A kind of preparation method of drug carrier with double response of magnetic-ph value
A dual-response, drug-based technology, applied in the direction of non-active ingredient medical preparations, active ingredient-containing medical preparations, pharmaceutical formulations, etc., can solve the problems of limited clinical application and low bioavailability of hydrophobic drugs, and achieve cost The effect of low cost and simple preparation method
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Embodiment 1
[0049] Preparation of Fe by Chemical Co-precipitation 3 o 4 Nanoparticles. Will Fe 2+ and Fe 3+ Mix according to the ratio of 1:2, add excess ammonia water, stir at a certain temperature (about 50°C) for 30 minutes, separate and precipitate with a magnet, wash with 0.5% ammonia water, and precipitate, add appropriate amount of deionized water and 0.5g polyethylene glycol, Ultrasonic mixing, heating and aging at 80°C for 30 min (600 r / min), repeated washing with deionized water, to obtain black ferrofluid 3 o 4 The nanoparticles were put into hydrochloric acid solution (0.1M), dispersed by ultrasonic, and washed three times with deionized water. Preparation of SiMNP composite nanoparticles. Take 0.01g clean Fe 3 o 4 Nanoparticles, put into 100ml ethanol solution (the volume ratio of ethanol to deionized water is 4:1), stir mechanically, add 1ml ammonia water (25%) dropwise, then add 0.1ml tetraethyl orthosilicate dropwise, stir at room temperature for 12 h ; Apply a ma...
Embodiment 2
[0051] Preparation of CDMNP magnetic composite nanomaterials. Dissolve 2.5g of β-CD in 50ml of dimethylformamide, add 0.5g of sodium hydride, stir at room temperature for 15 min, filter to obtain a white transparent solution, add 4ml of KH-560, and stir at 90°C for 5h under nitrogen protection. Cool to room temperature to obtain modified β-CD; add 1g SiMNP, add dropwise 1.5ml ammonia water (25%), stir at room temperature for 12h, enrich and suck out with magnet, rinse with dimethylformamide, deionized water and ethanol three times in sequence, Vacuum-dried at 50°C for 12 h to obtain brown-black CDMNP magnetic composite nanomaterials.
Embodiment 3
[0053] Preparation of CDMNP-PEG-CD vectors. Take an appropriate amount of CDMNP magnetic composite nanoparticles, place them in 20% polyethylene glycol solution, and stir mechanically at room temperature for 24 hours; the product is enriched and sucked out, washed with water, and dried in vacuum to obtain CDMNP-PEG composite materials. Take 0.05g of CDMNP-PEG composite material, place in 0.5g of β-CD saturated solution of dimethylformamide, ultrasonic at room temperature for 10 min, and stand overnight at 4°C; Wash each once, centrifuge for 10 min (3200 r / min), and collect the precipitate by magnetic adsorption; this process is repeated 3 times to remove residual β-CD and CDMNP-PEG composites. The precipitate was vacuum-dried and stored for future use.
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