Graphene conductive additive for conductive ink and preparation method

A technology of conductive additives and conductive inks, applied in inks, applications, household appliances, etc., can solve problems such as the inability to form an effective conductive network, and achieve the effects of low cost, simple process, and stable conductivity

Inactive Publication Date: 2018-11-30
CHENDU NEW KELI CHEM SCI CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0009] Aiming at the defect that graphene cannot form an effective conductive network in ink medium, the present invention proposes a preparation method of graphene conductive additive for conductive ink

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0032] Embodiment 1 A kind of preparation method of the graphene conductive additive for conductive ink

[0033] Follow these steps:

[0034]a. Add graphene oxide into water, ultrasonically disperse to obtain graphene oxide dispersion, then add isocyanate oligomer and silane, heat up to 60°C, then add ammonia water, absolute ethanol and reducing agent, mix and pass through sol-gel Graphene-doped SiO 2 Gel; Wherein, the weight ratio of graphene oxide and water is 1:150; The weight ratio of graphene oxide, isocyanate oligomer and silane is 3:80:20; Ammonia, absolute ethanol, reducing agent and graphene oxide The weight ratio is 40:80:0.1:1; The reducing agent used is hydrazine hydrate; Silane is trimethylchlorosilane;

[0035] The preparation method of the isocyanate oligomer is: adding trimethylolpropane to acetone, raising the temperature to 60°C, and then adding dibutyltin dilaurate; when the temperature rises to 65°C, adding hexamethylene diisocyanate, continuing Raise th...

Embodiment 2

[0037] Embodiment 2 A kind of preparation method of the graphene conductive additive for conductive ink

[0038] Follow these steps:

[0039] a. Add graphene oxide into water, ultrasonically disperse to obtain graphene oxide dispersion, then add isocyanate oligomer and silane, heat up to 60°C, then add ammonia water, absolute ethanol and reducing agent, mix and pass through sol-gel Graphene-doped SiO 2 Gel; Wherein, the weight ratio of graphene oxide and water is 1:200; The weight ratio of graphene oxide, isocyanate oligomer and silane is 4:80:20; Ammonia, dehydrated alcohol, reducing agent and graphene oxide The weight ratio is 40:85:0.1:1. The reducing agent used is hydrazine hydrate; Silane is triethylchlorosilane;

[0040] The preparation method of the isocyanate oligomer is: adding trimethylolpropane to acetone, raising the temperature to 60°C, and then adding dibutyltin dilaurate; when the temperature rises to 65°C, adding hexamethylene diisocyanate, continuing Raise...

Embodiment 3

[0042] Embodiment 3 A kind of preparation method of graphene conductive additive for conductive ink

[0043] Follow these steps:

[0044] a. Add graphene oxide into water, ultrasonically disperse to obtain graphene oxide dispersion, then add isocyanate oligomer and silane, heat up to 60°C, then add ammonia water, absolute ethanol and reducing agent, mix and pass through sol-gel Graphene-doped SiO 2 Gel; Wherein, the weight ratio of graphene oxide and water is 1:300; The weight ratio of graphene oxide, isocyanate oligomer and silane is 3:90:20; Ammonia, dehydrated alcohol, reducing agent and graphene oxide The weight ratio is 40:90:0.1:1. The reducing agent used is hydrazine hydrate; Silane is phenyl dimethyl chlorosilane;

[0045] The preparation method of the isocyanate oligomer is: adding trimethylolpropane to acetone, raising the temperature to 60°C, and then adding dibutyltin dilaurate; when the temperature rises to 65°C, adding hexamethylene diisocyanate, continuing R...

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Abstract

The invention relates to a graphene conductive additive for conductive ink and a preparation method, and belongs to the field of graphene conductive ink. The preparation method of the graphene conductive additive for the conductive ink comprises the following steps: a, adding graphene oxide in water, carrying out ultrasonic dispersion, then adding an isocyanate oligomer and silane, rising the temperature to 60 to 100 DEG C, then adding ammonia hydroxide, anhydrous ethanol and a reducing agent and mixing, thus obtaining graphene doped SiO2 gel through a sol-gel method; b, carrying out suction filtration on the graphene doped SiO2 gel, rising the temperature, and roasting for removing organic components, thus obtaining graphene loaded SiO2 microspheres of a three-dimensional porous structure; obtaining the graphene conductive additive, which is of a complete three-dimensional conductive network structure, for the conductive ink. The graphene conductive additive for the conductive ink, prepared by adopting the preparation method, is more stable in conductivity.

Description

technical field [0001] The invention relates to a graphene conductive additive for conductive ink and a preparation method, belonging to the field of graphene conductive ink. Background technique [0002] Conductive inks play a vital role in the fabrication of various conventional and flexible electronic devices. Traditional conductive inks are inks composed of gold, silver, copper powder or other metal powders or carbon powders and binders, which have high cost, complicated process, unstable resistivity, high molding and curing temperature, and easy oxidation and migration of metal particles. and other shortcomings. [0003] The Chinese patent application number 201310110327.X discloses a conductive ink, a transparent conductor and a preparation method thereof. The invention relates to a conductive ink, a transparent conductor and a preparation method thereof. The conductive ink comprises 50-90 parts of a metal conductive agent, 10-40 parts of a polymer resin, and 0.1-10 ...

Claims

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Application Information

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IPC IPC(8): C09D11/52
CPCC09D11/52
Inventor陈庆昝航
OwnerCHENDU NEW KELI CHEM SCI CO LTD