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Preparation method for stable perovskite solar cell light absorption layer

A light-absorbing layer and solar cell technology, applied in circuits, photovoltaic power generation, electrical components, etc., can solve the problems of unstable surface and uneven roughness of perovskite light-absorbing layer, achieve good chemical stability, overcome surface roughness, etc. Inhomogeneity, the effect of improving moisture resistance and UV resistance

Inactive Publication Date: 2016-08-17
TIANJIN VOCATIONAL INST
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0007] The purpose of the present invention is to provide a method for preparing a perovskite solar cell light-absorbing layer using organosilicon nanoparticles as a dispersant and a protective film, so as to overcome the instability and surface deterioration of the perovskite light-absorbing layer prepared by the existing method. rough uneven defect

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0037] PbI 2 Reagent 46.1g (100mmol) and CH 3 NH 3 Add 15.9g (100mmol) of reagent I into 200g dimethylformamide solvent, stir at 60-70°C for 12 h to obtain CH 3 NH 3 PB 3 Clear solution.

[0038] Mix 0.89g (5mmol) of methyltriethoxysilane, 16g (350mmol) of absolute ethanol, and 0.75g (40mmol) of deionized water, and then add 0.25g (1mmol) of hydriodic acid aqueous solution with a concentration of 50% by mass , make the pH of the solution 2-3, carry out the hydrolysis reaction at 60-70° C. for 4 hours, and obtain a 5% mass percent concentration of organosilicon nanoparticle dispersant solution. Add it to CH with stirring 3 NH 3 PB 3 CH containing silicone dispersant is obtained in solution 3 NH 3 PB 3 Clear solution. Then add 1 g of n-butyltin ethanol solution with a concentration of 5% by mass, add anhydrous ethanol solvent to adjust the solution quality to 310 g, and filter the solution to obtain a light-absorbing layer coating solution, which is transferred to a ...

Embodiment 2

[0041] PbI 2 Reagent 46.1g (100mmol) and CH 3 NH 3 Add 15.9g (100mmol) of reagent I into 200g dimethylformamide solvent, stir at 60-70°C for 12 h to obtain CH 3 NH 3 PB 3 Clear solution.

[0042] Mix 0.83g (4mmol) of tetraethoxysilane, 0.18g (1mmol) of methyltriethoxysilane, 16g (350mmol) of absolute ethanol, and 0.75g (40mmol) of deionized water, and then add 50% by mass 0.25 g (1 mmol) of aqueous solution of hydroiodic acid, the pH of the solution is 2-3, and the hydrolysis reaction is carried out at 30-40° C. for 4 hours to obtain an organic silicon nanoparticle dispersant solution. Add it to CH with stirring 3 NH 3 PB 3 CH containing silicone dispersant is obtained in solution 3 NH 3 PB 3 Clear solution. Anhydrous ethanol solvent was added to adjust the solution to 310 g, and the solution was precisely filtered to obtain a light-absorbing layer coating solution, which was transferred to a black plastic bottle for storage.

[0043] Use a needle tube to drop the...

Embodiment 3

[0045] PbI 2 Reagent 46.1g (100mmol) and CH 3 NH 3 Add 15.9g (100mmol) of reagent I into 200g dimethylformamide solvent, stir at 60-70°C for 12 h to obtain CH 3 NH 3 PB 3 Clear solution.

[0046] Mix 0.83g (4mmol) of tetraethoxysilane, 0.25g (1mmol) of silicone coupling agent KH570, 16g (350mmol) of absolute ethanol, and 0.75g (40mmol) of deionized water, and then add 50% concentration by mass 0.25 g (1 mmol) aqueous solution of hydroiodic acid, the pH of the solution is set to 2-3, and the hydrolysis reaction is carried out at 30-40° C. for 4 hours to obtain an organic silicon nanoparticle dispersant solution. Add it to CH with stirring 3 NH 3 PB 3 CH containing silicone dispersant is obtained in solution 3 NH 3 PB 3 Clear solution. Anhydrous ethanol solvent was added to adjust the solution to 310 g, and the solution was precisely filtered to obtain a coating solution for the light-absorbing layer.

[0047] Use a needle tube to drop the light-absorbing layer coat...

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PUM

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Abstract

The invention relates to a preparation method for a stable perovskite solar cell light absorption layer taking organic silicon nanoparticles as a dispersing agent and a protection film. PbI<2> and CH<3>NH<3>I solid are added to a dimethyl formamide organic solvent to be reacted and dissolved to obtain a CH<3>NH<3>PbI<3> solution; an organic silicon nanoparticle dispersing agent solution and an ethyl alcohol solution of a curing agent are added and then are filtered precisely to obtain a light absorption layer coating liquid; the coating liquid is added to a conductive glass substrate with a compact layer in a dropwise manner in a glove box, and the coating liquid is coated uniformly by a wire rod coating device; after the solvent is evaporated and dried in the air, the conductive glass substrate is coated with the coating liquid repeatedly; and finally, the conductive glass substrate is dried by hot air at a temperature of 90-110 DEG C for 30min to form a black perovskite light absorption layer with a smooth surface and uniform crystallization. After the perovskite light absorption layer is placed in the air for 30 days, the surface color, the surface resistance and water contact angle are not changed obviously; and the perovskite light absorption layer shows high chemical stability.

Description

technical field [0001] The invention relates to a method for preparing a stable light-absorbing layer of a perovskite solar cell, especially a method for preparing a light-absorbing layer of a perovskite solar cell using organic silicon nanoparticles as a dispersant and a protective film, which belongs to new energy and new technologies. material field. technical background [0002] Solar cells based on organometallic halide perovskite structured light-absorbing materials are called perovskite solar cells. At present, their photoelectric conversion efficiency has exceeded 20%, and it is expected to reach 50% in the future. In the future, they can be made into colorful thin film cell decorations. Installed on the surface of buildings to promote the development of photovoltaic integrated buildings. Although the photoelectric conversion efficiency data of perovskite solar cells are constantly being refreshed, insufficient attention has been paid to the existing problems in its...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): H01L51/42H01L51/44H01L51/48
CPCH10K71/12H10K30/00Y02E10/549
Inventor 李建生胡兴兰刘炳光
Owner TIANJIN VOCATIONAL INST