Fully-aromatic thermotropic liquid crystal polyester resin composition, molded object, and led reflector
A thermotropic liquid crystal and all-aromatic technology, applied in reflective reflectors, liquid crystal materials, semiconductor devices, etc., can solve the problems of reduced light reflectivity of reflectors, reduced LED brightness, and reduced output efficiency, achieving less discoloration, Excellent heat resistance, sufficient light reflectance effect
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preparation example Construction
[0079] As the preparation method of LCP of the present invention, for example, the following method can be enumerated: p-hydroxybenzoic acid, the above-mentioned aromatic dicarboxylic acid and the above-mentioned aromatic dihydroxy compound are composed of 65 mol % to 78 mol%, 11 mol%~17.5 mol% and 11 mol%~17.5 mol% were added, and melt polycondensation was carried out.
[0080] In the production of the LCP of the present invention, in order to shorten the melt polycondensation time and reduce the influence of the heat history in the process, it is preferable to carry out the melt polycondensation after acetylating the hydroxyl groups of the above-mentioned monomers in advance. In addition, in order to simplify the process, acetylation is preferably performed by supplying acetic anhydride to the monomer in the reaction tank, and the acetylation process is preferably performed using the same reaction tank as the melt polycondensation step. That is, it is preferable to carry out...
Embodiment
[0107] Hereinafter, the present invention will be described more specifically by way of examples, but the present invention is not limited to the following examples.
[0108] [First Example and Comparative Example]
[0109]
[0110] First, a production example of a wholly aromatic thermotropic liquid crystal polyester is shown below. In addition, Table 1 shows the monomer composition (mol %) and melting point of each polyester produced.
manufacture example 1
[0111] (Manufacture Example 1: Manufacture of Whole Aromatic Thermotropic Liquid Crystal Polyester (A))
[0112] With SUS 316 as a material, there is a double-helical stirring blade and an internal volume of 1700L polymerization tank (manufactured by Kobe Steel Co., Ltd.) to add p-hydroxybenzoic acid (manufactured by Ueno Pharmaceutical Co., Ltd.) 207.2kg (1.5 kilomoles), para Phthalic acid (manufactured by Mitsui Chemicals Co., Ltd.) 31.1 kg (0.19 kilomole), isophthalic acid (manufactured by A.G. International Chemical Co., Inc.) 17.3 kg (0.1 kilomole), 4,4'-dihydroxybiphenyl ( Honshu Chemical Industry Co., Ltd.) 54.3kg (0.29 kilomoles), as a catalyst, potassium acetate (KISHIDA CHEMICAL Co., Ltd.) 0.05kg and magnesium acetate (KISHIDA CHEMICAL Co., Ltd.) 0.15kg, two The decompression of the polymerization tank-nitrogen gas injection is carried out for nitrogen replacement, and then 215.7 kg (2.11 kilomoles) of acetic anhydride is further added, the rotation speed of the stir...
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Abstract
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