Metal oxide particles containing titanium oxide coated with silicon dioxide-stannic oxide complex oxide
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[0139]The present invention will be further described in detail with reference to the following examples. The present invention, however, is not limited to the examples
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Preparation Example 1
[0140]A water dispersion sol of titanium oxide-containing core particles (A1) was prepared based on Example 2 in Japanese Patent Application Publication No. H10-245224 (JP H10-245224 A).
[0141]Process (a): Into a 3-liter separable flask made of glass with a jacket, 293.8 g (79.8 g in terms of TiO2) of titanium tetrachloride (manufacture by Sumitomo Sitix Co., Ltd., a concentration of 27.2% by mass in terms of TiO2, Cl 32.0% by mass) and 371.6 g of water were poured to prepare 665 g of titanium chloride aqueous solution (12.0% by mass in terms of TiO2). Stirred with a stirring bar made of glass, the aqueous solution was heated to 50° C. and thereafter, 950.8 g of 35% by mass hydrogen peroxide aqueous solution and 566.4 g of metal tin powder (manufactured by Yamaishi Metal Co., Ltd., trade name AT-Sn, No. 200) were added with cooling. The addition of the hydrogen peroxide aqueous solution and the metal tin powder was performed such that first 31.5 g (0.265 mol) of ...
preparation example 2
[0145]A water dispersion sol of titanium oxide-containing core particles (A2) was prepared based on Example 2 in Japanese Patent Application Publication No. H10-310429 (JP H10-310429 A).
[0146]Process (a): Into a 3-liter separable flask made of glass with a jacket, 587.5 g (159.8 g in terms of TiO2) of titanium tetrachloride (27.2% by mass in terms of TiO2, Cl 32.0% by mass, manufacture by Sumitomo Sitix Co., Ltd.), 114.6 g (49.2 g in terms of ZrO2) of zirconium oxycarbonate and (43.0% by mass in terms of ZrO2), manufactured by Daiichi Kigenso Kagaku Kogyo Co., Ltd), and 629.6 g of water were poured to prepare 1331.7 g of a mixed aqueous solution of titanium chloride and zirconium oxychloride (12.0% by mass in terms of TiO2, 3.7% by mass in terms of ZrO2). Stirred with a stirring bar made of glass, the aqueous solution was heated to 60° C., and thereafter, 358.0 g of 35% by mass hydrogen, peroxide aqueous solution and 190.0 g of metal tin powder (manufactured by Yamaishi Metal Co., L...
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