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Method for preparing bimetal solid catalyst for biodiesel synthesis

A solid catalyst, biodiesel technology, applied in organic compound/hydride/coordination complex catalysts, physical/chemical process catalysts, chemical instruments and methods, etc., can solve the problems of high reaction temperature, long reaction time, reduction of , to achieve the effect of high efficiency, strong tolerance and simple process

Inactive Publication Date: 2011-05-18
GUANGZHOU INST OF ENERGY CONVERSION - CHINESE ACAD OF SCI
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

At the same time, the existing solid acid catalysts have high reaction temperature and long reaction time, and the reaction product water will reduce or even hinder the activity of the catalyst. The acid value of the oil is reduced to a lower level

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Solution 1: 0.02mol K4Fe(CN)6·3H2O was dissolved in 80ml double distilled water to prepare 0.25mol / l solution 1.

[0018] Solution 2: Dissolve 0.2 mol metal chloride salt (ZnCl2) in 20 ml tert-butanol and 20 ml double distilled water (add a small amount of HCl to avoid flocculent precipitation) to prepare 5 mol / l solution 2.

[0019] Solution 3: Dissolve 30 g of polyethylene glycol 4000 in 4 ml of water and 80 ml of tert-butanol at a ratio of 30:4:80 (g / ml / ml).

[0020] The solution 1 obtained above was slowly added dropwise to the solution 2 at 323K to form a precipitate, and magnetic stirring was carried out at the same time. Then solution 3 was added within 5-10 min, and stirring was continued for 2 h. filter. Wash 3-5 times with water (500ml of water each time). 313K vacuum drying to obtain a bimetallic solid catalyst.

[0021] The catalytic activity of the bimetallic solid catalyst was evaluated using rapeseed oil containing 10wt% free fatty acid and 10wt% mois...

Embodiment 2

[0026] Solution 1: 0.015mol K4Fe(CN)6·3H2O was dissolved in 60ml double distilled water to prepare 0.25mol / l solution 1.

[0027] Solution 2: Dissolve 0.2 mol metal chloride salt (ZnCl2) in 40 ml tert-butanol and 40 ml double distilled water (add a small amount of HCl to avoid flocculent precipitation) to prepare 5 mol / l solution 2.

[0028] Solution 3: Dissolve 20 g of polyethylene glycol 4000 in 4 ml of water and 60 ml of tert-butanol at a ratio of 20:4:60 (g / ml / ml).

[0029] The solution 1 obtained above was slowly added dropwise to the solution 2 at 323K to form a precipitate, and magnetic stirring was carried out at the same time. Then solution 3 was added within 5-10 min, and stirring was continued for 2 h. filter. Wash 3-5 times with water (500ml of water each time). 313K vacuum drying to obtain a bimetallic solid catalyst.

[0030] The catalytic activity of the bimetallic solid catalyst was evaluated using rapeseed oil containing 10wt% free fatty acid and 10wt% moi...

Embodiment 3

[0035] Solution 1: 0.025mol K4Fe(CN)6·3H2O was dissolved in 100ml double distilled water to prepare 0.25mol / l solution 1.

[0036] Solution 2: Dissolve 0.4 mol metal chloride salt (ZnCl2) in 20 ml tert-butanol and 20 ml double distilled water (add a small amount of HCl to avoid flocculent precipitation) to prepare 5 mol / l solution 2.

[0037] Solution 3: Dissolve 60 g of polyethylene glycol 4000 in 4 ml of water and 100 ml of tert-butanol at a ratio of 60:4:100 (g / ml / ml) to obtain 120 ml of a solution.

[0038] The solution 1 obtained above was slowly added dropwise to the solution 2 at 323K to form a precipitate, and magnetic stirring was carried out at the same time. Then add solution 3 within 5-l0min and continue stirring for 2h. filter. Wash 3-5 times with water (500ml of water each time). 313K vacuum drying to obtain a bimetallic solid catalyst.

[0039] The catalytic activity of the bimetallic solid catalyst was evaluated using rapeseed oil containing 10wt% free fatt...

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PUM

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Abstract

The invention provides a method for preparing bimetal solid catalyst for biodiesel synthesis, which comprises the following steps: (1) dissolving K4Fe(CN)6.3H2O into double-distilled water to prepare 0.25 mol / l of solution I; dissolving ZnCl2 into tertiary butanol and the double-distilled water with equal volume ratio, adding a small amount of HCl to prevent flocculent sediments and preparing 5 mol / l of solution II; dissolving polyethylene glycol 4000 into water and the tertiary butanol in a certain proportion of 30:4:80 g / ml / ml and preparing solution III; (2) dropwise adding the solution II into the solution I slowly in the volume ratio of the solution I: the solution II: the solution III of 60-100:40-80:60-120 at the temperature of 323K to generate sediments and stirring; then adding the solution III in 5-10 minutes and continuously stirring for two hours; filtering, washing by the water and drying in vacuum of 313K to acquire the bimetal solid catalyst. The method has simple process and high efficiency. Compared with the traditional solid acid-base catalyst, the catalyst prepared by the invention has functions of solid acid catalyst and solid base catalyst and can carry out catalytic esterification reaction and ester exchange reaction synchronously, and the catalyst has high tolerance on water.

Description

technical field [0001] The invention relates to the technical field of chemistry and chemical engineering, in particular to a preparation method of a bimetallic solid catalyst used for biodiesel synthesis. technical background [0002] Solid acid and solid base have been developed in the field of chemical catalysis for a long time. Due to the requirements of biodiesel green conversion technology, in recent years, people have begun to study the application of solid acid and base in biodiesel conversion technology. [0003] A solid base is a solid that donates electrons to the reactants. As a catalyst, its active center has a very strong ability to donate or accept electrons, and it has a surface anion hole, that is, the free electron center is formed by the surface O 2 - or O 2 - -OH (composition. The solid bases used for biodiesel conversion studied at home and abroad include: alkali metal and alkaline earth metal oxide types, including: MgO, CaO, SrO, BaO, Na 2 O, K 2...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J31/26B01J31/06C11C3/10C11C3/04
CPCY02E50/13Y02E50/10
Inventor 吕鹏梅颜芳袁振宏罗文王忠铭李惠文
Owner GUANGZHOU INST OF ENERGY CONVERSION - CHINESE ACAD OF SCI