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Recovery of modifier compounds and polar organic compounds from a poly (arylene sulfide)

A polyarylene sulfide and organic compound technology, applied in the preparation of organic compounds, preparation of hydroxyl compounds, separation/purification of carboxylic acid compounds, etc., can solve high production costs, high costs, high raw materials and waste treatment costs And other issues

Inactive Publication Date: 2002-10-30
SOLVAY SA
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

First, in quenching and flashing P(AS) processes, regulators used to synthesize high molecular weight P(AS) can only be used once in these processes and cannot be captured and used in subsequent processes
This constitutes a high production cost of P(AS) due to higher raw material and waste disposal costs
Second, the POC used in this process can be recycled, but the cost is high
When running a hexanol extraction system, 30-40 pounds of n-hexanol needs to be processed for every pound of P(AS) produced, which results in high equipment and operating costs

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0067] The following examples illustrate that methanol can be separated from NMP by fractional distillation.

[0068] 75 grams of methanol and 75 grams of NMP (Fisher purity grade) were added to a 250 mL round bottom flask containing the azeotrope chips. The flask was connected to a vacuum jacketed fractionation column. The round bottom flask was heated with a heating mantle, and the vacuum jacketed fractionation column was slowly heated due to internal reflux. Vapor begins to flow through the condenser and into the receiver, producing an overhead liquid stream. The flow of steam was slow until the temperature of the fractionation column increased with further heating of the round bottom flask. Once the boiling point of NMP is reached, the flow of the overhead liquid stream continues again. The vacuum jacketed fractionation column was then cooled to room temperature. The round bottom flask was then turned off from heating.

[0069] Fractions of the overhead liquid stream ...

Embodiment 2

[0072] This example illustrates that the recycle mixture can be separated to form methanol and a recycle feed mixture.

[0073] Take 504.20cm 3 Continuous speed per hour A recycle mixture containing 78.03 wt% NMP, 15.90 wt% methanol and 6.07 wt% sodium acetate was fed to a laboratory continuous still. A small amount of NMP was added to the still at the beginning. The still was heated until the recycle mixture began to reflux, at which point the still had a temperature of about 210°C and the temperature of the entire column was about 66-208°C. Make the overhead stream enter the overhead condenser through the overhead deflector, and then enter the overhead receiver to recover the methanol stream. The tower top deflector is designed to collect for 0.2 minutes and discharge to the top receiver for 5 seconds. The circulating raw material mixture is 87.40cm 3 / hr pumped from the still. After about 1 hour, a sample of the methanol stream was collected and a recycle feed mixture ...

Embodiment 3

[0078] This example demonstrates that the addition of water to the recycle mixture helps prevent the accumulation of sodium acetate at the bottom of the still.

[0079] The same process steps as in Example 2 were used except that the recycle mixture contained 14.60 wt% methanol, 72.00 wt% NMP, 4.60 wt% sodium acetate and 8.8 wt% water. The temperature of the distiller is about 190-198°C, and the temperature of the whole column is about 68-102°C. The tower top deflector is designed to collect for 0.3 minutes and discharge to the top receiver for 5 seconds.

[0080] Samples of the methanol stream and recycle feed mixture were collected after 8.66 hours of distillation and analyzed by gas chromatography. The recycled feed mixture contained 97.53 wt% NMP, 0.00 wt% methanol, 1.63 wt% water and 0.16 wt% other compounds. The methanol stream contained 97.36 wt% methanol, 0.03 wt% NMP, 2.60 wt% water and 0.02 wt% other compounds. Negligible precipitation of sodium acetate at the bot...

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PUM

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Abstract

A process is provided to recover at least one modifier compound and at least one polar organic compound from a P(AS) recycle mixture.

Description

field of invention [0001] The field to which the present invention relates is the recovery of at least one regulator compound and at least one polar organic compound from polyarylene sulfide recycle mixtures. In the description of the present application, at least one polar organic compound is referred to as POC, and polyarylene sulfide is referred to as P(AS). Background of the invention [0002] The production of P(AS) has been used industrially and commercially for a long time. P(AS) can be molded into various articles including but not limited to parts, films and fibers using techniques such as injection molding and extrusion. These articles can be used in various fields requiring heat and chemical resistance. For example, P(AS) can be used as a material for the preparation of electrical and electronic components and automobile parts. [0003] In general, P(AS) can be prepared by contacting reactants comprising at least one dihaloaromatic comp...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C07D207/267C07C29/80C07C31/04C07C51/43C07C53/10C07C319/14C07C321/30C08G75/02C08J11/00
CPCC08G75/0281C07D207/267C08J11/02Y02W30/52
Inventor J·S·佛多J·F·盖贝尔F·C·小维达里
Owner SOLVAY SA