Aqueous composite resin composition, coating agent containing the same, and multilayer body using the coating agent
A composite resin and composition technology, applied in the direction of synthetic resin layered products, coatings, adhesive types, etc., can solve problems such as deterioration of plastic substrates, and achieve excellent durability, weather resistance, and excellent rust resistance. Effect
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[0178] Next, the present invention will be described more specifically by way of examples and comparative examples.
Synthetic example 1
[0179] Synthesis Example 1 [Preparation Example of Methyltrimethoxysilane Condensate (a3'-1)]
[0180] In a reaction vessel equipped with a stirrer, a thermometer, a dropping funnel, a condenser, and a nitrogen inlet, 1421 parts by mass of methyltrimethoxysilane (MTMS) was fed, and the temperature was raised to 60°C.
[0181] Next, a mixture of 0.17 parts by mass of "A-3" [isopropyl acid phosphate manufactured by Sakai Chemical Co., Ltd.] and 207 parts by mass of deionized water was dropped in the reaction vessel for 5 minutes, and then the ℃ temperature for 4 hours to carry out hydrolysis condensation reaction.
[0182] The condensate obtained by the hydrolysis-condensation reaction is subjected to a temperature of 40-60° C. and a reduced pressure of 300-10 mmHg (referring to the condition that the reduced pressure at the beginning of methanol distillation is 300 mmHg and the final reduced pressure is 10 mmHg. The following are the same.) Distillation, and methanol and water...
Synthetic example 2
[0184] Synthesis Example 2 [Preparation Example of Ethyltrimethoxysilane Condensate (a3'-2)]
[0185] In a reaction vessel equipped with a stirrer, a thermometer, a dropping funnel, a condenser, and a nitrogen inlet, 1296 parts by mass of ethyltrimethoxysilane (ETMS) was fed, and the temperature was raised to 60°C.
[0186] Next, a mixture of 0.14 parts by mass of "A-3" [isopropyl acid phosphate manufactured by Sakai Chemical Co., Ltd.] and 171 parts by mass of deionized water was dropped in the reaction vessel for 5 minutes, and then the ℃ temperature for 4 hours to carry out hydrolysis condensation reaction.
[0187] Distill the condensate obtained by the hydrolysis and condensation reaction at a temperature of 40 to 60°C and a reduced pressure of 300 to 10 mmHg, and remove the generated methanol and water, thereby obtaining ethyltrimethylmethanol with a number average molecular weight of 1100 1000 parts by mass of a liquid mixture (70 mass % of active ingredient) of the co...
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