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Method for catalyzing complete hydrogenation of polyalphaolefin into saturated alkane

A technology of complete hydrogenation and α-olefins, which is applied in the field of fine chemicals, can solve the problems of double bond destruction, quality and performance degradation, loss of meaning, etc., and achieve the effect of simple preparation process, good stability and low cost

Inactive Publication Date: 2013-07-10
FUDAN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Even if it is not in such an environment, the oxygen in the air will destroy the double bond, thereby greatly reducing the quality and performance of the product and losing its original meaning

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] Ni (1%) / Nano Al 2 O 3 The catalyst is prepared as follows:

[0024] Weigh the weight ratio as nickel nitrate: water: nano alumina = 0.5:13.3:10, and dissolve it with distilled water. Then add nano-alumina, and sonicate in an ultrasonic machine for 5-60 minutes after being completely mixed. After the mixing is complete, ventilate and age at room temperature for 5-24 hours. Then it is ventilated and dried at 70°C to obtain the dried mixture and then heated and roasted in a muffle furnace at a heating temperature of 400-600°C. The roasting time is 1-10h. Before use, put the catalyst in a mixture of hydrogen and nitrogen (H 2 Content 1%-100%) in the presence of 200 oC -500 o Reduction in C range to obtain Ni / Al 2 O 3 catalyst.

[0025] Add 10 grams of Ni (1%) / nano Al 2 O 3 The catalyst is put into a stainless steel reaction tube with a diameter of 8 mm, and the polyalphaolefin (C 100 H 200 ) After mixing with hydrogen, pass it into the reaction tube and enter the catalytic ...

Embodiment 2

[0027] Ni (3%) / Nano Al 2 O 3 The catalyst is prepared as follows:

[0028] Weigh the weight ratio as nickel nitrate: water: nano alumina = 1.5: 13: 10, and dissolve it with distilled water. Then add nano-alumina, and sonicate in an ultrasonic machine for 5-60 minutes after being completely mixed. After the mixing is complete, ventilate and age at room temperature for 5-24 hours. Then it is ventilated and dried at 70°C to obtain the dried mixture and then heated and roasted in a muffle furnace at a heating temperature of 400-600°C. The roasting time is 1-10h. Before use, put the catalyst in a mixture of hydrogen and nitrogen (H 2 Content 1%-100%) in the presence of 200 oC -500 o Reduction in C range to obtain Ni / Al 2 O 3 catalyst.

[0029] Add 10 grams of Ni (3%) / nano Al 2 O 3 The catalyst is put into a stainless steel reaction tube with a diameter of 8 mm, and the polyalphaolefin (C 80 H 160 ) After mixing with hydrogen, pass it into the reaction tube and enter the catalytic b...

Embodiment 3

[0031] Ni (5%) / Nano Al 2 O 3 The catalyst is prepared as follows:

[0032] Weigh the weight ratio as nickel nitrate: water: nano alumina=2.5:12.6:10, and dissolve it with distilled water. Then add nano-alumina, and sonicate in an ultrasonic machine for 5-60 minutes after being completely mixed. After the mixing is complete, ventilate and age at room temperature for 5-24 hours. Then it is ventilated and dried at 70°C to obtain the dried mixture and then heated and roasted in a muffle furnace at a heating temperature of 400-600°C. The roasting time is 1-10h. Before use, put the catalyst in a mixture of hydrogen and nitrogen (H 2 Content 1%-100%) in the presence of 200 oC -500 o Reduction in C range to obtain Ni / Al 2 O 3 catalyst.

[0033] Add 10 grams of Ni(5%) / nano Al 2 O 3 The catalyst is put into a stainless steel reaction tube with a diameter of 8 mm, and the polyalphaolefin (C 60 H 120 ) After mixing with hydrogen, pass it into the reaction tube and enter the catalytic bed ...

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PUM

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Abstract

The invention belongs to the technical field of fine chemistry, in particular to a method for complete hydrogenation of polyalphaolefin into saturated alkane. The method synthesizes a Ni / nano Al2O3 catalyst by using an immersion process. The polyalphaolefin can be catalytically reduced into saturated alkane under the conditions that: the Ni / nano Al2O3 catalyst is used, the reaction temperature is60 to 200 DEG C, the pressure range is from 1.0 to 6.0Mpa, the liquid hourly space velocity is 0.4 to 0.8<-1>, and the molar ratio of hydrogen to polyalphaolefin is 5 to 20. The method of the invention is simple in process and low in cost and has a bright application prospect.

Description

Technical field [0001] The invention belongs to the technical field of fine chemicals, and specifically relates to a supported Ni / nano Al 2 O 3 The catalyst is used in a method for the complete hydrogenation of polyalphaolefins to synthesize saturated alkanes. Background technique [0002] After the 1970s, with the technological progress of various engines and other mechanical equipment and the increasingly pressing requirements of "energy saving" and "environmental protection", the main properties of lubricating oil such as viscosity-temperature, volatility, and thermal oxidation stability were also proposed. In response to increasingly stringent requirements, the quality performance of natural mineral base oils is approaching the limit, and it is difficult to re-modulate products with higher performance and specifications. This directly promotes the development of synthetic base oils. In recent years, due to the stricter specifications of lubricating oil, especially internal c...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07C5/03C07C9/22B01J23/755
Inventor 沈伟侯磊熊德胜俞超孙超周海波黄镇申高岭秦枫徐华龙
Owner FUDAN UNIV