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Preparation method of graphene in specific size

A specific size and graphene technology, applied in graphene, chemical instruments and methods, inorganic chemistry, etc., can solve the problem of high cost and achieve the effect of low cost, high efficiency and good size controllability

Inactive Publication Date: 2016-10-12
王奉瑾
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Chemical vapor deposition can produce large-size, high-quality graphene films, but the cost is high at this stage, and the generated graphene needs to be attached to the substrate

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] The present embodiment provides a kind of preparation method of graphene of specific size, and concrete steps are as follows:

[0022] A: Use copper foil with a size of 2*2mm as the catalytic substrate, clean the surface with hydrochloric acid, remove the oxide layer on the surface of the copper foil, dry it and place it in the reactor;

[0023] B: Into the reactor, a helium gas with a flow rate of 600 sccm was introduced for 0.5 h to remove impurity gases, and then a hydrogen gas with a flow rate of 500 sccm was introduced;

[0024] C: Raise the temperature of the copper foil to 970°C, and feed in methane with a flow rate of 600 sccm. The methane is cracked to generate carbon atoms. With the assistance of hydrogen, the carbon atoms are adsorbed on the copper surface and grow into graphene;

[0025] D: Rapidly cool down to room temperature, take out the product, and separate and transfer graphene and copper foil by mechanical peeling method. The time required for the r...

Embodiment 2

[0027] The present embodiment provides a kind of preparation method of graphene of specific size, and concrete steps are as follows:

[0028] A: Use nickel foil with a size of 1*2mm as the catalytic substrate, clean the surface with hydrochloric acid, remove the oxide layer on the surface of the nickel foil, dry it and place it in the reactor;

[0029] B: Into the reactor, a helium gas with a flow rate of 600 sccm was introduced for 0.5 h to remove impurity gases, and then a hydrogen gas with a flow rate of 300 sccm was introduced;

[0030] C: Raise the temperature of the nickel foil to 1050°C, and feed ethylene with a flow rate of 400 sccm. The ethylene is cracked to generate carbon atoms. With the assistance of hydrogen, the carbon atoms are adsorbed on the surface of the nickel foil and grow into graphene;

[0031] D: Rapidly cool down to room temperature, take out the product, and use mechanical stripping method to separate and transfer graphene from nickel foil. The time...

Embodiment 3

[0033] The present embodiment provides a kind of preparation method of graphene of specific size, and concrete steps are as follows:

[0034] A: Use a hexagonal copper-nickel alloy sheet with a side length of 1mm as the catalytic substrate, clean the surface with hydrochloric acid, remove the oxide layer on the surface of the copper-nickel alloy, dry it and place it in the reactor;

[0035] B: Into the reactor, the argon gas with a flow rate of 500 sccm was introduced for 0.5 h to remove impurity gases, and then the hydrogen gas with a flow rate of 400 sccm was introduced;

[0036] C: Raise the temperature of the copper-nickel alloy to 800°C, and feed in acetylene with a flow rate of 500 sccm. The acetylene is cracked to generate carbon atoms. With the assistance of hydrogen, the carbon atoms are adsorbed on the surface of the copper-nickel alloy and grow into graphene;

[0037] D: Rapidly cool down to room temperature, take out the product, and separate and transfer graphene ...

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Abstract

The invention provides a preparation method of graphene in a specific size. A metal foil in a specific size is used as a catalyst matrix, and a carbon source is introduced to generate the graphene in the specific size on the surface of the metal foil. The specific steps are as follows: A, performing acid pickling on the metal foil in the specific size to remove a surface oxidation layer; B, exhausting a foreign gas in a reactor, and introducing a catalyst gas; C, raising the temperature of the metal foil to 600 to 1,200 DEG C, introducing a gaseous carbon source, enabling the gaseous carbon source to be subjected to splitting decomposition to produce carbon atoms, and enabling the carbon atoms to be adsorbed on the surface of the metal foil, so as to produce the graphene; D, rapidly cooling to the room temperature, so as to separate the metal foil and the graphene. The method has the advantages of low cost, high efficiency, good controllability of size, high applicability to mass production, and the like.

Description

technical field [0001] The invention relates to a method for preparing graphene, in particular to a method for preparing graphene with a specific size. Background technique [0002] Graphene is a two-dimensional crystal composed of carbon atoms with only one atomic thickness. Graphene is the thinnest and hardest nanomaterial in the world. It is almost completely transparent and only absorbs 2.3% of light; its thermal conductivity is as high as 5300 W / (m K), which is higher than that of carbon nanotubes and diamonds. The electron mobility exceeds 15 000 cm2 / (V s), which is higher than carbon nanotubes or silicon crystals, while the resistivity is only about 10-6 Ω cm, which is lower than copper or silver, and is the material with the smallest resistivity in the world . These excellent characteristics make it have a wide range of applications and good application prospects, and can be used in high-performance nanoelectronic devices, composite materials, field emission materi...

Claims

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Application Information

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IPC IPC(8): C01B31/04
CPCC01B2204/32
Inventor 王奉瑾
Owner 王奉瑾