Potassium ion binding polymers for pharmaceutical compositions
A kind of technology of acrylic polymer, copolymer
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Embodiment 1
[0151] Synthesis of Core-Shell Crosslinked Polyallylamine Particles
[0152] In this process, spherical particles are formed by the reverse suspension method, in which the prepolymer (polyallylamine) is crosslinked with epichlorohydrin. Block copolymers can be used to increase the mechanical stability of the droplets during the crosslinking reaction and can provide an outer shell membrane that is chemically immobilized on the core particle.
[0153] General method for synthesizing block copolymers
[0154] Block copolymers are prepared by the RAFT living radical polymerization method. Use dithiocarbazide compound as reversible chain transfer agent (CTA) and diazonitrile radical initiator (AMVN) in the reaction, represent respectively as follows:
[0155]
[0156] Synthesis of the first block of poly(n-butyl acrylate-co-tert-butyl acrylate)
[0157] n-Butyl acrylate (25 g, 195 mmol) and tert-butyl acrylate (25 g, 195 mmol) were mixed with CTA (173:1 monomer:CTA, 616 mg, 2...
Embodiment 2
[0206] Synthesis of 1,3 Diaminopropane / Epichlorohydrin Crosslinked Particles (Denoted as: Particle-Pi-4-s)
[0207] The reactor used was a 3 L volume baffled three neck round bottom flask equipped with oil bath heating, a water cooled reflux condenser and a mechanical stirrer with a 3 inch propeller. First, a solution of 1,3-diaminopropane (90.2g, 1.21mole) dissolved in 90.2g of water, a surfactant (6.4g of branched chain sodium dodecylbenzenesulfonate dissolved in 100g of water) and 1kg of toluene were added to the in this reactor. The initial batch was stirred at 600 rpm for 2 minutes and then at 300 rpm for 10 minutes before the addition of epichlorohydrin. During the remainder of the test, the same stirring speed was maintained throughout. The reaction solution was heated to 80°C and maintained at this temperature throughout the test period.
[0208] In another container, a solution of 40% by mass of epichlorohydrin in toluene was prepared. 1.2 equivalents of epichlo...
Embodiment 3
[0214] Preparation of Ethylcellulose Shell / 1,3-Diaminopropane Epichlorohydrin Crosslinked Core Particles prepare
[0215] The granules obtained in Example 2 were spray coated with a shell of ethylcellulose polymer using a Wurster fluid bed coater 2""-4"" / 6"" portable unit. The fluidized bed unit was run using a 30% by weight solids aqueous emulsion ( ECD, FMC Corporation), deposited on the core particles to form a coating with an average thickness of 5 microns.
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