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Preparation method of magnetic nanometer material for treating 2-chlorine-3-pyridinecarbaldehydes waste

A pyridine formaldehyde, magnetic nanotechnology, applied in water/sewage treatment, chemical instruments and methods, adsorption water/sewage treatment, etc., can solve the problems of affecting adsorption efficiency, easy loss, affecting water quality, etc., and achieve the effect of wide concentration range

Inactive Publication Date: 2012-08-15
CHANGZHOU YAHUAN ENVIRONMENTAL PROTECTION TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0002] 2-Chloro-3-pyridine carboxaldehyde, due to the existence of pyridine ring, makes the chemical properties of the molecule stable, is a component that is difficult to remove in formaldehyde wastewater, and is highly irritating; when the concentration is low, it inhibits the growth of microorganisms in water; when it is high, it makes protein deterioration , microorganisms are difficult to survive, seriously affecting water quality
However, nano-scale particles are extremely small, and they are easily lost when filtered through a microporous membrane, and the adsorbent is dispersed in an aqueous solution to form a gel, which is not conducive to solid-liquid separation and affects adsorption efficiency.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0023] Place 1.5g tetrabutylammonium phosphate and 4.5g cobalt nitrate hexahydrate in a 100mL beaker, add 5.0mL concentrated nitric acid, 30mL deionized water, stir and dissolve; place the mixture solution in an ultrasonic water bath with a frequency of 30KHz for 2h , Add 10mL of sodium hydroxide solution with a concentration of 1.0mol / L, and use an external magnetic field to separate and dry the resulting paste to obtain Co 2 O 3 Precipitation: The precipitate obtained above was washed with acetone and deionized water three times in sequence, and then placed in 50 mL of 0.2mol / L NaBH 4 Activated in the solution for 2h, filtered by a microporous membrane, and separated by a magnetic field to obtain Co 2 O 3 The solid powder was dried in a vacuum drying oven at a constant temperature of 130°C for 30 minutes, cooled to room temperature, and 15 mL of triethanolamine with a concentration of 1.5 mol / L was added; in an ultrasonic water bath with a frequency of 20 KHz for 20 minutes, se...

example 2

[0027] Put 2.5g of tetrabutylammonium phosphate and 5.0g of cobalt nitrate hexahydrate in a 100mL beaker, add 6.0mL of concentrated nitric acid and 35mL of deionized water in sequence, after stirring and dissolving, place the mixture solution in an ultrasonic water bath with a frequency of 30KHz 2.5h, add 12mL of sodium hydroxide solution with a concentration of 1.0mol / L, and use an external magnetic field to separate and dry the resulting paste to obtain Co 2 O 3 precipitation. The precipitate obtained above was washed with acetone and deionized water three times in turn, and placed in 50 mL with a concentration of 0.3mol / LNaBH 4 After activation treatment in solution for 2.5h, after filtration by microporous membrane, Co 2 O 3 The solid powder was dried in a constant temperature vacuum drying oven at 130°C for 38 minutes, cooled to room temperature, and 18 mL of triethanolamine at a concentration of 1.5 mol / L was added. Finally, it was separated in an ultrasonic water bath wit...

example 3

[0031] Put 3.0g tetrabutylammonium phosphate and 5.5g cobalt nitrate hexahydrate in a 100mL beaker, add 6.5mL concentrated nitric acid and 40mL deionized water successively, stir and dissolve, then place the mixture solution in an ultrasonic water bath with a frequency of 30KHz 3h, add 13mL of sodium hydroxide solution with a concentration of 1.0mol / L, use an external magnetic field to separate and dry the resulting paste to obtain Co 2 O 3 precipitation. The precipitate obtained above was washed with acetone and deionized water 3 times each, and then placed in 50mL with a concentration of 0.4mol / LNaBH 4 Activated in the solution for 3 hours, filtered by a microporous membrane, and separated by a magnetic field to obtain Co 2 O 3 The solid powder was dried in a thermostatic vacuum drying oven at 130°C for 45 minutes, cooled to room temperature, and 22 mL of triethanolamine with a concentration of 1.5 mol / L was added. Finally, it was separated in an ultrasonic water bath with a f...

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Abstract

The invention discloses a preparation method of a magnetic nanometer material for treating 2-chlorine-3-pyridinecarbaldehydes waste water, comprising the following steps of: putting 1.5-3.0g of tetrabutylammonium phosphate and 4.5-6.0g of cobalt nitrate hexahydrate into a 100mL beaker, adding 5.0-7.5mL of concentrated nitric acid and 30-45mL of deionized water, stirring and dissolving; placing the mixture into an ultrasonic water bath with the frequency of 30KHz for 2-3h, adding 10-15mL of NaOH with the concentration of 1.0mol / L, and separating and drying paste obtained after reaction by utilizing an external magnetic field to obtain Co2O3 sediment; washing the sediment three times respectively with acetone and deionized water, activating for 2-4h in 50mL of NaBH4 solution with the concentration of 0.2-0.5mol / L, filtering by using a microporous membrane, separating by a magnetic field to obtain solid powder, drying in a 130-DEG C constant temperature vacuum drying oven for 30-50min, cooling to the room temperature, and adding 15-25mL of triethanolamine with the concentration of 1.5mol / L; and carrying out ultrasonic water bath with the frequency of 20KHz for 20-25min, and separating by utilizing the external magnetic field.

Description

technical field [0001] The invention relates to a material preparation method for treating 2-chloro-3-pyridine formaldehyde waste water, in particular to a preparation method of a magnetic nanometer material, and belongs to the technical field of formaldehyde waste water treatment. Background technique [0002] 2-Chloro-3-pyridine carboxaldehyde, due to the existence of pyridine ring, makes the chemical properties of the molecule stable, is a component that is difficult to remove in formaldehyde wastewater, and is highly irritating; when the concentration is low, it inhibits the growth of microorganisms in water; when it is high, it makes protein deterioration , microorganisms are difficult to survive, seriously affecting water quality. [0003] At present, domestic and foreign researchers are limited to chemical and biological methods for the treatment of formaldehyde wastewater. Oxidation technology has simple process, good oxidation treatment effect and no secondary poll...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J20/06B01J20/28B01J20/30C02F1/28C02F1/58C02F101/34C02F101/36
Inventor 雷春生雷思宇谢芳
Owner CHANGZHOU YAHUAN ENVIRONMENTAL PROTECTION TECH