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Method for preparing battery capacitor composite electrode by dry method

A composite electrode and battery capacitor technology, which is applied in battery electrodes, electrode manufacturing, electrode rolling/calendering, etc., can solve the problems of electrode density drop, device charge and discharge capacity drop, etc., and achieve increased compaction density, energy density and The effect of cycle life and simple process

Active Publication Date: 2017-05-10
NINGBO CRRC NEW ENERGY TECH CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, due to the hybrid battery capacitor, a certain proportion of capacitor carbon is added to one or both electrodes of the positive and negative electrodes of the lithium battery, which leads to a decrease in the electrode density and a decrease in the charge and discharge capacity of the device in the process.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0029] LiMnPO 4 , activated carbon, additive S metallocene complex, PTFE and carbon nanotubes are mixed at a ratio of 44:44:2:5:5, and mixed at a high speed for 1h to form a positive electrode dry powder; the obtained mixed powder is passed through a powder press at 5t-40t Press down to make a 145 μm thick continuous positive electrode dry electrode film; on the front and back of the 20 μm thick corroded aluminum foil, evenly coat a 3 μm thick conductive adhesive by dip coating, and apply the above conductive adhesive layer to a dry electrode film with the same width Put it on the conductive adhesive, and pass through the hot rolling roller, the composite film is thinned and pressed tightly on the porous aluminum foil to obtain a positive composite electrode with a thickness of 260 μm, the rolling ratio is 19%, and the electrode density is 1.31g / cm 3 , compared with the conventional wet electrode, the rolling ratio is 12%, and the electrode density is 1.13g / cm 3 . In the co...

Embodiment 2

[0031]Mix artificial graphite, hard carbon, PTFE and carbon nanotubes at a ratio of 68:22:5:5, and mix at high speed for 1 hour to form a negative electrode mixed dry powder; press the obtained mixed powder into a continuous dry electrode with a thickness of 55 μm Diaphragm. On the front and back of the 9μm thick copper foil, apply a 2μm thick conductive adhesive evenly by dip coating, place the dry electrode film with the same width as the above conductive adhesive layer on the conductive adhesive, and pass it through a hot rolling roller, The composite film is thinned and pressed tightly on the porous aluminum foil to obtain a negative composite electrode with a thickness of 100 μm, a rolling ratio of 19%, and an electrode density of 1.38 g / cm 3 , compared with the conventional wet electrode, the rolling ratio is 11%, and the electrode density is 1.08g / cm 3 . In the composite electrode obtained by this method, the composite network formed by PTFE and CNT is respectively em...

example 3

[0033] Will LiNi 1 / 3 co 1 / 3 mn 1 / 3 o 2 , carbon airgel, additive S (metal-naphthalene complex), PVDF and conductive carbon black are mixed at a ratio of 30:58:1:5:6, and mixed at a high speed for 1h to form a positive electrode dry powder; the obtained mixed powder is passed through a powder press In the case of 5t-40t, it is pressed into a continuous positive dry electrode film with a thickness of 130 μm; On the front and back of the 20μm thick corroded aluminum foil, evenly apply a 3μm thick conductive adhesive by dip coating, place the dry electrode film with the same width as the above conductive adhesive layer on the conductive adhesive, and pass it through a hot roller. The composite film is thinned and pressed tightly on the porous aluminum foil to obtain a positive composite electrode with a thickness of 250 μm, a rolling ratio of 18%, and an electrode density of 1.35 g / cm 3 , compared with the conventional wet electrode, the rolling ratio is 10%, and the electrode...

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Abstract

The invention relates to a method for preparing a battery capacitor composite electrode by a dry method. The method comprises the following steps of weighing composite electrode raw materials which comprise an A type active material, a B type active material, binder dry powder and a conductive agent, fully mixing the composite electrode raw materials, heating to 500-580 DEG C in nitrogen and / or argon inert atmosphere, performing high-temperature calcining at the temperature for 2-8h, and then cooling to room temperature, wherein the flowing speed of the inert gas is 200-280ml / min and the temperature rising speed is 4-9 DEG C / min; preparing the mixed composite electrode raw materials into a dry electrode film through extrusion; and coating the surface of a current collector with a conductive glue layer with thickness of 1-10[mu]m to obtain a conductive coating layer, pasting the prepared dry electrode film on the conductive coating layer, and grinding to obtain the battery capacitor composite electrode. The battery capacitor composite electrode is prepared by the dry method, so that the process is simple, any water content is not required, the electrode compaction density of the battery capacitor is improved, and the energy density and the cycle life of a device are improved and prolonged.

Description

technical field [0001] The invention relates to a dry method for preparing composite electrodes for battery capacitors. Background technique [0002] Supercapacitors and lithium-ion batteries are two of the most popular energy storage devices on the market today. Lithium-ion battery is a green secondary battery with high energy density, high average output voltage, low self-discharge and no toxic substances. The energy density is 100Wh / kg to 150Wh / kg, and the maximum working voltage can reach 4V. Supercapacitor is an energy storage device based on the principle of electric double layer energy storage and the principle of redox quasi-capacitance with high reversibility. It has the advantages of high power density, short charge and discharge time, long cycle life, and wide operating temperature range. Disadvantages such as relatively low energy density. [0003] The difference in specific energy and specific power between lithium-ion batteries and supercapacitors determines ...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): H01M4/139H01M4/04B82Y30/00
CPCB82Y30/00H01M4/0435H01M4/139Y02E60/10
Inventor 阮殿波袁峻傅冠生乔志军周洲黄益杨斌
Owner NINGBO CRRC NEW ENERGY TECH CO LTD