexylcarbodiimide is 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide hydrochloride Substitute for pyridine N , N -Dimethylformamide was substituted to obtain 6-(L-menthoxyacetic acid)-D-galactopyranosyl ester with a yield of 63.5%; HR-TOFMS (+Q) m / z : 377.2183 ( [C 18 h 32 o 8 +H] + Calculated value: 377.2175 ).
Embodiment 3
[0036] Preparation of 6-(L-menthoxyacetic acid)-D-mannopyranosyl ester (compound III):
[0037] The operation process is the same as in Example 1, except that D-glucose is replaced by D-mannose, and dicyclohexylcarbodiimide is replaced by N-ethoxycarbonyl-2-ethoxy-1,2-dihydroquinoline to obtain 6-(L-Mengoxyacetic acid)-D-mannopyranosyl ester, yield 52.7%; HR-TOFMS (+Q) m / z : 377.2178( [C 18 h 32 o 8 +H] + Calculated value: 377.2175 ).
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